中国科学院机构知识库网格
Chinese Academy of Sciences Institutional Repositories Grid
Characterization of submicron aerosols and effect on visibility during a severe haze-fog episode in Yangtze River Delta, China

文献类型:期刊论文

作者Shen, X. J.1; Sun, J. Y.1,2; Zhang, X. Y.1; Zhang, Y. M.1; Zhang, L.1; Che, H. C.1; Ma, Q. L.3; Yu, X. M.3; Yue, Y.3; Zhang, Y. W.1
刊名ATMOSPHERIC ENVIRONMENT
出版日期2015-11-01
卷号120页码:307-316
ISSN号1352-2310
关键词Particle number size distribution Light extinction of submicron aerosol Secondary aerosol formation Severe haze-fog Air mass origin
DOI10.1016/j.atmosenv.2015.09.011
通讯作者Sun, J. Y.(jysun@cams.cma.gov.cn)
英文摘要Particle size, composition and optical properties were measured at a regional atmosphere background station in the Yangtze River Delta (YRD) to understand the formation and evolution of haze-fog episodes in Jan. 2013. The peak of particle number size distribution was in the size range of 80-100 nm during the measurements. PM1 mass concentration contributed 84% to the total particle mass (PM10). Based on visibility and ambient relative humidity, three types of weather conditions (i.e., clear, haze and fog) were classified in this study. The extinction coefficients of PM1 and PM10 under dry conditions were simulated by the Mie model. Under dry conditions, PM1 was found to contribute approximately 91% to the light extinction coefficient of PM10. However, the PM1 with the assumption of dry state was found to contribute approximately 85% to the ambient extinction coefficient of PM10 during clear conditions, 58% during haze conditions and approximately 41% during fog conditions. The variation of the dry PM1 contribution was related to the water uptake of particles under different relative humidity conditions. A severe haze-fog event on Jan. 14-17 was discussed in more detail as a case study. Two episodes were chosen to show that nitrate and organics dominated the aerosol component during the severe haze-fog episode and were related to secondary aerosol formation and air mass origin. Nitrate played a more dominant role than sulfate in heavy haze formation in the YRD region, which was different from the North China Plain region. (C) 2015 The Authors. Published by Elsevier Ltd. This is an open access article under the CC BY-NC-ND license (http://creativecommons.org/licenses/by-nc-nd/4.0/).
收录类别SCI
WOS关键词NUMBER SIZE DISTRIBUTIONS ; OPTICAL-PROPERTIES ; POLLUTION EPISODE ; EASTERN CHINA ; BOUNDARY-LAYER ; JANUARY 2013 ; PLAIN ; POLLUTANTS ; MECHANISM ; REGION
WOS研究方向Environmental Sciences & Ecology ; Meteorology & Atmospheric Sciences
WOS类目Environmental Sciences ; Meteorology & Atmospheric Sciences
语种英语
出版者PERGAMON-ELSEVIER SCIENCE LTD
WOS记录号WOS:000364255700032
URI标识http://www.irgrid.ac.cn/handle/1471x/2557191
专题寒区旱区环境与工程研究所
通讯作者Sun, J. Y.
作者单位1.Chinese Acad Meteorol Sci, Inst Atmospher Composit, Key Lab Atmospher Chem CMA, Beijing, Peoples R China
2.Chinese Acad Sci, Cold & Arid Reg Environm & Engn Res Inst, State Key Lab Cryospher Sci, Lanzhou, Peoples R China
3.Meteorol Bur Zhejiang Prov, Linan Atmospher Background Stn, Hangzhou, Peoples R China
推荐引用方式
GB/T 7714
Shen, X. J.,Sun, J. Y.,Zhang, X. Y.,et al. Characterization of submicron aerosols and effect on visibility during a severe haze-fog episode in Yangtze River Delta, China[J]. ATMOSPHERIC ENVIRONMENT,2015,120:307-316.
APA Shen, X. J..,Sun, J. Y..,Zhang, X. Y..,Zhang, Y. M..,Zhang, L..,...&Zhang, Y. W..(2015).Characterization of submicron aerosols and effect on visibility during a severe haze-fog episode in Yangtze River Delta, China.ATMOSPHERIC ENVIRONMENT,120,307-316.
MLA Shen, X. J.,et al."Characterization of submicron aerosols and effect on visibility during a severe haze-fog episode in Yangtze River Delta, China".ATMOSPHERIC ENVIRONMENT 120(2015):307-316.

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来源:寒区旱区环境与工程研究所

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