Controlled Growth of MoS2 Nanosheets on 2D N-Doped Graphdiyne Nanolayers for Highly Associated Effects on Water Reduction
文献类型：期刊论文
| 作者 | Yu, Huidi1,2; Xue, Yurui1,2; Hui, Lan1,2; Zhang, Chao1,2; Zhao, Yingjie3; Li, Zhibo3; Li, Yuliang1,2 |
| 刊名 | ADVANCED FUNCTIONAL MATERIALS
 |
| 出版日期 | 2018-05-09 |
| 卷号 | 28期号:19 |
| 关键词 | Heterostructures Hydrogen Generation Molybdenum Disulfide Nitrogen-doped Graphdiyne Water Splitting |
| ISSN号 | 1616-301X |
| DOI | 10.1002/adfm.201707564 |
| 英文摘要 | The first utilization of nitrogen-doped graphdiyne (NGDY) as an efficient catalytic promoter for hydrogen evolution reaction (HER) is reported. X-ray powder diffraction and X-ray photoelectron spectroscopy studies indicate the presence of strong interactions between NGDY and MoS2, which should effectively facilitate the charge transport behavior and improvement of the HER kinetics. The creative hybridization of MoS2 and NGDY endows such heterostructure with structural and compositional advantages for boosting the catalytic activity (low overpotential of 186 mV at 10 mA cm(-2) and Tafel slope of 63 mV dec(-1)) and extraordinary stability (higher than all reported MoS2-based materials and even better than that of commercial Pt and almost all benchmarked electrocatalysts). All of the results not only demonstrate that NGDY can be used as an effective catalytic promoter for hydrogen production, but also provide new strategy for fabricating efficient watersplitting electrodes. |
| 语种 | 英语 |
| WOS记录号 | WOS:000431615300019 |
| 出版者 | WILEY-V C H VERLAG GMBH |
| 源URL | [http://ir.iccas.ac.cn/handle/121111/43151]  |
| 专题 | 中国科学院化学研究所 |
| 通讯作者 | Xue, Yurui; Li, Yuliang |
| 作者单位 | 1.Chinese Acad Sci, Inst Chem, Beijing 100190, Peoples R China 2.Univ Chinese Acad Sci, Beijing 100049, Peoples R China 3.Qingdao Univ Sci & Technol, Sch Polymer Sci & Engn, Qingdao 266042, Peoples R China |
| 推荐引用方式 GB/T 7714 | Yu, Huidi,Xue, Yurui,Hui, Lan,et al. Controlled Growth of MoS2 Nanosheets on 2D N-Doped Graphdiyne Nanolayers for Highly Associated Effects on Water Reduction[J]. ADVANCED FUNCTIONAL MATERIALS,2018,28(19). |
| APA | Yu, Huidi.,Xue, Yurui.,Hui, Lan.,Zhang, Chao.,Zhao, Yingjie.,...&Li, Yuliang.(2018).Controlled Growth of MoS2 Nanosheets on 2D N-Doped Graphdiyne Nanolayers for Highly Associated Effects on Water Reduction.ADVANCED FUNCTIONAL MATERIALS,28(19). |
| MLA | Yu, Huidi,et al."Controlled Growth of MoS2 Nanosheets on 2D N-Doped Graphdiyne Nanolayers for Highly Associated Effects on Water Reduction".ADVANCED FUNCTIONAL MATERIALS 28.19(2018). |
入库方式： OAI收割
来源：化学研究所
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