Evaluation of a CMAQ simulation at high resolution over the UK for the calendar year 2003
文献类型：期刊论文
| 作者 | Chemel, C.1; Sokhi, R. S.1; Yu, Y.1,2,3; Hayman, G. D.4; Vincent, K. J.5; Dore, A. J.6; Tang, Y. S.6; Prain, H. D.1; Fisher, B. E. A.7 |
| 刊名 | ATMOSPHERIC ENVIRONMENT
 |
| 出版日期 | 2010-08-01 |
| 卷号 | 44期号:24页码:2927-2939 |
| 关键词 | Air quality Numerical simulation Model performance Evaluation |
| ISSN号 | 1352-2310 |
| DOI | 10.1016/j.atmosenv.2010.03.029 |
| 通讯作者 | Chemel, C.(c.chemel@herts.ac.uk) |
| 英文摘要 | A comprehensive 'operational' evaluation of the performance of the Community Multiscale Air Quality (CMAQ) modelling system version 4.6 was conducted in support of pollution assessment in the UK for the calendar year 2003. The model was run on multiple grids using one-way nests down to a horizontal resolution as fine as 5 km over the whole of the UK. The model performance was evaluated for pollutants with standards and limit values (e.g. O(3), PM(10)) and species contributing to acidic and nitrogenous deposition (e.g. NH(3), SO(4)(2-), NO(3)(-), NH(4)(+)) against data from operational national monitoring networks. The key performance characteristics of the modelling system were found to be variable according to acceptance criteria and to depend on the type (e.g. urban, rural) and location of the sites, as well as on the time of the year. As regards the techniques that were used for 'operational' evaluation, performance generally complied with expected levels and ranged from good (e.g. O(3), SO(4)(2-) to moderate (e.g. PM(10), NO(3)(-)). At a few sites low correlations and large standard deviations for some species (e.g. SO(2)) suggest that these sites are subject to local factors (e.g. topography, emission sources) that are not well described in the model. Overall, the model tends to over predict O(3) and under predict aerosol species (except SO(4)(2-)). Discrepancies between predicted and observed concentrations may be due to a variety of intertwined factors, which include inaccuracies in meteorological predictions, chemical boundary conditions, temporal variability in emissions, and uncertainties in the treatment of gas and aerosol chemistry. Further work is thus required to investigate the respective contributions of such factors on the predicted concentrations. (C) 2010 Elsevier Ltd. All rights reserved. |
| 收录类别 | SCI |
| WOS关键词 | COMPREHENSIVE PERFORMANCE EVALUATION ; 1999 SOUTHERN OXIDANTS ; AIR-QUALITY MODELS ; ATMOSPHERIC TRANSPORT ; ACID DEPOSITION ; UNITED-KINGDOM ; PART II ; METEOROLOGICAL MODEL ; PARTICULATE MATTER ; CHEMICAL MECHANISM |
| WOS研究方向 | Environmental Sciences & Ecology ; Meteorology & Atmospheric Sciences |
| WOS类目 | Environmental Sciences ; Meteorology & Atmospheric Sciences |
| 语种 | 英语 |
| WOS记录号 | WOS:000280277700016 |
| 出版者 | PERGAMON-ELSEVIER SCIENCE LTD |
| URI标识 | http://www.irgrid.ac.cn/handle/1471x/2556336 |
| 专题 | 寒区旱区环境与工程研究所 |
| 通讯作者 | Chemel, C. |
| 作者单位 | 1.Univ Hertfordshire, Ctr Atmospher & Instrumentat Res, Hatfield AL10 9AB, Herts, England 2.Chinese Acad Sci, Inst Plateau Atmospher Phys Cold & Arid Reg Envir, Lanzhou 730000, Gansu, Peoples R China 3.Chinese Acad Sci, Engn Res Inst, Lanzhou 730000, Gansu, Peoples R China 4.Ctr Ecol & Hydrol Wallingford, Wallingford OX10 8BB, Oxon, England 5.Harwell Int Business Ctr, AEA Energy & Environm, Didcot OX11 0QR, Oxon, England 6.Ctr Ecol & Hydrol Edinburgh, Penicuik EH26 0QB, Midlothian, Scotland 7.Environm Agcy, Reading RG1 8DQ, Berks, England |
| 推荐引用方式 GB/T 7714 | Chemel, C.,Sokhi, R. S.,Yu, Y.,et al. Evaluation of a CMAQ simulation at high resolution over the UK for the calendar year 2003[J]. ATMOSPHERIC ENVIRONMENT,2010,44(24):2927-2939. |
| APA | Chemel, C..,Sokhi, R. S..,Yu, Y..,Hayman, G. D..,Vincent, K. J..,...&Fisher, B. E. A..(2010).Evaluation of a CMAQ simulation at high resolution over the UK for the calendar year 2003.ATMOSPHERIC ENVIRONMENT,44(24),2927-2939. |
| MLA | Chemel, C.,et al."Evaluation of a CMAQ simulation at high resolution over the UK for the calendar year 2003".ATMOSPHERIC ENVIRONMENT 44.24(2010):2927-2939. |
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来源：寒区旱区环境与工程研究所
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