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Atmospheric pollution for trace elements in the remote high-altitude atmosphere in central Asia as recorded in snow from Mt. Qomolangma (Everest) of the Himalayas

文献类型:期刊论文

作者Lee, Khanghyun1; Do Hur, Soon1; Hou, Shugui2; Hong, Sungmin1; Qin, Xiang2; Ren, Jiawen2; Liu, Yapping2; Rosman, Keuin J. R.3; Barbante, Carlo4,5; Boutron, Claude F.6,7,8
刊名SCIENCE OF THE TOTAL ENVIRONMENT
出版日期2008-10-01
卷号404期号:1页码:171-181
关键词Trace elements Mt. Everest Monsoon and non-monsoon Anthropogenic pollution Fallout flux
ISSN号0048-9697
DOI10.1016/j.scitotenv.2008.06.022
通讯作者Hong, Sungmin(smhong@kopri.re.kr)
英文摘要A series of 42 snow samples covering over a one-year period from the fall of 2004 to the summer of 2005 were collected from a 2.1-m snow pit at a high-altitude site on the northeastern slope of Mt. Everest. These samples were analyzed for Al, V, Cr, Mn, Co, Ni, Cu, Zn, As, Rb, Sr, Cd, Sb, Pb, and Bi in order to characterize the relative contributions from anthropogenic and natural sources to the fallout of these elements in central Himalayas. Our data were also considered in the context of monsoon versus non-monsoon seasons. The mean concentrations of the majority of the elements were determined to be at the pg g(-1) level with a strong variation in concentration with snow depth. While the mean concentrations of most of the elements were significantly higher during the non-monsoon season than during the monsoon season, considerable variability in the trace element inputs to the snow was observed during both periods. Cu, Zn, As, Cd, Sb, and Bi displayed high crustal enrichment factors (EFc) in most samples, while Cr, Ni, Rb, and Pb show high EFc values in some of the samples. Our data indicate that anthropogenic inputs are potentially important for these elements in the remote high-altitude atmosphere in the central Himalayas. The relationship between the EFc of each element and the Al concentration indicates that a dominant input of anthropogenic trace elements occurs during both the monsoon and non-monsoon seasons, when crustal contribution is relatively minor. Finally, a comparison of the trace element fallout fluxes calculated in our samples with those recently obtained at Mont Blanc, Greenland, and Antarctica provides direct evidence for a geographical gradient of the atmospheric pollution with trace elements on a global scale. (C) 2008 Elsevier B.V. All rights reserved.
收录类别SCI
WOS关键词CENTRAL GREENLAND SNOW ; MONT-BLANC ICE ; ANTARCTIC SNOW ; HEAVY-METALS ; SEASONAL-VARIATIONS ; EAST ANTARCTICA ; LEAD ISOTOPES ; CHEMICAL-COMPOSITION ; ANTHROPOGENIC LEAD ; FRESHSNOW SAMPLES
WOS研究方向Environmental Sciences & Ecology
WOS类目Environmental Sciences
语种英语
WOS记录号WOS:000260268300018
出版者ELSEVIER SCIENCE BV
URI标识http://www.irgrid.ac.cn/handle/1471x/2556041
专题寒区旱区环境与工程研究所
通讯作者Hong, Sungmin
作者单位1.Korea Polar Res Inst, Inchon 406840, South Korea
2.Chinese Acad Sci, Cold & Arid Reg Environm & Engn Res Inst, State Key Lab Cryospher Sci, Lanzhou 730000, Peoples R China
3.Curtin Univ Technol, Dept Imaging & Appl Phys, Perth, WA 6845, Australia
4.Univ Venice, Dept Environm Sci, I-30123 Venice, Italy
5.Univ Venice, CNR, Ctr Studies Environm Chem & Technol, I-30123 Venice, Italy
6.CNRS, UMR 5183, Lab Glaciol & Geophys Environm, F-38402 St Martin Dheres, France
7.Univ Grenoble 1, Inst Univ France, Observ Sci Univers, F-38041 Grenoble, France
8.Univ Grenoble 1, Inst Univ France, Unite Format & Rech Phys, F-38041 Grenoble, France
推荐引用方式
GB/T 7714
Lee, Khanghyun,Do Hur, Soon,Hou, Shugui,et al. Atmospheric pollution for trace elements in the remote high-altitude atmosphere in central Asia as recorded in snow from Mt. Qomolangma (Everest) of the Himalayas[J]. SCIENCE OF THE TOTAL ENVIRONMENT,2008,404(1):171-181.
APA Lee, Khanghyun.,Do Hur, Soon.,Hou, Shugui.,Hong, Sungmin.,Qin, Xiang.,...&Boutron, Claude F..(2008).Atmospheric pollution for trace elements in the remote high-altitude atmosphere in central Asia as recorded in snow from Mt. Qomolangma (Everest) of the Himalayas.SCIENCE OF THE TOTAL ENVIRONMENT,404(1),171-181.
MLA Lee, Khanghyun,et al."Atmospheric pollution for trace elements in the remote high-altitude atmosphere in central Asia as recorded in snow from Mt. Qomolangma (Everest) of the Himalayas".SCIENCE OF THE TOTAL ENVIRONMENT 404.1(2008):171-181.

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