Isotopic compositions of U-236, Pu-239, and Pu-240 in soil contaminated by the Fukushima Daiichi Nuclear Power Plant accident
文献类型：期刊论文
| 作者 | Okayama, Kumiko; Yamada, Masatoshi; Yang GS(杨国胜); Yang, Guosheng; Tazoe, Hirofumi; Hayano, Kazuhiko |
| 刊名 | SCIENTIFIC REPORTS
 |
| 出版日期 | 2017 |
| 卷号 | 7页码:13619 |
| ISSN号 | 2045-2322 |
| DOI | 10.1038/s41598-017-13998-6 |
| 文献子类 | Article |
| 英文摘要 | Six years after the Fukushima Daiichi Nuclear Power Plant (FDNPP) accident, data for U-236 and U-236/U-238 have remained limited to a few heavily contaminated samples. In the present study, activities of U-236, Pu-239, and Pu-240, along with other U isotopes in 46 soil samples both heavily and lightly contaminated by this accident were measured by inductively coupled plasma-mass spectrometry (ICP-MS) and triple-quadrupole ICP-MS. The U-236 activities and U-236/U-238 atom ratios in these soil samples were in the range of (0.469-24.4) x 10(-5) Bq kg(-1) and ((0.099-1.35) x 10(-7)), respectively. Higher Pu-240/Pu-239 atom ratios (0.245-0.312) and Pu-238/Pu239+240 activity ratios (0.859-1.62) indicated Pu contamination originated from this accident and global fallout in some samples. For those soil samples along with black substances collected along roads in Fukushima Prefecture, high linear correlations were presented between U-236 activities and Pu239+240 activities (Pearson's r = 0.755, p < 0.01), and between U-236 activities and Pu-238 activities (Pearson's r = 0.844, p < 0.01). The analysis of these soil samples confirmed the release of U-236, although in trace amounts, during the FDNPP accident. |
| WOS关键词 | PLASMA-MASS SPECTROMETRY ; ENVIRONMENTAL-SAMPLES ; PU ISOTOPES ; ICP-MS ; PLUTONIUM ; RATIO ; FALLOUT ; AMS ; URANIUM ; IDENTIFICATION |
| WOS研究方向 | Science & Technology - Other Topics |
| 语种 | 英语 |
| WOS记录号 | WOS:000413191500058 |
| 源URL | [http://ir.ihep.ac.cn/handle/311005/284865]  |
| 专题 | 高能物理研究所_核技术应用研究中心 |
| 作者单位 | 中国科学院高能物理研究所 |
| 推荐引用方式 GB/T 7714 | Okayama, Kumiko,Yamada, Masatoshi,Yang GS,et al. Isotopic compositions of U-236, Pu-239, and Pu-240 in soil contaminated by the Fukushima Daiichi Nuclear Power Plant accident[J]. SCIENTIFIC REPORTS,2017,7:13619. |
| APA | Okayama, Kumiko,Yamada, Masatoshi,杨国胜,Yang, Guosheng,Tazoe, Hirofumi,&Hayano, Kazuhiko.(2017).Isotopic compositions of U-236, Pu-239, and Pu-240 in soil contaminated by the Fukushima Daiichi Nuclear Power Plant accident.SCIENTIFIC REPORTS,7,13619. |
| MLA | Okayama, Kumiko,et al."Isotopic compositions of U-236, Pu-239, and Pu-240 in soil contaminated by the Fukushima Daiichi Nuclear Power Plant accident".SCIENTIFIC REPORTS 7(2017):13619. |
入库方式： OAI收割
来源：高能物理研究所
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