A simplified formulation of linear and nonlinear spectroscopy of ordered molecular systems
文献类型：期刊论文
| 作者 | Wang, HF |
| 刊名 | CHINESE JOURNAL OF CHEMICAL PHYSICS
 |
| 出版日期 | 2004-06-01 |
| 卷号 | 17期号:3页码:362-368 |
| 关键词 | Linear And nonLinear Spectroscopy Second Harmonic Generation Sum Frequency Generation Vibrational Spectroscopy General Orientational Functional Ordered Molecular System |
| ISSN号 | 1003-7713 |
| 英文摘要 | A simplified formulation for treating the linear and nonlinear spectroscopy of ordered molecular systems is presented, in order to help experimentalists to have an explicit physical picture and quantitative tool on using linear and nonlinear spectroscopy to study molecules in ordered molecular systems. This formulation is expended from our recent quantitative orientational and polarization treatment on second-order nonlinear spectroscopic techniques in interface studies, namely, the Second Harmonic Generation (SHG) and Sum Frequency Generation-Vibrational Polarization Spectroscopy (SFG-VPS). The key to this formulation is to simplify the effective linear or nonlinear molecular susceptibility and construct the general orientational functional with a clear approach to calculate the orientational and intensity parameters from the experimental parameters, which deter-mines the orientational and polarization behavior of the general orientational functional in a particular experimental configuration. Also discussed are the advantages of coherent spectroscopic techniques over incoherent ones for the accurate measurement of orientation and ordering of ordered molecular system. |
| 语种 | 英语 |
| WOS记录号 | WOS:000222521100022 |
| 出版者 | SCIENCE CHINA PRESS |
| 源URL | [http://ir.iccas.ac.cn/handle/121111/81563]  |
| 专题 | 中国科学院化学研究所 |
| 通讯作者 | Wang, HF |
| 作者单位 | Chinese Acad Sci, Inst Chem, Ctr Mol Sci, State Key Lab Mol React Dynam, Beijing 100080, Peoples R China |
| 推荐引用方式 GB/T 7714 | Wang, HF. A simplified formulation of linear and nonlinear spectroscopy of ordered molecular systems[J]. CHINESE JOURNAL OF CHEMICAL PHYSICS,2004,17(3):362-368. |
| APA | Wang, HF.(2004).A simplified formulation of linear and nonlinear spectroscopy of ordered molecular systems.CHINESE JOURNAL OF CHEMICAL PHYSICS,17(3),362-368. |
| MLA | Wang, HF."A simplified formulation of linear and nonlinear spectroscopy of ordered molecular systems".CHINESE JOURNAL OF CHEMICAL PHYSICS 17.3(2004):362-368. |
入库方式： OAI收割
来源：化学研究所
浏览0
下载0
收藏0
其他版本
除非特别说明，本系统中所有内容都受版权保护，并保留所有权利。