The aerosol optical properties and PM2.5 components over the world's largest industrial zone in Tangshan, North China
文献类型：期刊论文
| 作者 | Zhang, Kequan1; Ma, Yongjing1,2; Xin, Jinyuan2,3; Liu, Zirui2; Ma, Yining1,2; Gao, Dongdong3; Wu, Junsong4; Zhang, Wenyu1; Wang, Yuesi2; Shen, Pengke5 |
| 刊名 | ATMOSPHERIC RESEARCH
 |
| 出版日期 | 2018-03-01 |
| 卷号 | 201页码:226-234 |
| ISSN号 | 0169-8095 |
| 关键词 | Tangshan Industrial aerosols Aerosol optical properties PM2.5 chemical component |
| DOI | 10.1016/j.atmosres.2017.10.025 |
| 通讯作者 | Xin, Jinyuan(xjy@mail.iap.ac.cn) |
| 英文摘要 | To achieve an in-depth understanding of the aerosol optical properties in the highly-industrial region of Tangshan, we provided systematic aerosol optical properties analysis in this largest industrial zone for the first time. The aerosol optical datasets (2013.05-2015.04) and chemical component data of PM2.5 (2014-2015) obtained from the Tangshan site of the campaign on atmospheric aerosol research (CARE-China) network were analyzed. The results showed that the Tangshan region was seriously affected by fine-mode industrial aerosols all year, which would promote the accumulation of pollutants and influence the atmospheric circulation through changing the vertical temperature gradient. The annual average aerosol optical depth (AOD) and Angstrom exponent (a) were 0.80 +/- 0.26 and 1.05 +/- 0.10, respectively. The aerosol optical properties revealed significant seasonal characteristics. The maximum seasonal average AOD (1.03 +/- 0.62) and a (1.12 +/- 0.19) accompanied the highest seasonal secondary inorganic aerosol concentrations (SIA: So(4)(2-),NO3-,NH4+), 53.33 mu g/m(3), occurred in summer, and this phenomenon was attributed to the photochemical reactions favored by the high temperature and humidity. During the spring, frequent dust events led to the maximum Ca-2(+) concentration of 6.57 mu g/m(3) and the lowest seasonal a of 0.98 +/- 0.31. Coal was used for generating heat in winter, resulting in the highest levels of pollutant emissions (Cl- Elemental carbon (EC) and organic carbon (OC)). The aerosol type classifications showed that the industrial aerosols were the main controls in the summer and fall, representing 56%-58% of the total aerosols. While for spring and winter, mixed aerosols represented 53%-54% of the total aerosols. Hygroscopic growth effect of aerosols existed all year, which could enhance the negative radiative forcing and eventually cool the earth-atmosphere system. The classification Wing for Tangshan data showed high AOD values ( > 0.70) were mainly clustered in the fine-mode growth wing and coarse-mode. Of these values, summer showed a dense AOD distribution and the highest magnitude of fine-mode AODs, with a corresponding fine particle fraction of eta similar to 90% and an Rf similar to 0.20 mu m. In addition, spring showed the most coarse-mode aerosols. |
| WOS关键词 | RADIATIVE PROPERTIES ; ATMOSPHERIC AEROSOL ; PHYSICAL-PROPERTIES ; SUN-PHOTOMETER ; URBAN SITE ; CLIMATOLOGY ; DEPTH ; AERONET ; REGION ; MODIS |
| 资助项目 | National Basic Research Program of China[2016YFC0202001] ; National Natural Science Foundation of China[41375036] ; National Natural Science Foundation of China[41222033] ; National Basic Research Program of China (973 Program)[2014CB441200] |
| WOS研究方向 | Meteorology & Atmospheric Sciences |
| 语种 | 英语 |
| 出版者 | ELSEVIER SCIENCE INC |
| WOS记录号 | WOS:000418981500018 |
| 资助机构 | National Basic Research Program of China ; National Natural Science Foundation of China ; National Basic Research Program of China (973 Program) |
| 源URL | [http://ir.igsnrr.ac.cn/handle/311030/60588]  |
| 专题 | 中国科学院地理科学与资源研究所 |
| 通讯作者 | Xin, Jinyuan |
| 作者单位 | 1.Lanzhou Univ, Key Lab Arid Climat Change & Reducing Disaster Ga, Coll Atmospher Sci, Lanzhou 730000, Gansu, Peoples R China 2.Chinese Acad Sci, Inst Atmospher Phys, State Key Lab Atmospher Boundary Layer Phys & Atm, Beijing 100029, Peoples R China 3.Chengdu Univ Informat Technol, Plateau Atmosphere & Environm Key Lab Sichuan Pro, Chengdu 610225, Sichuan, Peoples R China 4.Shanxi JinHuart Keyuan Environm Resources Sci & T, Beijing, Peoples R China 5.Chinese Acad Sci, Inst Geog Sci & Nat Resources Res, Key Lab Land Surface Pattern & Simulat, Beijing, Peoples R China |
| 推荐引用方式 GB/T 7714 | Zhang, Kequan,Ma, Yongjing,Xin, Jinyuan,et al. The aerosol optical properties and PM2.5 components over the world's largest industrial zone in Tangshan, North China[J]. ATMOSPHERIC RESEARCH,2018,201:226-234. |
| APA | Zhang, Kequan.,Ma, Yongjing.,Xin, Jinyuan.,Liu, Zirui.,Ma, Yining.,...&Shen, Pengke.(2018).The aerosol optical properties and PM2.5 components over the world's largest industrial zone in Tangshan, North China.ATMOSPHERIC RESEARCH,201,226-234. |
| MLA | Zhang, Kequan,et al."The aerosol optical properties and PM2.5 components over the world's largest industrial zone in Tangshan, North China".ATMOSPHERIC RESEARCH 201(2018):226-234. |
入库方式： OAI收割
来源：地理科学与资源研究所
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