Fabrication of a Single-Atom Platinum Catalyst for the Hydrogen Evolution Reaction: A New Protocol by Utilization of HxMoO3-x with Plasmon Resonance
文献类型：期刊论文
| 作者 | Xu, Q ; Wang JO(王嘉鸥); Chu SQ(储胜启); Wang, JO; Chu, SQ; Du, Y; Chen, J; Yan, PF; Liu, W
|
| 刊名 | CHEMCATCHEM
 |
| 出版日期 | 2018 |
| 卷号 | 10期号:5页码:946-950 |
| 关键词 | amorphous materials hydrogen molybdenum surface plasmon resonance single-atom catalysts |
| ISSN号 | 1867-3880 |
| DOI | 10.1002/cctc.201701777 |
| 文献子类 | Article |
| 英文摘要 | Single-atom catalysts (SACs) play a key role in many chemical processes owing to highly desirable atom efficiency, but the challenging synthesis of these catalysts limits their commercialization and application on a large scale. Herein, we report a facile strategy to integrate atomic Pt into richly deficient MoO3-x. The core of the experimental strategy was the fabrication and utilization of HxMoO3-x with plasmon resonance that contained intercalated H+. The obtained catalyst was found to possess remarkable electrocatalytic activity toward the hydrogen evolution reaction that was even comparable to that of commercial Pt/C, whereas the amount of Pt used was reduced to only 10% of the amount of commercial Pt/C used. Therefore, this work not only supplies a new synthesis route to SACs but also reveals the potential relation between plasmon resonance materials and the fabrication of single-atom catalysts. |
| 电子版国际标准刊号 | 1867-3899 |
| WOS关键词 | CO OXIDATION ; EFFICIENT ; NANOSHEETS ; PERFORMANCE ; ALPHA-MOO3 ; GRAPHENE ; CLUSTERS ; SURFACE ; H-MOO3 ; WATER |
| WOS研究方向 | Chemistry |
| 语种 | 英语 |
| WOS记录号 | WOS:000426844600009 |
| 源URL | [http://ir.ihep.ac.cn/handle/311005/285712]  |
| 专题 | 高能物理研究所_粒子天体物理中心 高能物理研究所_多学科研究中心 |
| 作者单位 | 中国科学院高能物理研究所 |
| 推荐引用方式 GB/T 7714 | Xu, Q,Wang JO,Chu SQ,et al. Fabrication of a Single-Atom Platinum Catalyst for the Hydrogen Evolution Reaction: A New Protocol by Utilization of HxMoO3-x with Plasmon Resonance[J]. CHEMCATCHEM,2018,10(5):946-950. |
| APA | Xu, Q.,王嘉鸥.,储胜启.,Wang, JO.,Chu, SQ.,...&Liu, W.(2018).Fabrication of a Single-Atom Platinum Catalyst for the Hydrogen Evolution Reaction: A New Protocol by Utilization of HxMoO3-x with Plasmon Resonance.CHEMCATCHEM,10(5),946-950. |
| MLA | Xu, Q,et al."Fabrication of a Single-Atom Platinum Catalyst for the Hydrogen Evolution Reaction: A New Protocol by Utilization of HxMoO3-x with Plasmon Resonance".CHEMCATCHEM 10.5(2018):946-950. |
入库方式： OAI收割
来源：高能物理研究所
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