Polythiophene-Peptide Biohybrid Assemblies for Enhancing Photoinduced Hydrogen Evolution
文献类型：期刊论文
| 作者 | Lu, Huan1; Zhou, Chengcheng1; Zhou, Xin1; Sun, Han1; Bai, Haotian1; Wang, Yunxia1; Lv, Fengting1; Liu, Libing1; Ma, Yuguo2,3; Wang, Shu1 |
| 刊名 | ADVANCED ELECTRONIC MATERIALS
 |
| 出版日期 | 2017-11-01 |
| 卷号 | 3期号:11 |
| 关键词 | Assemblies Hydrogen Evolution Peptides Photocatalysis Polythiophene |
| ISSN号 | 2199-160X |
| DOI | 10.1002/aelm.201700164 |
| 英文摘要 | The self-assembly of short peptide offers versatile processes for adjusting the ordered stacking of organic functional materials to enhance photoinduced electron transfer. Herein, this study presents the first demonstration of the use of A(16-22) peptide to prepare polythiophene/A(16-22) assemblies for a photocatalytic water splitting system. Isothermal titration microcalorimetry results show that the driving forces for polythiophene/A(16-22) assembly formation are electrostatic interactions, as well as hydrogen bonds and hydrophobic interactions. The assemblies accelerate the photoinduced electrons transfer from polythiophene upon light excitation and eventually enhance the hydrogen evolution. This work opens a new way into the development of biohybrid materials as novel photocatalytic water splitting platform for hydrogen evolution. |
| 语种 | 英语 |
| WOS记录号 | WOS:000416047700011 |
| 出版者 | WILEY |
| 源URL | [http://ir.iccas.ac.cn/handle/121111/45079]  |
| 专题 | 中国科学院化学研究所 |
| 通讯作者 | Lv, Fengting; Ma, Yuguo; Wang, Shu |
| 作者单位 | 1.Chinese Acad Sci, Inst Chem, Beijing Natl Lab Mol Sci, Beijing 100190, Peoples R China 2.Peking Univ, Beijing Natl Lab Mol Sci, Ctr Soft Matter Sci & Engn, Coll Chem,Minist Educ, Beijing 100871, Peoples R China 3.Peking Univ, Minist Educ, Key Lab Polymer Chem & Phys, Coll Chem, Beijing 100871, Peoples R China |
| 推荐引用方式 GB/T 7714 | Lu, Huan,Zhou, Chengcheng,Zhou, Xin,et al. Polythiophene-Peptide Biohybrid Assemblies for Enhancing Photoinduced Hydrogen Evolution[J]. ADVANCED ELECTRONIC MATERIALS,2017,3(11). |
| APA | Lu, Huan.,Zhou, Chengcheng.,Zhou, Xin.,Sun, Han.,Bai, Haotian.,...&Wang, Shu.(2017).Polythiophene-Peptide Biohybrid Assemblies for Enhancing Photoinduced Hydrogen Evolution.ADVANCED ELECTRONIC MATERIALS,3(11). |
| MLA | Lu, Huan,et al."Polythiophene-Peptide Biohybrid Assemblies for Enhancing Photoinduced Hydrogen Evolution".ADVANCED ELECTRONIC MATERIALS 3.11(2017). |
入库方式： OAI收割
来源：化学研究所
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