Plasma synthesis of oxidized graphene foam supporting Pd nanoparticles as a new catalyst for one-pot synthesis of dibenzyls
文献类型：期刊论文
| 作者 | Ren, Liang1; Yang, Fan1; Wang, Chunxia2; Li, Yongfeng1; Liu, Hailing1; Tu, Zhiqiang1; Zhang, Liqiang1; Liu, Zhichang1; Gao, Jinsen1; Xu, Chunming1 |
| 刊名 | RSC ADVANCES
 |
| 出版日期 | 2014 |
| 卷号 | 4期号:108页码:63048-63054 |
| ISSN号 | 2046-2069 |
| DOI | 10.1039/c4ra11060a |
| 英文摘要 | We have developed an environmentally-friendly method for the synthesis of Pd nanoparticle (Pd NPs) decorated different graphene supports, and the morphology and structure of the hybrids are characterized by transmission electron microscopy, X-ray diffraction, X-ray photoelectron spectroscopy and elemental mappings. Four hybrid materials based on graphene foam (GF), oxidized graphene foam (OGF), graphene oxide (GO) and reduced graphene oxide (RGO) have been used to catalyze Heck coupling reactions, and the effect of support on the activity of the hybrid material has been studied. Our results have revealed that Pd NP decorated OGF (Pd/OGF) is the most active catalyst, showing better performance than the commercial Pd/C catalyst. More importantly, the Pd/OGF catalyst has been successfully used for one-pot synthesis of dibenzyls with different aryl bromides and olefins, which has simplified the separation and purification process and realized a green organic synthesis process. |
| 语种 | 英语 |
| WOS记录号 | WOS:000345701500032 |
| 出版者 | ROYAL SOC CHEMISTRY |
| 源URL | [http://ir.iccas.ac.cn/handle/121111/52273]  |
| 专题 | 中国科学院化学研究所 |
| 通讯作者 | Li, Yongfeng |
| 作者单位 | 1.China Univ Petr, State Key Lab Heavy Oil Proc, Beijing 102249, Peoples R China 2.Chinese Acad Sci, Beijing Natl Lab Mol Sci, Key Lab Analyt Chem Living Biosyst, Inst Chem, Beijing 100190, Peoples R China |
| 推荐引用方式 GB/T 7714 | Ren, Liang,Yang, Fan,Wang, Chunxia,et al. Plasma synthesis of oxidized graphene foam supporting Pd nanoparticles as a new catalyst for one-pot synthesis of dibenzyls[J]. RSC ADVANCES,2014,4(108):63048-63054. |
| APA | Ren, Liang.,Yang, Fan.,Wang, Chunxia.,Li, Yongfeng.,Liu, Hailing.,...&Xu, Chunming.(2014).Plasma synthesis of oxidized graphene foam supporting Pd nanoparticles as a new catalyst for one-pot synthesis of dibenzyls.RSC ADVANCES,4(108),63048-63054. |
| MLA | Ren, Liang,et al."Plasma synthesis of oxidized graphene foam supporting Pd nanoparticles as a new catalyst for one-pot synthesis of dibenzyls".RSC ADVANCES 4.108(2014):63048-63054. |
入库方式： OAI收割
来源：化学研究所
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