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Dynamics and diagenesis of trace metals in sediments of the Changjiang Estuary

文献类型：期刊论文

作者Duan, Liqin1,2,3,4; Song, Jinming1,2,3,4; Liang, Xianmeng1,3; Yin, Meiling1,3; Yuan, Huamao1,2,3,4; Li, Xuegang1,2,3,4; Ren, Chengzhe1,3; Zhou, Bu1; Kang, Xuming5; Yin, Xuebo2,3,4,6
刊名SCIENCE OF THE TOTAL ENVIRONMENT
出版日期2019-07-20
卷号675页码:247-259
ISSN号0048-9697
关键词Trace metals Porewater Early diagenesis Seasonal cycling Benthic fluxes The Changjiang Estuary
DOI10.1016/j.scitotenv.2019.04.190
通讯作者Duan, Liqin(duanliqin@qdio.ac.cn) ; Song, Jinming(jmsong@qdio.ac.cn)
英文摘要The seasonal dynamics and diagenesis of trace metals at two contrasting coastal sites were studied to determine the mechanism that drove the diffusive release of trace metals from sediments in the Changjiang Estuary. Porewater trace metal concentrations were 53.4-4829 nM for Zn, 11.0-344 nM for Cu, 7.75-221 nM for Cr, 2.71-61.1 nM for Co, 0.822-42.7 nM for Pb and 0.037-4.22 nM for Cd. The concentrations and profiles of trace metals in the porewater and solid phase displayed obvious regional and seasonal variations. This variation was mainly reflected in the surface layer and the depth of the suboxic and anoxic layers. Regionally, surface porewater trace metal concentrations in the seasonal hypoxic region were higher than those in the aerobic region due to changes in the redox conditions being beneficial to the release of trace metals. Seasonally, surface porewater trace metal concentrations decreased in summer compared to spring due to their removal by forming metal sulfides in summer. Solid profiles of the trace metals supported their dynamic variations in the porewater. The partition coefficient suggested that the formation of Fe/Mn (hydr) oxides was effective for the removal of trace metal in oxidizing condition, while the formation of sulfides was conducive to the removal of trace metals in reducing condition. The combination of porewater with solid phase data suggested that the dynamics of Cu, Zn, Cr and Co were mainly controlled by Fe and Mn diagenesis, the dynamics of Cd were affected by S cycling, and the dynamics of Pb were disturbed by anthropogenic inputs and benthic organism activities. Estimation of benthic fluxes indicated that sediments were an important source of trace metals in the water column. The contributions of trace metals by sediments to the water column of the Changjiang Estuary were only one order of magnitude lower than those by riverine fluxes. (C) 2019 Elsevier B.V. All rights reserved.
资助项目National Natural Science Foundation of China[41676068] ; Aoshan Technology Innovation Program of the Qingdao National Laboratory for Marine Science and Technology, China[2016ASKJ02-4] ; National Natural Science Foundation of China-Shandong Joint Fund[U1606404] ; Youth Innovation Promotion Association of the Chinese Academy of Sciences[2016191] ; Foundation for Huiquan Young Scholar of Institute of Oceanology, Chinese Academy of Sciences, China
WOS研究方向Environmental Sciences & Ecology
语种英语
出版者ELSEVIER SCIENCE BV
WOS记录号WOS:000467391900023
源URL[http://ir.qdio.ac.cn/handle/337002/161373]  
专题海洋研究所_海洋生态与环境科学重点实验室
海洋研究所_海洋地质与环境重点实验室
通讯作者Duan, Liqin; Song, Jinming
作者单位1.Chinese Acad Sci, Inst Oceanol, CAS Key Lab Marine Ecol & Environm Sci, Qingdao 266071, Shandong, Peoples R China
2.Qingdao Natl Lab Marine Sci & Technol, Lab Marine Ecol & Environm Sci, Qingdao 266237, Shandong, Peoples R China
3.Univ Chinese Acad Sci, Beijing 100049, Peoples R China
4.Chinese Acad Sci, Ctr Ocean Mega Sci, Qingdao 266071, Shandong, Peoples R China
5.Chinese Acad Fishery Sci, Yellow Sea Fisheries Res Inst, Minist Agr, Key Lab Testing & Evaluat Aquat Prod Safety & Qua, Qingdao 266071, Shandong, Peoples R China
6.Chinese Acad Sci, Inst Oceanol, CAS Key Lab Marine Geol & Environm, Qingdao 266071, Shandong, Peoples R China
推荐引用方式
GB/T 7714		 Duan, Liqin,Song, Jinming,Liang, Xianmeng,et al. Dynamics and diagenesis of trace metals in sediments of the Changjiang Estuary[J]. SCIENCE OF THE TOTAL ENVIRONMENT,2019,675:247-259.
APA Duan, Liqin.,Song, Jinming.,Liang, Xianmeng.,Yin, Meiling.,Yuan, Huamao.,...&Yin, Xuebo.(2019).Dynamics and diagenesis of trace metals in sediments of the Changjiang Estuary.SCIENCE OF THE TOTAL ENVIRONMENT,675,247-259.
MLA Duan, Liqin,et al."Dynamics and diagenesis of trace metals in sediments of the Changjiang Estuary".SCIENCE OF THE TOTAL ENVIRONMENT 675(2019):247-259.

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来源：海洋研究所

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