Transport of Semivolatile Organic Compounds to the Tibetan Plateau: Spatial and Temporal Variation in Air Concentrations in Mountainous Western Sichuan, China
文献类型：期刊论文
| 作者 | Liu, Wenjie1,2; Chen, Dazhou1,3; Liu, Xiande1; Zheng, Xiaoyan1; Yang, Wen1; Westgate, John N.4,5; Wania, Frank4,5 |
| 刊名 | ENVIRONMENTAL SCIENCE & TECHNOLOGY
 |
| 出版日期 | 2010-03-01 |
| 卷号 | 44期号:5页码:1559-1565 |
| ISSN号 | 0013-936X |
| DOI | 10.1021/es902764z |
| 通讯作者 | Liu, Xiande(xiande.liu@gmail.com) |
| 英文摘要 | The distribution of organochlorine pesticides and polychlorinated biphenyls in air along an altitudinal transect on Balang Mountain in western China was measured by deploying XAD-2 resin based passive air samplers in duplicate at seven sites with elevations ranging from 1242 to 4485 m above sea level for five consecutive six-month periods between 2005 and 2008, Analyzed by gas chromatography-high resolution mass spectrometry, concentrations of hexachlorobenzene were highest followed by hexachlorocyclohexanes, DDT-related compounds and PCB congeners 28 and 52. Except for hexachlorobenzene, which had largely uniform concentrations in space and time, there were clear seasonal variations with concentrations in summer being higher than in winter. With a few exceptions, concentrations that vary little with altitude suggest that the presence of these chemicals in the area is almost entirely due to atmospheric transport, most likely from the Chengdu plain. This is supported by similarities in the relative abundance of different compounds and in the differences between summer and winter concentrations measured in the city of Chengdu and in the mountains. Furthermore, air mass trajectories during the sampling period often originate to the East, passing over the Western part of the Sichuan basin, including the Chengdu plain, prior to arriving at the sampling sites. Higher summer time values in the mountains are due to more contaminated air being blown into the region, presumably due either to higher pesticide usage in summer or due to higher temperatures leading to higher evaporation in source regions. Air and soil from the region are in equilibrium with respect to alpha-HCH, gamma-HCH, and HCB, whereas a situation of net deposition prevails for p,p'-DDE and p,p'-DDT. |
| 收录类别 | SCI |
| WOS关键词 | POLYBROMINATED DIPHENYL ETHERS ; NORTH-AMERICAN ATMOSPHERE ; ORGANOCHLORINE PESTICIDES ; GAMMA-HEXACHLOROCYCLOHEXANE ; POLYCHLORINATED-BIPHENYLS ; SEASONAL-VARIATIONS ; POLLUTANTS ; HEXACHLOROBENZENE ; ENVIRONMENT ; CANADA |
| WOS研究方向 | Engineering ; Environmental Sciences & Ecology |
| WOS类目 | Engineering, Environmental ; Environmental Sciences |
| 语种 | 英语 |
| WOS记录号 | WOS:000274842000010 |
| 出版者 | AMER CHEMICAL SOC |
| URI标识 | http://www.irgrid.ac.cn/handle/1471x/2556355 |
| 专题 | 寒区旱区环境与工程研究所 |
| 通讯作者 | Liu, Xiande |
| 作者单位 | 1.Chinese Res Inst Environm Sci, Beijing 100012, Peoples R China 2.Chinese Acad Sci, Cold & Arid Reg Environm & Engn Res Inst, Lanzhou 730000, Peoples R China 3.Natl Res Ctr Certified Reference Mat, Beijing 100013, Peoples R China 4.Univ Toronto Scarborough, Dept Chem, Toronto, ON M1C 1A4, Canada 5.Univ Toronto Scarborough, Dept Phys & Environm Sci, Toronto, ON M1C 1A4, Canada |
| 推荐引用方式 GB/T 7714 | Liu, Wenjie,Chen, Dazhou,Liu, Xiande,et al. Transport of Semivolatile Organic Compounds to the Tibetan Plateau: Spatial and Temporal Variation in Air Concentrations in Mountainous Western Sichuan, China[J]. ENVIRONMENTAL SCIENCE & TECHNOLOGY,2010,44(5):1559-1565. |
| APA | Liu, Wenjie.,Chen, Dazhou.,Liu, Xiande.,Zheng, Xiaoyan.,Yang, Wen.,...&Wania, Frank.(2010).Transport of Semivolatile Organic Compounds to the Tibetan Plateau: Spatial and Temporal Variation in Air Concentrations in Mountainous Western Sichuan, China.ENVIRONMENTAL SCIENCE & TECHNOLOGY,44(5),1559-1565. |
| MLA | Liu, Wenjie,et al."Transport of Semivolatile Organic Compounds to the Tibetan Plateau: Spatial and Temporal Variation in Air Concentrations in Mountainous Western Sichuan, China".ENVIRONMENTAL SCIENCE & TECHNOLOGY 44.5(2010):1559-1565. |
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来源：寒区旱区环境与工程研究所
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