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Template-Free Synthesis of Cube-like Ag/AgCl Nanostructures via a Direct-Precipitation Protocol: Highly Efficient Sunlight-Driven Plasmonic Photocatalysts

文献类型:期刊论文

作者Zhu, Mingshan; Chen, Penglei; Ma, Wanhong; Lei, Bin; Liu, Minghua
刊名ACS APPLIED MATERIALS & INTERFACES
出版日期2012-11-01
卷号4期号:11页码:6386-6392
关键词Silver/silver Chloride Direct-precipitation Cube-like Nanostucture Plasmonic Photocatalyst Visible-light Or Sunlight Photodegradation
ISSN号1944-8244
DOI10.1021/am302100u
英文摘要In this paper, we report that cube-like Ag/AgCl nanostructures could be facilely fabricated in a one-pot manner through a direct-precipitation protocol under ambient conditions, wherein no additional issues such as external energy (e.g., high temperature or high pressure), surfactants, or reducing agents are required. In terms of using sodium chloride (NaCl) as chlorine source and silver acetate (CH3COOAg) as silver source, it is disclosed that simply by adding an aqueous solution of NaCl into an aqueous solution of CH3COOAg Ag/AgCl nanostructures with a cube-like geometry, could be successfully formulated. We show that thus-formulated cube-like Ag/AgCl nanospecies could be used as high-performance yet durable visible-light-driven or sunlight-driven plasmonic photocatalysts for the photodegradation of methyl orange (MO) and 4-chlorophenol (4-CP) pollutants. Compared with the commercially available P25-TiO2, and the Ag/AgCl nanospheres previously fabricated via a surfactant-assisted method, our current cube-like Ag/AgCl nanostructures could exhibit much higher photocatalytic performance. Our template free protocol might open up new and varied opportunities for an easy synthesis of cube-like Ag/AgCl-based high-performance sunlight-driven plasmonic photocatalysts for organic pollutant elimination.
语种英语
WOS记录号WOS:000311521900089
出版者AMER CHEMICAL SOC
源URL[http://ir.iccas.ac.cn/handle/121111/47951]  
专题中国科学院化学研究所
通讯作者Chen, Penglei
作者单位Chinese Acad Sci, Beijing Natl Lab Mol Sci, CAS Key Lab Colloid Interface & Chem Thermodynam, Inst Chem, Beijing 100190, Peoples R China
推荐引用方式
GB/T 7714
Zhu, Mingshan,Chen, Penglei,Ma, Wanhong,et al. Template-Free Synthesis of Cube-like Ag/AgCl Nanostructures via a Direct-Precipitation Protocol: Highly Efficient Sunlight-Driven Plasmonic Photocatalysts[J]. ACS APPLIED MATERIALS & INTERFACES,2012,4(11):6386-6392.
APA Zhu, Mingshan,Chen, Penglei,Ma, Wanhong,Lei, Bin,&Liu, Minghua.(2012).Template-Free Synthesis of Cube-like Ag/AgCl Nanostructures via a Direct-Precipitation Protocol: Highly Efficient Sunlight-Driven Plasmonic Photocatalysts.ACS APPLIED MATERIALS & INTERFACES,4(11),6386-6392.
MLA Zhu, Mingshan,et al."Template-Free Synthesis of Cube-like Ag/AgCl Nanostructures via a Direct-Precipitation Protocol: Highly Efficient Sunlight-Driven Plasmonic Photocatalysts".ACS APPLIED MATERIALS & INTERFACES 4.11(2012):6386-6392.

入库方式: OAI收割

来源:化学研究所

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