Striking Influence about HZSM-5 Content and Nickel Catalyst on Catalytic Carbonization of Polypropylene and Polyethylene into Carbon Nanomaterials
文献类型：期刊论文
| 作者 | Gong, Jiang1,2; Feng, Jingdong1; Liu, Jie1; Muhammad, Raheel1; Chen, Xuecheng1,3; Jiang, Zhiwei1,2; Mijowska, Ewa3; Wen, Xin1; Tang, Tao1 |
| 刊名 | INDUSTRIAL & ENGINEERING CHEMISTRY RESEARCH
 |
| 出版日期 | 2013-11-06 |
| 卷号 | 52期号:44页码:15578-15588 |
| ISSN号 | 0888-5885 |
| DOI | 10.1021/ie402178b |
| 英文摘要 | A one-pot approach was established to effectively convert polypropylene (PP) and linear low density polyethylene (LLDPE) into carbon nanomaterials (CNMs) including cup-stacked carbon nanotubes and carbon nanofibers under the combined catalysis of HZSM-5/NiO or HZSM-5/Ni2O3 at 700 degrees C. The effects of HZSM-5 content, a nickel catalyst, and the carbon precursor on the morphology, microstructure, phase structure, and thermal stability of CNMs were investigated with scanning electron microscopy, transmission electron microscopy (TEM), high-resolution TEM, X-ray diffraction, Raman spectroscopy, and thermal gravimetric analysis. The effect of HZSM-5 content on the degradation products of PP and LLDPE was analyzed by gas chromatography and gas chromatography mass spectrometry. With increasing HZSM-5 content, the yields of light hydrocarbons and aromatics increased due to proton acid sites on the surface of HZSM-5 catalyzing cracking of PP or LLDPE degradation products. This one-pot approach provides a novel potential way to largely transform mixed waste polyolefin into high value-added CNMs. |
| 语种 | 英语 |
| WOS记录号 | WOS:000326774700041 |
| 出版者 | AMER CHEMICAL SOC |
| 源URL | [http://ir.iccas.ac.cn/handle/121111/46495]  |
| 专题 | 中国科学院化学研究所 |
| 通讯作者 | Chen, Xuecheng |
| 作者单位 | 1.Chinese Acad Sci, Changchun Inst Appl Chem, State Key Lab Polymer Phys & Chem, Changchun 130022, Peoples R China 2.Univ Chinese Acad Sci, Beijing 100049, Peoples R China 3.West Pomeranian Univ Technol, Inst Chem & Environm Engn, PL-70322 Szczecin, Poland |
| 推荐引用方式 GB/T 7714 | Gong, Jiang,Feng, Jingdong,Liu, Jie,et al. Striking Influence about HZSM-5 Content and Nickel Catalyst on Catalytic Carbonization of Polypropylene and Polyethylene into Carbon Nanomaterials[J]. INDUSTRIAL & ENGINEERING CHEMISTRY RESEARCH,2013,52(44):15578-15588. |
| APA | Gong, Jiang.,Feng, Jingdong.,Liu, Jie.,Muhammad, Raheel.,Chen, Xuecheng.,...&Tang, Tao.(2013).Striking Influence about HZSM-5 Content and Nickel Catalyst on Catalytic Carbonization of Polypropylene and Polyethylene into Carbon Nanomaterials.INDUSTRIAL & ENGINEERING CHEMISTRY RESEARCH,52(44),15578-15588. |
| MLA | Gong, Jiang,et al."Striking Influence about HZSM-5 Content and Nickel Catalyst on Catalytic Carbonization of Polypropylene and Polyethylene into Carbon Nanomaterials".INDUSTRIAL & ENGINEERING CHEMISTRY RESEARCH 52.44(2013):15578-15588. |
入库方式： OAI收割
来源：化学研究所
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