中国科学院机构知识库网格
Chinese Academy of Sciences Institutional Repositories Grid
Facile Two-Step Synthesis of All-Inorganic Perovskite CsPbX3 (X = Cl, Br, and I) Zeolite-Y Composite Phosphors for Potential Backlight Display Application

文献类型:期刊论文

作者Sun, Jia-Yi1,2; Rabouw, Freddy T.3; Yang, Xian-Feng4; Huang, Xie-Yi1,2; Jing, Xi-Ping5; Ye, Shi1,2; Zhang, Qin-Yuan1,2
刊名ADVANCED FUNCTIONAL MATERIALS
出版日期2017-12-01
卷号27期号:45
ISSN号1616-301X
关键词Encapsulation Light-emitting Diodes Perovskite Quantum Dots Zeolites
DOI10.1002/adfm.201704391
英文摘要Recently developed CsPbX3 (X = Cl, Br, and I) perovskite quantum dots (QDs) hold great potential for various applications owing to their superior optical properties, such as tunable emissions, high quantum efficiency, and narrow linewidths. However, poor stability under ambient conditions and spontaneous ion exchange among QDs hinder their application, for example, as phosphors in white-light-emitting diodes (WLEDs). Here, a facile two-step synthesis procedure is reported for luminescent and color-tunable CsPbX3-zeolite-Y composite phosphors, where perovskite QDs are encapsulated in the porous zeolite matrix. First zeolite-Y is infused with Cs+ ions by ion exchange from an aqueous solution and then forms CsPbX3 QDs by diffusion and reaction with an organic solution of PbX2. The zeolite encapsulation reduces degradation and improves the stability of the QDs under strong illumination. A WLED is fabricated using the resulting microscale composites, with Commission Internationale de I'Eclairage (CIE) color coordinates (0.38, 0.37) and achieving 114% of National Television Standards Committee (NTSC) and 85% of the ITU-R Recommendation BT.2020 (Rec.2020) coverage.
语种英语
出版者WILEY-V C H VERLAG GMBH
WOS记录号WOS:000416828500022
源URL[http://ir.iccas.ac.cn/handle/121111/45133]  
专题中国科学院化学研究所
通讯作者Ye, Shi
作者单位1.South China Univ Technol, State Key Lab Luminescent Mat & Devices, Guangzhou 510641, Guangdong, Peoples R China
2.South China Univ Technol, Guangdong Prov Key Lab Fiber Laser Mat & Appl Tec, Guangzhou 510641, Guangdong, Peoples R China
3.Univ Utrecht, Debye Inst Nanomat Sci, Princetonplein 1, NL-3584 CC Utrecht, Netherlands
4.South China Univ Technol, Analyt & Testing Ctr, Guangzhou 510641, Guangdong, Peoples R China
5.Peking Univ, Beijing Natl Lab Mol Sci, State Key Lab Rare Earth Mat Chem & Applicat, Coll Chem & Mol Engn, Beijing 100871, Peoples R China
推荐引用方式
GB/T 7714
Sun, Jia-Yi,Rabouw, Freddy T.,Yang, Xian-Feng,et al. Facile Two-Step Synthesis of All-Inorganic Perovskite CsPbX3 (X = Cl, Br, and I) Zeolite-Y Composite Phosphors for Potential Backlight Display Application[J]. ADVANCED FUNCTIONAL MATERIALS,2017,27(45).
APA Sun, Jia-Yi.,Rabouw, Freddy T..,Yang, Xian-Feng.,Huang, Xie-Yi.,Jing, Xi-Ping.,...&Zhang, Qin-Yuan.(2017).Facile Two-Step Synthesis of All-Inorganic Perovskite CsPbX3 (X = Cl, Br, and I) Zeolite-Y Composite Phosphors for Potential Backlight Display Application.ADVANCED FUNCTIONAL MATERIALS,27(45).
MLA Sun, Jia-Yi,et al."Facile Two-Step Synthesis of All-Inorganic Perovskite CsPbX3 (X = Cl, Br, and I) Zeolite-Y Composite Phosphors for Potential Backlight Display Application".ADVANCED FUNCTIONAL MATERIALS 27.45(2017).

入库方式: OAI收割

来源:化学研究所

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