Self-organized graphene crystal patterns
文献类型:期刊论文
作者 | Wu, Bin1; Geng, Dechao1; Xu, Zhiping2,3; Guo, Yunlong1; Huang, Liping1; Xue, Yunzhou1; Chen, Jianyi1; Yu, Gui1; Liu, Yunqi1 |
刊名 | NPG ASIA MATERIALS
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出版日期 | 2013-02-01 |
卷号 | 5 |
关键词 | Graphene Pattern Crystal Growth Snowflakes Chemical Vapor Deposition |
ISSN号 | 1884-4049 |
DOI | 10.1038/am.2012.68 |
英文摘要 | The phenomenon of ordered pattern formation is universal in nature but involves complex non-equilibrium processes that are highly important for both fundamental research and applied materials systems. Among countless pattern systems, a snowflake is possibly the most fascinating example offered by nature. Here, we report that single-layered and single-crystalline graphene flakes (GFs) with highly regular and hexagonal symmetric patterns can be grown on a liquid copper surface using a CH4 chemical vapor deposition (CVD) method. The different morphologies of these GFs can be precisely tailored by varying the composition of the inert gas/H-2 carrier gas mixture used to produce the GFs, and the GF edges can be continuously tuned over the full spectrum from negative to zero to positive curvature in a controllable way. The family of GF crystal patterns is remarkably analogous to that of snowflakes, representing an ideal two-dimensional (2D) growth system. Pattern formations from compact to dendritic GFs can be explained by the continuous modulation of the competition between adatom diffusion along island edges or corners and surface diffusion processes. NPG Asia Materials (2013) 5, e36; doi:10.1038/am.2012.68; published online 1 February 2013 |
语种 | 英语 |
WOS记录号 | WOS:000315349500002 |
出版者 | NATURE PUBLISHING GROUP |
源URL | [http://ir.iccas.ac.cn/handle/121111/54881] ![]() |
专题 | 中国科学院化学研究所 |
通讯作者 | Liu, Yunqi |
作者单位 | 1.Chinese Acad Sci, Inst Chem, Key Lab Organ Solids, Beijing Natl Lab Mol Sci, Beijing 100190, Peoples R China 2.Tsinghua Univ, Dept Engn Mech, Beijing 100084, Peoples R China 3.Tsinghua Univ, Ctr Nano & Micro Mech, Beijing 100084, Peoples R China |
推荐引用方式 GB/T 7714 | Wu, Bin,Geng, Dechao,Xu, Zhiping,et al. Self-organized graphene crystal patterns[J]. NPG ASIA MATERIALS,2013,5. |
APA | Wu, Bin.,Geng, Dechao.,Xu, Zhiping.,Guo, Yunlong.,Huang, Liping.,...&Liu, Yunqi.(2013).Self-organized graphene crystal patterns.NPG ASIA MATERIALS,5. |
MLA | Wu, Bin,et al."Self-organized graphene crystal patterns".NPG ASIA MATERIALS 5(2013). |
入库方式: OAI收割
来源:化学研究所
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