Tin(IV) Sulfide Greatly Improves the Catalytic Performance of UiO-66 for Carbon Dioxide Cycloaddition
文献类型：期刊论文
| 作者 | Cheng, Xiuyan1,2; Zhang, Bingxing1,2; Shi, Jinbiao1,2; Zhang, Jianling1,2,3; Zheng, Lirong3; Zhang, Jing; Shao, Dan1,2; Tan, Xiuniang1,2; Han, Buxing1,2; Yang, Guanying1,2 |
| 刊名 | CHEMCATCHEM
 |
| 出版日期 | 2018-07-19 |
| 卷号 | 10期号:14页码:2945-2948 |
| 关键词 | Cycloaddition Heterogeneous Catalysis Metal-organic Frameworks Nanoparticles Tin Sulfide |
| ISSN号 | 1867-3880 |
| DOI | 10.1002/cctc.201800411 |
| 英文摘要 | To overcome the limitations of metal-organic frameworks (MOFs) for catalysis (e.g., low catalytic activities resulting from blockage of the active metal centers by organic linkers) is of great importance. Herein, we demonstrate the formation of UiO-66 nanoparticles with ultrasmall size and linker defects with the aid of SnS2 nanosheets. The UiO-66 nanoparticles supported by SnS2 nanosheets were found to exhibit excellent catalytic activity for the cycloaddition reaction of CO2 with propylene oxide under solvent-free and co-catalyst-free conditions. Outstandingly, the catalytic activity was 11times higher than that of the pure UiO-66 catalyst under optimum conditions. We thus provide a promising route to modify MOF particles thus to promote their catalytic performance. |
| 语种 | 英语 |
| WOS记录号 | WOS:000439756600003 |
| 出版者 | WILEY-V C H VERLAG GMBH |
| 源URL | [http://ir.iccas.ac.cn/handle/121111/42269]  |
| 专题 | 中国科学院化学研究所 |
| 通讯作者 | Zhang, Jianling |
| 作者单位 | 1.Chinese Acad Sci, Inst Chem, CAS Key Lab Colloid Interface & Chem Thermodynam, Beijing 100190, Peoples R China 2.Univ Chinese Acad Sci, Sch Chem & Chem Engn, Beijing 100049, Peoples R China 3.Chinese Acad Sci, Inst High Energy Phys, BSRF, Beijing 100049, Peoples R China |
| 推荐引用方式 GB/T 7714 | Cheng, Xiuyan,Zhang, Bingxing,Shi, Jinbiao,et al. Tin(IV) Sulfide Greatly Improves the Catalytic Performance of UiO-66 for Carbon Dioxide Cycloaddition[J]. CHEMCATCHEM,2018,10(14):2945-2948. |
| APA | Cheng, Xiuyan.,Zhang, Bingxing.,Shi, Jinbiao.,Zhang, Jianling.,Zheng, Lirong.,...&Yang, Guanying.(2018).Tin(IV) Sulfide Greatly Improves the Catalytic Performance of UiO-66 for Carbon Dioxide Cycloaddition.CHEMCATCHEM,10(14),2945-2948. |
| MLA | Cheng, Xiuyan,et al."Tin(IV) Sulfide Greatly Improves the Catalytic Performance of UiO-66 for Carbon Dioxide Cycloaddition".CHEMCATCHEM 10.14(2018):2945-2948. |
入库方式： OAI收割
来源：化学研究所
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