Can I-129 track Cs-135, U-236, Pu-239, and Pu-240 apart from I-131 in soil samples from Fukushima Prefecture, Japan?
文献类型：期刊论文
| 作者 | Yang, Guosheng; Yamada, Masatoshi; Yang GS(杨国胜); Tazoe, Hirofumi |
| 刊名 | SCIENTIFIC REPORTS
 |
| 出版日期 | 2017 |
| 卷号 | 7页码:15369 |
| ISSN号 | 2045-2322 |
| DOI | 10.1038/s41598-017-15714-w |
| 文献子类 | Article |
| 英文摘要 | In the present study, I-129 activities and I-129/I-127 atom ratios were measured in 60 soil samples contaminated by the Fukushima Daiichi Nuclear Power Plant (FDNPP) accident. The I-127 concentrations, I-129 activities, and I-129/I-127 atom ratios in dry-weight were observed to be 0.121-23.6 mg kg(-1), 0.962-275 mBq kg(-1), and (0.215-79.3) x 10(-7), respectively. The maximum values of both I-129 activities and I-129/I-127 atom ratios in Japanese soil increased about three orders of magnitude due to this accident. The equation logy = 0.877logx + 0.173 (Pearson's r = 0.936; x, I-129 concentration; y, I-131 concentration; decay-corrected to March 11, 2011) instead of a simple constant may be a better way to express the relationship between I-129 and I-131 in Japanese soil affected by both global fallout and FDNPP accident fallout. In addition, a moderate correlation was observed between I-129 and Cs-135 (logy = 0.624logx + 1.01, Pearson's r = 0.627; x, I-129 activity; y, Cs-135 activity). However, I-129 presented larger fractionations with less volatile radionuclides, such as U-236, Pu-239, and Pu-240. These findings indicated Cs-135 could be roughly estimated from I-129 or I-131; this is advantageous as fewer Cs-135 data are available and Cs-135/Cs-137 is being considered a promising tracer during radiocesium source identification. |
| WOS关键词 | NUCLEAR-POWER-PLANT ; ACCELERATOR MASS-SPECTROMETRY ; ENVIRONMENTAL-SAMPLES ; ATMOSPHERIC FALLOUT ; ISOTOPIC RATIO ; PU ISOTOPES ; ACCIDENT ; RADIONUCLIDES ; SYSTEM |
| WOS研究方向 | Science & Technology - Other Topics |
| 语种 | 英语 |
| WOS记录号 | WOS:000415022900005 |
| 源URL | [http://ir.ihep.ac.cn/handle/311005/284866]  |
| 专题 | 高能物理研究所_核技术应用研究中心 |
| 作者单位 | 中国科学院高能物理研究所 |
| 推荐引用方式 GB/T 7714 | Yang, Guosheng,Yamada, Masatoshi,Yang GS,et al. Can I-129 track Cs-135, U-236, Pu-239, and Pu-240 apart from I-131 in soil samples from Fukushima Prefecture, Japan?[J]. SCIENTIFIC REPORTS,2017,7:15369. |
| APA | Yang, Guosheng,Yamada, Masatoshi,杨国胜,&Tazoe, Hirofumi.(2017).Can I-129 track Cs-135, U-236, Pu-239, and Pu-240 apart from I-131 in soil samples from Fukushima Prefecture, Japan?.SCIENTIFIC REPORTS,7,15369. |
| MLA | Yang, Guosheng,et al."Can I-129 track Cs-135, U-236, Pu-239, and Pu-240 apart from I-131 in soil samples from Fukushima Prefecture, Japan?".SCIENTIFIC REPORTS 7(2017):15369. |
入库方式： OAI收割
来源：高能物理研究所
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