Combined potential of three catalysis types on TiO2 nanotube (TNT)/Ti and nanoparticle (TNP)/Ti photoelectrodes: A comparative study
文献类型:期刊论文
作者 | Zhang, Aiyong1; Zhou, Minghua1; Han, Lu1; Zhou, Qixing1,2 |
刊名 | APPLIED CATALYSIS A-GENERAL
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出版日期 | 2010-09-15 |
卷号 | 385期号:1-2页码:114-122 |
关键词 | Combined Degradation Photocatalysis Electrocatalysis Tio2 Nanotube (Tnt) Tio2 Nanoparticle (Tnp) Azo Dye |
ISSN号 | 0926-860X |
DOI | 10.1016/j.apcata.2010.06.053 |
英文摘要 | The one-dimensional TiO2 nanotubes (1DTNT/Ti)photoelectrode with a huge anodic area of 38 cm(2) were successfully prepared for the first time, with satisfactory morphological integrity, structural strength and distinguished photoactivity, and then utilized in a combined degradation system. A novel and photo-driven combined degradation system (TBPE system), which was functionally comprised of photon-efficient thin-film photocatalysis, conventional bulk-phase photocatalysis and photocarrier-efficient electrocatalysis, was developed on the vertically ordered and upright oriented 1D TNT/Ti rotating photoelectrode (TNT-TBPE system). Its properties were compared to those of the randomly packed zero-dimensional TiO2 nanoparticles (0D TNP/Ti) rotating photoelectrode (TNP-TBPE system). Under the optimized operation conditions, the degradation of methyl orange (MO) was comparatively studied in the TNT-TBPE and TNP-TBPE systems. A 7.6-32.3% degradation enhancement and 20% larger stability indicated the excellent degradation activity and photochemical stability of TBPE system on novel 1D TNT/Ti compared to existing 0D TNP/Ti photoelectrode. The difference was attributed to the functional combination of these three catalysis types and the effective incorporation of 1D TNT/Ti rotating photoelectrode. (c) 2010 Elsevier B.V. All rights reserved. |
WOS研究方向 | Chemistry ; Environmental Sciences & Ecology |
语种 | 英语 |
WOS记录号 | WOS:000281991000013 |
出版者 | ELSEVIER SCIENCE BV |
源URL | [http://210.72.129.5/handle/321005/121371] ![]() |
专题 | 中国科学院沈阳应用生态研究所 |
通讯作者 | Zhou, Minghua |
作者单位 | 1.Nankai Univ, Coll Environm Sci & Engn, Minist Educ, Key Lab Pollut Proc & Environm Criteria, Tianjin 300071, Peoples R China 2.Chinese Acad Sci, Inst Appl Ecol, Key Lab Terr Ecol Proc, Shenyang 110016, Peoples R China |
推荐引用方式 GB/T 7714 | Zhang, Aiyong,Zhou, Minghua,Han, Lu,et al. Combined potential of three catalysis types on TiO2 nanotube (TNT)/Ti and nanoparticle (TNP)/Ti photoelectrodes: A comparative study[J]. APPLIED CATALYSIS A-GENERAL,2010,385(1-2):114-122. |
APA | Zhang, Aiyong,Zhou, Minghua,Han, Lu,&Zhou, Qixing.(2010).Combined potential of three catalysis types on TiO2 nanotube (TNT)/Ti and nanoparticle (TNP)/Ti photoelectrodes: A comparative study.APPLIED CATALYSIS A-GENERAL,385(1-2),114-122. |
MLA | Zhang, Aiyong,et al."Combined potential of three catalysis types on TiO2 nanotube (TNT)/Ti and nanoparticle (TNP)/Ti photoelectrodes: A comparative study".APPLIED CATALYSIS A-GENERAL 385.1-2(2010):114-122. |
入库方式: OAI收割
来源:沈阳应用生态研究所
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