Thermally Activated Delayed Fluorescence Conjugated Polymers with Backbone-Donor/Pendant-Acceptor Architecture for Nondoped OLEDs with High External Quantum Efficiency and Low Roll-Off
文献类型：期刊论文
| 作者 | Yang, Yike1,2; Wang, Shumeng1; Zhu, Yunhui1,2; Wang, Yanjie1,2; Zhan, Hongmei1; Cheng, Yanxiang1 |
| 刊名 | ADVANCED FUNCTIONAL MATERIALS
 |
| 出版日期 | 2018-03-07 |
| 卷号 | 28期号:10 |
| 关键词 | Acceptor Benzophenone Conjugated Polymer Electroluminescence Thermally Activated Delayed Fluorescence |
| ISSN号 | 1616-301X |
| DOI | 10.1002/adfm.201706916 |
| 英文摘要 | Most thermally activated delayed fluorescence (TADF) emitters have to be doped in the host for fabricating efficient organic light-emitting diodes (OLEDs) and always suffer from quick efficiency roll-off at high brightness, which severely affect their commercial application in display and lighting fields. In the work, a series of the polymers are synthesized by copolymerization of two carbazole monomers and one acridine derivative monomer containing benzophenone acceptor group. The obtained polymers therefore possess a conjugated backbone with carbazole/acridine moieties and benzophenone pendant to form the twisted donor/acceptor structure. Consequently, the TADF features inherited from the acridine derivative are maintained and improved by managing the content of acridine derivative monomer in the polymers. Solution-processed OLEDs obtained from using neat polymer films exhibit comparable performance with organic TADF small molecules, achieving a maximum external quantum efficiency (EQE) of 18.1% and a very slow roll-off with EQE of 17.8% at the luminance of 1000 cd m(-2). |
| 语种 | 英语 |
| WOS记录号 | WOS:000426603700031 |
| 出版者 | WILEY-V C H VERLAG GMBH |
| 源URL | [http://ir.iccas.ac.cn/handle/121111/45839]  |
| 专题 | 中国科学院化学研究所 |
| 通讯作者 | Zhan, Hongmei; Cheng, Yanxiang |
| 作者单位 | 1.Chinese Acad Sci, State Key Lab Polymer Phys & Chem, Changchun Inst Appl Chem, Changchun 130022, Jilin, Peoples R China 2.Univ Chinese Acad Sci, Beijing 100049, Peoples R China |
| 推荐引用方式 GB/T 7714 | Yang, Yike,Wang, Shumeng,Zhu, Yunhui,et al. Thermally Activated Delayed Fluorescence Conjugated Polymers with Backbone-Donor/Pendant-Acceptor Architecture for Nondoped OLEDs with High External Quantum Efficiency and Low Roll-Off[J]. ADVANCED FUNCTIONAL MATERIALS,2018,28(10). |
| APA | Yang, Yike,Wang, Shumeng,Zhu, Yunhui,Wang, Yanjie,Zhan, Hongmei,&Cheng, Yanxiang.(2018).Thermally Activated Delayed Fluorescence Conjugated Polymers with Backbone-Donor/Pendant-Acceptor Architecture for Nondoped OLEDs with High External Quantum Efficiency and Low Roll-Off.ADVANCED FUNCTIONAL MATERIALS,28(10). |
| MLA | Yang, Yike,et al."Thermally Activated Delayed Fluorescence Conjugated Polymers with Backbone-Donor/Pendant-Acceptor Architecture for Nondoped OLEDs with High External Quantum Efficiency and Low Roll-Off".ADVANCED FUNCTIONAL MATERIALS 28.10(2018). |
入库方式： OAI收割
来源：化学研究所
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