Supramolecular Radical Anions Triggered by Bacteria In Situ for Selective Photothermal Therapy
文献类型：期刊论文
| 作者 | Yang, Yuchong1; He, Ping2; Wang, Yunxia2; Bai, Haotian2; Wang, Shu2; Xu, Jiang-Fei1; Zhang, Xi1 |
| 刊名 | ANGEWANDTE CHEMIE-INTERNATIONAL EDITION
 |
| 出版日期 | 2017-12-18 |
| 卷号 | 56期号:51页码:16239-16242 |
| ISSN号 | 1433-7851 |
| 关键词 | Host-guest Systems Photothermal Therapy Radical Anions Supramolecular Chemistry |
| DOI | 10.1002/anie.201708971 |
| 英文摘要 | A supramolecular complex that can be selectively reduced to radical anions in situ by facultative anaerobic bacteria is reported. To this end, a water-soluble bifunctional monomer bearing perylene diimide was synthesized, and its supramolecular complex with cucurbit[7] uril was fabricated on the basis of host-guest complexation, which could be reduced to forming radical anions in the presence of E. coli. It was found that this supramolecular complex could display different ability of generating radical anions by facultative anaerobic and aerobic bacteria in terms of their various reductive abilities. The selective antibacterial activity of the supramolecular complex could be realized by the photothermal performance of the radical anions under near-infrared irradiation. It is anticipated that this method may lead to a novel bacteria-responsive photothermal therapy to regulate balance of bacterial flora. |
| 语种 | 英语 |
| 出版者 | WILEY-V C H VERLAG GMBH |
| WOS记录号 | WOS:000419399800017 |
| 源URL | [http://ir.iccas.ac.cn/handle/121111/45399]  |
| 专题 | 中国科学院化学研究所 |
| 通讯作者 | Xu, Jiang-Fei; Zhang, Xi |
| 作者单位 | 1.Tsinghua Univ, Dept Chem, Key Lab Organ Optoelect & Mol Engn, Beijing 100084, Peoples R China 2.Chinese Acad Sci, Inst Chem, Key Lab Organ Solids, Beijing 100190, Peoples R China |
| 推荐引用方式 GB/T 7714 | Yang, Yuchong,He, Ping,Wang, Yunxia,et al. Supramolecular Radical Anions Triggered by Bacteria In Situ for Selective Photothermal Therapy[J]. ANGEWANDTE CHEMIE-INTERNATIONAL EDITION,2017,56(51):16239-16242. |
| APA | Yang, Yuchong.,He, Ping.,Wang, Yunxia.,Bai, Haotian.,Wang, Shu.,...&Zhang, Xi.(2017).Supramolecular Radical Anions Triggered by Bacteria In Situ for Selective Photothermal Therapy.ANGEWANDTE CHEMIE-INTERNATIONAL EDITION,56(51),16239-16242. |
| MLA | Yang, Yuchong,et al."Supramolecular Radical Anions Triggered by Bacteria In Situ for Selective Photothermal Therapy".ANGEWANDTE CHEMIE-INTERNATIONAL EDITION 56.51(2017):16239-16242. |
入库方式： OAI收割
来源：化学研究所
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