Sustainable Conversion of Mixed Plastics into Porous Carbon Nanosheets with High Performances in Uptake of Carbon Dioxide and Storage of Hydrogen
文献类型：期刊论文
| 作者 | Gong, Jiang1,2; Michalkiewicz, Beata3; Chen, Xuecheng1,3; Mijowska, Ewa3; Liu, Jie1; Jiang, Zhiwei1; Wen, Xin1; Tang, Tao1 |
| 刊名 | ACS SUSTAINABLE CHEMISTRY & ENGINEERING
 |
| 出版日期 | 2014-12-01 |
| 卷号 | 2期号:12页码:2837-2844 |
| 关键词 | Mixed Plastics Sustainable Approach Porous Carbon Nanosheet Carbon Dioxide Hydrogen |
| ISSN号 | 2168-0485 |
| DOI | 10.1021/sc500603h |
| 英文摘要 | Conversion of waste plastics into high value added carbon nanomaterials has gained wide research interest due to the requirement of sustainable development and the ever-increasing generation of waste plastics. However, most of studies are limited to single component plastic; besides, little attention has been paid to carbon nanosheets (CNS). Herein, CNS were prepared by catalytic carbonization of mixed plastics consisting of polypropylene, polyethylene, polystyrene, poly(ethylene terephthalate), and polyvinyl chloride on organically modified montmorillonite. After KOH activation, porous CNS (PCNS) were produced. The morphology, microstructure, phase structure, textural property, surface element composition, and thermal stability of PCNS were investigated. PCNS contained randomly oriented lattice fringes and showed a layered morphology consisting of thin, leaf-like, agglomerated nanosheets ranging from hundreds of nanometers to several micrometers in length. Besides, PCNS exhibited high specific surface area (1734 m(2)/g) and large pore volume (2.441 cm(3)/g). More importantly, PCNS displayed high performances in the uptake of carbon dioxide and storage of hydrogen. It is believed that this work not only paves the way for utilization of mixed waste plastics but also provides a facile sustainable approach for the large scale production of valuable PCNS for energy storage and environmental remediation. |
| 语种 | 英语 |
| WOS记录号 | WOS:000345734800025 |
| 出版者 | AMER CHEMICAL SOC |
| 源URL | [http://ir.iccas.ac.cn/handle/121111/53045]  |
| 专题 | 中国科学院化学研究所 |
| 通讯作者 | Chen, Xuecheng |
| 作者单位 | 1.Chinese Acad Sci, Changchun Inst Appl Chem, State Key Lab Polymer Phys & Chem, Changchun 130022, Peoples R China 2.Univ Chinese Acad Sci, Beijing 100049, Peoples R China 3.West Pomeranian Univ Technol, Inst Chem & Environm Engn, PL-70322 Szczecin, Poland |
| 推荐引用方式 GB/T 7714 | Gong, Jiang,Michalkiewicz, Beata,Chen, Xuecheng,et al. Sustainable Conversion of Mixed Plastics into Porous Carbon Nanosheets with High Performances in Uptake of Carbon Dioxide and Storage of Hydrogen[J]. ACS SUSTAINABLE CHEMISTRY & ENGINEERING,2014,2(12):2837-2844. |
| APA | Gong, Jiang.,Michalkiewicz, Beata.,Chen, Xuecheng.,Mijowska, Ewa.,Liu, Jie.,...&Tang, Tao.(2014).Sustainable Conversion of Mixed Plastics into Porous Carbon Nanosheets with High Performances in Uptake of Carbon Dioxide and Storage of Hydrogen.ACS SUSTAINABLE CHEMISTRY & ENGINEERING,2(12),2837-2844. |
| MLA | Gong, Jiang,et al."Sustainable Conversion of Mixed Plastics into Porous Carbon Nanosheets with High Performances in Uptake of Carbon Dioxide and Storage of Hydrogen".ACS SUSTAINABLE CHEMISTRY & ENGINEERING 2.12(2014):2837-2844. |
入库方式： OAI收割
来源：化学研究所
浏览0
下载0
收藏0
其他版本
除非特别说明，本系统中所有内容都受版权保护，并保留所有权利。