The designing strategies of graphene-based peroxidase mimetic materials
文献类型：期刊论文
| 作者 | Wen, Yanjie1; Yan, Linyin2; Ling, Yong-Chien1 |
| 刊名 | SCIENCE CHINA-CHEMISTRY
 |
| 出版日期 | 2018-03-01 |
| 卷号 | 61期号:3页码:266-275 |
| ISSN号 | 1674-7291 |
| 关键词 | Graphene Graphene Oxide Graphene-based Composites Artificial Enzymes Biomimetic Chemistry Nanozymes Functional Nanomaterials |
| DOI | 10.1007/s11426-017-9127-y |
| 英文摘要 | Natural enzymes have been praised highly as ideal catalysts, presumably owing to their remarkable advantages of high efficiency, high selectivity, and mild reaction conditions. The reports of chemical simulation and systematic synthesis of natural enzymes such as peroxidase (POD) are rare because of their complex biological structures. POD represents a large family of oxidoreductases and offers a wide range of applications in many fields of science. Recent advance in the fusion of nanomaterial, catalysis, and biochemistry has inspired the development of artificial enzymes implemented with desired catalytic features of natural enzymes. Herein, we review the redox chemistry of POD and compare its catalytic performance to graphene-based nanomaterials (G-NMs) as POD mimetic nanoenzymes bases on catalytic center, binding site, and carrier function. Based on the viewpoints of stereo chemistry and molecular kinetic and dynamics in heterogeneous system, we evaluate and compare the suitability of different NMs as artificial enzyme constituent. We propose that reevaluates design strategies of graphene-based peroxidase (G-POD) mimetic materials and emphasizes on their selectivity (role as catalytic center, binding site, or carrier) is of uttermost. |
| 语种 | 英语 |
| 出版者 | SCIENCE PRESS |
| WOS记录号 | WOS:000427405000002 |
| 源URL | [http://ir.iccas.ac.cn/handle/121111/45785]  |
| 专题 | 中国科学院化学研究所 |
| 通讯作者 | Yan, Linyin; Ling, Yong-Chien |
| 作者单位 | 1.Taiwan Tsing Hua Univ, Hsinchu 30013, Taiwan 2.Chinese Acad Sci, Beijing Natl Lab Mol Sci, Inst Chem, Beijing 100190, Peoples R China |
| 推荐引用方式 GB/T 7714 | Wen, Yanjie,Yan, Linyin,Ling, Yong-Chien. The designing strategies of graphene-based peroxidase mimetic materials[J]. SCIENCE CHINA-CHEMISTRY,2018,61(3):266-275. |
| APA | Wen, Yanjie,Yan, Linyin,&Ling, Yong-Chien.(2018).The designing strategies of graphene-based peroxidase mimetic materials.SCIENCE CHINA-CHEMISTRY,61(3),266-275. |
| MLA | Wen, Yanjie,et al."The designing strategies of graphene-based peroxidase mimetic materials".SCIENCE CHINA-CHEMISTRY 61.3(2018):266-275. |
入库方式： OAI收割
来源：化学研究所
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