Anchoring zero valence single atoms of nickel and iron on graphdiyne for hydrogen evolution
文献类型：期刊论文
| 作者 | Xue, Yurui1; Huang, Bolong2; Yi, Yuanping1,3; Guo, Yuan1; Zuo, Zicheng1; Li, Yongjun1,3; Jia, Zhiyu1; Liu, Huibiao1,3; Li, Yuliang1,3 |
| 刊名 | NATURE COMMUNICATIONS
 |
| 出版日期 | 2018-04-13 |
| 卷号 | 9 |
| ISSN号 | 2041-1723 |
| DOI | 10.1038/s41467-018-03896-4 |
| 英文摘要 | Electrocatalysis by atomic catalysts is a major focus of chemical and energy conversion effort. Although transition-metal-based bulk electrocatalysts for electrochemical application on energy conversion processes have been reported frequently, anchoring the stable transitionmetal atoms (e. g. nickel and iron) still remains a practical challenge. Here we report a strategy for fabrication of ACs comprising only isolated nickel/iron atoms anchored on graphdiyne. Our findings identify the very narrow size distributions of both nickel (1.23 angstrom) and iron (1.02 angstrom), typical sizes of single-atom nickel and iron. The precision of this method motivates us to develop a general approach in the field of single-atom transition-metal catalysis. Such atomic catalysts have high catalytic activity and stability for hydrogen evolution reactions. |
| 语种 | 英语 |
| WOS记录号 | WOS:000429921000017 |
| 出版者 | NATURE PUBLISHING GROUP |
| 源URL | [http://ir.iccas.ac.cn/handle/121111/45957]  |
| 专题 | 中国科学院化学研究所 |
| 通讯作者 | Li, Yuliang |
| 作者单位 | 1.Chinese Acad Sci, Inst Chem, Key Lab Organ Solids, Beijing 100190, Peoples R China 2.Hong Kong Polytech Univ Hung Hom, Dept Appl Biol & Chem Technol, Kowloon, Hong Kong, Peoples R China 3.Univ Chinese Acad Sci, Beijing 100049, Peoples R China |
| 推荐引用方式 GB/T 7714 | Xue, Yurui,Huang, Bolong,Yi, Yuanping,et al. Anchoring zero valence single atoms of nickel and iron on graphdiyne for hydrogen evolution[J]. NATURE COMMUNICATIONS,2018,9. |
| APA | Xue, Yurui.,Huang, Bolong.,Yi, Yuanping.,Guo, Yuan.,Zuo, Zicheng.,...&Li, Yuliang.(2018).Anchoring zero valence single atoms of nickel and iron on graphdiyne for hydrogen evolution.NATURE COMMUNICATIONS,9. |
| MLA | Xue, Yurui,et al."Anchoring zero valence single atoms of nickel and iron on graphdiyne for hydrogen evolution".NATURE COMMUNICATIONS 9(2018). |
入库方式： OAI收割
来源：化学研究所
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