Planar FAPbBr(3) Solar Cells with Power Conversion Efficiency above 10%
文献类型:期刊论文
作者 | Zhang, Yongfei1; Liang, Yongqi1; Wang, Yajuan1; Guo, Fengwan2; Sun, Licheng1,3; Xu, Dongsheng2 |
刊名 | ACS ENERGY LETTERS |
出版日期 | 2018-08-01 |
卷号 | 3期号:8页码:1808-1814 |
ISSN号 | 2380-8195 |
DOI | 10.1021/acsenergylett.8b00540 |
英文摘要 | Bromide-based hybrid perovskites are of particular interest not only due to the fact that they offer a way to go beyond the Shockley-Queisser limit via the tandem cell scheme but single junction devices of them can also achieve reasonably high efficiency with high stability for solar energy conversion. However, the highest power conversion efficiency achieved up to now for FAPbBr(3) single-junction solar cells is only 8.2%, which is far below the efficiency of-17% predicted from detailed balance analysis. Here, a two-step method (the intermolecule exchange pathway) was systematically optimized for the fabrication of high quality FAPbBr(3) films. A molecule of urea, structurally similar to formamidinium, is introduced as an additive to tune the intermolecular ion exchange procedure. SnO2 is introduced as an electron-selective contact to the planar structured FAPbBr(3) solar cells. As a result, a power conversion efficiency of 10.61% and a V-oc of 1.56 V are achieved with planar structured solar cells, both of which represent the highest value ever reported for FAPbBr(3) solar cells. |
语种 | 英语 |
出版者 | AMER CHEMICAL SOC |
WOS记录号 | WOS:000441852800005 |
源URL | [http://ir.iccas.ac.cn/handle/121111/42335] |
专题 | 中国科学院化学研究所 |
通讯作者 | Liang, Yongqi; Sun, Licheng; Xu, Dongsheng |
作者单位 | 1.DUT, DUT KTH Joint Educ & Res Ctr Mol Devices, State Key Lab Fine Chem, Inst Artificial Photosynth, Dalian 116024, Peoples R China 2.Peking Univ, Beijing Natl Lab Mol Sci, State Key Lab Struct Chem Unstable & Stable Speci, Coll Chem & Mol Engn, Beijing 100871, Peoples R China 3.KTH Royal Inst Technol, Sch Chem Sci & Engn, Dept Chem, S-10044 Stockholm, Sweden |
推荐引用方式 GB/T 7714 | Zhang, Yongfei,Liang, Yongqi,Wang, Yajuan,et al. Planar FAPbBr(3) Solar Cells with Power Conversion Efficiency above 10%[J]. ACS ENERGY LETTERS,2018,3(8):1808-1814. |
APA | Zhang, Yongfei,Liang, Yongqi,Wang, Yajuan,Guo, Fengwan,Sun, Licheng,&Xu, Dongsheng.(2018).Planar FAPbBr(3) Solar Cells with Power Conversion Efficiency above 10%.ACS ENERGY LETTERS,3(8),1808-1814. |
MLA | Zhang, Yongfei,et al."Planar FAPbBr(3) Solar Cells with Power Conversion Efficiency above 10%".ACS ENERGY LETTERS 3.8(2018):1808-1814. |
入库方式: OAI收割
来源:化学研究所
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