Selective electroreduction of carbon dioxide to formic acid on electrodeposited SnO2@N-doped porous carbon catalysts
文献类型：期刊论文
| 作者 | Lu, Lu1,2; Sun, Xiaofu1,2; Ma, Jun1; Zhu, Qinggong1; Wu, Congyi1; Yang, Dexin1,2; Han, Buxing1,2 |
| 刊名 | SCIENCE CHINA-CHEMISTRY
 |
| 出版日期 | 2018-02-01 |
| 卷号 | 61期号:2页码:228-235 |
| ISSN号 | 1674-7291 |
| 关键词 | Co2 Reduction Electrocatalyst Ionic Liquid Porous Carbon Green Chemistry |
| DOI | 10.1007/s11426-017-9118-6 |
| 英文摘要 | Electrocatalytic reduction of CO2 is a promising route for energy storage and utilization. Herein we synthesized SnO2 nanosheets and supported them on N-doped porous carbon (N-PC) by electrodeposition for the first time. The SnO2 and N-PC in the SnO2@N-PC composites had exellent synergistic effect for electrocatalytic reduction of CO2 to HCOOH. The Faradaic efficiency of HCOOH could be as high as 94.1% with a current density of 28.4 mA cm(-2) in ionic liquid-MeCN system. The reaction mechanism was proposed on the basis of some control experiments. This work opens a new way to prepare composite electrode for electrochemical reduction of CO2. |
| 语种 | 英语 |
| 出版者 | SCIENCE PRESS |
| WOS记录号 | WOS:000424012300014 |
| 源URL | [http://ir.iccas.ac.cn/handle/121111/45481]  |
| 专题 | 中国科学院化学研究所 |
| 通讯作者 | Sun, Xiaofu; Han, Buxing |
| 作者单位 | 1.Chinese Acad Sci, Beijing Natl Lab Mol Sci, CAS Res Educ Ctr Excellence Mol Sci,Inst Chem, CAS Key Lab Colloid & Interface & Thermodynam, Beijing 100190, Peoples R China 2.Univ Chinese Acad Sci, Sch Chem & Chem Engn, Beijing 100049, Peoples R China |
| 推荐引用方式 GB/T 7714 | Lu, Lu,Sun, Xiaofu,Ma, Jun,et al. Selective electroreduction of carbon dioxide to formic acid on electrodeposited SnO2@N-doped porous carbon catalysts[J]. SCIENCE CHINA-CHEMISTRY,2018,61(2):228-235. |
| APA | Lu, Lu.,Sun, Xiaofu.,Ma, Jun.,Zhu, Qinggong.,Wu, Congyi.,...&Han, Buxing.(2018).Selective electroreduction of carbon dioxide to formic acid on electrodeposited SnO2@N-doped porous carbon catalysts.SCIENCE CHINA-CHEMISTRY,61(2),228-235. |
| MLA | Lu, Lu,et al."Selective electroreduction of carbon dioxide to formic acid on electrodeposited SnO2@N-doped porous carbon catalysts".SCIENCE CHINA-CHEMISTRY 61.2(2018):228-235. |
入库方式： OAI收割
来源：化学研究所
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