Application of equilibrium partitioning approach to the derivation of sediment quality guidelines for metals in Dianchi Lake
文献类型:期刊论文
作者 | Chen Yun-Zeng; Yang Hao; Zhang Zhen-Ke; Qin Ming-Zhou; Jin Feng; Lu Jun-Jie |
刊名 | PEDOSPHERE
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出版日期 | 2007-06-01 |
卷号 | 17期号:3页码:284-294 |
关键词 | acid volatile sulfide fine material normalization method organic carbon sediment quality guidelines |
ISSN号 | 1002-0160 |
通讯作者 | Yang Hao(yanghao@njnu.edu.cn) |
英文摘要 | For the past 20 years, numerous studies have been carried out on the application of equilibrium partitioning approach (EqPA) for the derivation of sediment quality guidelines (SQGs). However, for metals, few Equilibrium-partitioning-based numerical SQGs have been developed or are currently available because of the confounding factors mediating the bioavailability of metals. A study was conducted at Dianchi Lake, which is a heavily eutrophicated lake on the Yunnan-Guizhou Plateau, China with the focus on the measurement of partitioning coefficient (Kp) and SQGs derivation and normalization to acid volatile sulfide (AVS), fine material, and organic carbon. Using new normalization methods, SQGs were formulated for seven metals including copper, zinc, lead, cadmium, chromium, mercury, and arsenic in Dianchi Lake. In Dianchi Lake sediments, the fine material contributed 25.4%-36.0% to the SQG values, with the largest contribution to the SQG value of mercury; AVS contributed 2.9%-75.0% to the SQG values, with the largest contribution to the SQG value of cadmium. This indicated that the fine material and the AVS were the most important controlling factors to the bioavailability of mercury and cadmium, respectively. The contribution of total organic carbon (TOC) to the SQG values of copper and lead was 3.8% and 7.1%, respectively, indicating that at relatively lower concentrations, the contribution of TOC was not significant. In addition to normalization methods, appropriate procedures for the application of EqPA including sample collection, storage, and analysis are also essential to improve the reliability of SQGs. The normalized Dianchi Lake SQGs were higher than most of the empirically based SQGs developed in North America, but lower than Hong Kong interim SQGs except for cadmium and arsenic. The differences could be attributed to the approaches used for derivation of SQGs and the water quality criteria adopted and the differences in the physical and chemical characteristics of the sediments. |
收录类别 | SCI |
WOS关键词 | ACID-VOLATILE SULFIDE ; FRESH-WATER ECOSYSTEMS ; TRACE-METALS ; TOXICITY ; NORMALIZATIONS ; VALUES ; MODEL |
WOS研究方向 | Agriculture |
WOS类目 | Soil Science |
语种 | 英语 |
WOS记录号 | WOS:000246824900002 |
出版者 | SCIENCE CHINA PRESS |
URI标识 | http://www.irgrid.ac.cn/handle/1471x/2558717 |
专题 | 南京土壤研究所 |
通讯作者 | Yang Hao |
作者单位 | 1.Henan Univ, Inst Resources & Environm, Kaifeng 475001, Peoples R China 2.Chinese Acad Sci, Inst Soil Sci, State Key Lab Soil & Sustainable Agr, Nanjing 210008, Peoples R China 3.Nanjing Normal Univ, Coll Geog, Nanjing 210097, Peoples R China 4.Nanjing Univ, Key Lab Coast & Isl Dev, MOE, Nanjing 210093, Peoples R China |
推荐引用方式 GB/T 7714 | Chen Yun-Zeng,Yang Hao,Zhang Zhen-Ke,et al. Application of equilibrium partitioning approach to the derivation of sediment quality guidelines for metals in Dianchi Lake[J]. PEDOSPHERE,2007,17(3):284-294. |
APA | Chen Yun-Zeng,Yang Hao,Zhang Zhen-Ke,Qin Ming-Zhou,Jin Feng,&Lu Jun-Jie.(2007).Application of equilibrium partitioning approach to the derivation of sediment quality guidelines for metals in Dianchi Lake.PEDOSPHERE,17(3),284-294. |
MLA | Chen Yun-Zeng,et al."Application of equilibrium partitioning approach to the derivation of sediment quality guidelines for metals in Dianchi Lake".PEDOSPHERE 17.3(2007):284-294. |
入库方式: iSwitch采集
来源:南京土壤研究所
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