A Versatile and Robust Approach to Stimuli-Responsive Protein Multilayers with Biologically Enabled Unique Functions
文献类型：期刊论文
| 作者 | Zhang, Xue-Jian1,2; Wang, Xiao-Wei1; Da, Xiao-Di1; Shi, Yanlin3; Liu, Chunli3; Sun, Fei4; Yang, Shuguang2; Zhang, Wen-Bin1 |
| 刊名 | BIOMACROMOLECULES
 |
| 出版日期 | 2018-03-01 |
| 卷号 | 19期号:3页码:1065-1073 |
| ISSN号 | 1525-7797 |
| DOI | 10.1021/acs.biomac.8b00190 |
| 英文摘要 | Protein-based materials call for innovative processing techniques to integrate their unique biologically enabled functions with other materials of complementary features. Herein, we report the covalent protein layer-by-layer assembly via orthogonal "Tag-Catcher" reactions as a facile and robust approach to make entirely protein-based multilayers on a variety of substrates. Programmed assembly of native telechelic proteins not only endows the materials valuable stimuli-sensitive behaviors, but also unique properties unparalleled by any synthetic counterparts. As proof of concept, super uranyl-binding protein (SUP) is immobilized on silica gel by this method with tunable capacity and enhanced capability for uranyl sequestration. Not only is the capturing performance enhanced in the multilayer setup, it also confers resilience to recycling, allowing efficient harvest of uranyl with an average of 90% and 60% recovery rate in over 10 cycles from water and synthetic seawater, respectively. The approach is the first entirely protein-based multilayers covalently assembled by the layer-by-layer method. It provides a platform for immobilizing proteins with synergistic enhancement of function and resilience and expands the scope and capability of genetically encoded protein-based materials. |
| 语种 | 英语 |
| WOS记录号 | WOS:000427539600036 |
| 出版者 | AMER CHEMICAL SOC |
| 源URL | [http://ir.iccas.ac.cn/handle/121111/45833]  |
| 专题 | 中国科学院化学研究所 |
| 通讯作者 | Yang, Shuguang; Zhang, Wen-Bin |
| 作者单位 | 1.Peking Univ, Coll Chem & Mol Engn, Ctr Soft Matter Sci & Engn, Key Lab Polymer Chem & Phys,Minist Educ, Beijing 100871, Peoples R China 2.Donghua Univ, Coll Mat Sci & Engn, Ctr Adv Low Dimens Mat, State Key Lab Modificat Chem Fibers & Polymer Mat, Shanghai 201620, Peoples R China 3.Peking Univ, Beijing Natl Lab Mol Sci, Coll Chem & Mol Engn, Fundamental Sci Lab Radiochem & Radiat Chem, Beijing 100871, Peoples R China 4.Hong Kong Univ Sci & Technol, Depnt Chem & Biol Engn, Kowloon, Hong Kong, Peoples R China |
| 推荐引用方式 GB/T 7714 | Zhang, Xue-Jian,Wang, Xiao-Wei,Da, Xiao-Di,et al. A Versatile and Robust Approach to Stimuli-Responsive Protein Multilayers with Biologically Enabled Unique Functions[J]. BIOMACROMOLECULES,2018,19(3):1065-1073. |
| APA | Zhang, Xue-Jian.,Wang, Xiao-Wei.,Da, Xiao-Di.,Shi, Yanlin.,Liu, Chunli.,...&Zhang, Wen-Bin.(2018).A Versatile and Robust Approach to Stimuli-Responsive Protein Multilayers with Biologically Enabled Unique Functions.BIOMACROMOLECULES,19(3),1065-1073. |
| MLA | Zhang, Xue-Jian,et al."A Versatile and Robust Approach to Stimuli-Responsive Protein Multilayers with Biologically Enabled Unique Functions".BIOMACROMOLECULES 19.3(2018):1065-1073. |
入库方式： OAI收割
来源：化学研究所
浏览0
下载0
收藏0
其他版本
除非特别说明，本系统中所有内容都受版权保护，并保留所有权利。