Triple Acceptors in a Polymeric Architecture for Balanced Ambipolar Transistors and High-Gain Inverters
文献类型：期刊论文
| 作者 | Yi, Zhengran1,2; Jiang, Yingying3,4; Xu, Long1; Zhong, Cheng5; Yang, Jie1; Wang, Qijun1; Xiao, Junwu1; Liao, Xueming5; Wang, Shuai1; Guo, Yunlong3,4 |
| 刊名 | ADVANCED MATERIALS
 |
| 出版日期 | 2018-08-09 |
| 卷号 | 30期号:32 |
| ISSN号 | 0935-9648 |
| 关键词 | Ambipolar Polymer Semiconductor Effective Mass Molecular Architecture Molecular Packing Organic Thin-film Transistor |
| DOI | 10.1002/adma.201801951 |
| 英文摘要 | The exploration of novel molecular architectures is crucial for the design of high-performance ambipolar polymer semiconductors. Here, a triple-acceptors architecture strategy to design the ambipolar polymer DPP-2T-DPP-TBT is introduced. The utilization of this architecture enables DPP-2T-DPP-TBT to achieve deep-lying highest occupied molecular orbital (HOMO)/lowest unoccupied molecular orbital (LUMO) levels of -5.38/-4.19 eV, and strong intermolecular interactions, which are favorable for hole/electron injection and intermolecular hopping through -stacking. All these factors result in excellent ambipolar transport characteristics and promising applications in complementary-like circuits for DPP-2T-DPP-TBT under ambient conditions with high hole/electron mobilities and a gain value of up to 3.01/3.84 cm(2) V-1 s(-1) and 171, respectively, which are among the best performances in ambipolar polymer organic thin-film transistors and associated complementary-like circuits, especially in top-gate device configuration with low-cost glass as substrates. These results demonstrate that the triple-acceptors architecture strategy is an effective way for designing high-performance ambipolar polymer semiconductors. |
| 语种 | 英语 |
| 出版者 | WILEY-V C H VERLAG GMBH |
| WOS记录号 | WOS:000440813300015 |
| 源URL | [http://ir.iccas.ac.cn/handle/121111/41924]  |
| 专题 | 化学研究所_有机固体实验室 |
| 通讯作者 | Wang, Shuai; Guo, Yunlong; Liu, Yunqi |
| 作者单位 | 1.Huazhong Univ Sci & Technol, Sch Chem & Chem Engn, Wuhan 430074, Peoples R China 2.Wuhan Inst Technol, Sch Chem Engn & Pharm, Wuhan 430205, Hubei, Peoples R China 3.Chinese Acad Sci, Beijing Natl Lab Mol Sci, Key Lab Organ Solids, Inst Chem, Beijing 100190, Peoples R China 4.Univ Chinese Acad Sci, Beijing 100049, Peoples R China 5.Wuhan Univ, Dept Chem, Hubei Key Lab Organ & Polymer Optoelect Mat, Wuhan 430072, Peoples R China 6.Tianjin Univ, Tianjin Key Lab Mol Optoelect Sci, Dept Chem, Sch Sci, Tianjin 300072, Peoples R China 7.Collaborat Innovat Ctr Chem Sci & Engn Tianjin, Tianjin 300072, Peoples R China |
| 推荐引用方式 GB/T 7714 | Yi, Zhengran,Jiang, Yingying,Xu, Long,et al. Triple Acceptors in a Polymeric Architecture for Balanced Ambipolar Transistors and High-Gain Inverters[J]. ADVANCED MATERIALS,2018,30(32). |
| APA | Yi, Zhengran.,Jiang, Yingying.,Xu, Long.,Zhong, Cheng.,Yang, Jie.,...&Liu, Yunqi.(2018).Triple Acceptors in a Polymeric Architecture for Balanced Ambipolar Transistors and High-Gain Inverters.ADVANCED MATERIALS,30(32). |
| MLA | Yi, Zhengran,et al."Triple Acceptors in a Polymeric Architecture for Balanced Ambipolar Transistors and High-Gain Inverters".ADVANCED MATERIALS 30.32(2018). |
入库方式： OAI收割
来源：化学研究所
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