Nanocatalysts for Electrocatalytic Oxidation of Ethanol
文献类型：期刊论文
| 作者 | Bai, Juan1; Liu, Danye2,3; Yang, Jun2,3; Chen, Yu1 |
| 刊名 | CHEMSUSCHEM
 |
| 出版日期 | 2019-05-21 |
| 卷号 | 12期号:10页码:2117-2132 |
| 关键词 | direct alcohol fuel cell electrocatalyst nanomaterials noble metals |
| ISSN号 | 1864-5631 |
| DOI | 10.1002/cssc.201803063 |
| 英文摘要 | The use of ethanol as a fuel in direct alcohol fuel cells depends not only on its ease of production from renewable sources, but also on overcoming the challenges of storage and transportation. In an ethanol-based fuel cell, highly active electrocatalysts are required to break the C-C bond in ethanol for its complete oxidation at lower overpotentials, with the aim of increasing the cell performance, ethanol conversion rates, and fuel efficiency. In recent decades, the development of wet-chemistry methods has stimulated research into catalyst design, reactivity tailoring, and mechanistic investigations, and thus, created great opportunities to achieve efficient oxidation of ethanol. In this Minireview, the nanomaterials tested as electrocatalysts for the ethanol oxidation reaction in acid or alkaline environments are summarized. The focus is mainly on nanomaterials synthesized by using wet-chemistry methods, with particular attention on the relationship between the chemical and physical characteristics of the catalysts, for example, catalyst composition, morphology, structure, degree of alloying, presence of oxides or supports, and their activity for ethanol electro-oxidation. As potential alternatives to noble metals, non-noble-metal catalysts for ethanol oxidation are also briefly reviewed. Insights into further enhancing the catalytic performance through the design of efficient electrocatalysts are also provided. |
| WOS关键词 | REDUCED GRAPHENE OXIDE ; HIGH-INDEX FACETS ; CARBON NITRIDE ELECTROCATALYSTS ; HIGHLY EFFICIENT CATALYSTS ; SHAPE-CONTROLLED SYNTHESIS ; DENSITY-FUNCTIONAL THEORY ; OXYGEN REDUCTION REACTION ; ALKALINE DIRECT ETHANOL ; AT-AGPD NANOPARTICLES ; IN-SITU FTIR |
| 资助项目 | National Natural Science Foundation of China[21875133] ; National Natural Science Foundation of China[21573240] ; Fundamental Research Funds for the Central Universities[GK201901002] ; 111 Project[B14041] ; Institute of Process Engineering, Chinese Academy of Sciences[MPCS-2017-A-02] |
| WOS研究方向 | Chemistry ; Science & Technology - Other Topics |
| 语种 | 英语 |
| WOS记录号 | WOS:000472806800005 |
| 出版者 | WILEY-V C H VERLAG GMBH |
| 资助机构 | National Natural Science Foundation of China ; Fundamental Research Funds for the Central Universities ; 111 Project ; Institute of Process Engineering, Chinese Academy of Sciences |
| 源URL | [http://ir.ipe.ac.cn/handle/122111/30010]  |
| 专题 | 中国科学院过程工程研究所 |
| 通讯作者 | Yang, Jun; Chen, Yu |
| 作者单位 | 1.Shaanxi Normal Univ, Sch Mat Sci & Engn, Minist Educ,Key Lab Macromol Sci Shaanxi Prov, Shaanxi Key Lab Adv Energy Devices,Key Lab Appl S, Xian 710062, Shaanxi, Peoples R China 2.Chinese Acad Sci, Inst Proc Engn Address, State Key Lab Multiphase Complex Syst, Beijing 100190, Peoples R China 3.Univ Chinese Acad Sci, Beijing 100049, Peoples R China |
| 推荐引用方式 GB/T 7714 | Bai, Juan,Liu, Danye,Yang, Jun,et al. Nanocatalysts for Electrocatalytic Oxidation of Ethanol[J]. CHEMSUSCHEM,2019,12(10):2117-2132. |
| APA | Bai, Juan,Liu, Danye,Yang, Jun,&Chen, Yu.(2019).Nanocatalysts for Electrocatalytic Oxidation of Ethanol.CHEMSUSCHEM,12(10),2117-2132. |
| MLA | Bai, Juan,et al."Nanocatalysts for Electrocatalytic Oxidation of Ethanol".CHEMSUSCHEM 12.10(2019):2117-2132. |
入库方式： OAI收割
来源：过程工程研究所
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