Tin(IV) Sulfide Greatly Improves the Catalytic Performance of UiO-66 for Carbon Dioxide Cycloaddition
文献类型：期刊论文
| 作者 | Zhang, BX ; Cheng, XY; Zheng LR(郑黎荣); Zhang J(张静); Yang, GY; Han, BX; Tan, XN; Shao, D; Zhang, J; Zheng, LR
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| 刊名 | CHEMCATCHEM
 |
| 出版日期 | 2018 |
| 卷号 | 10期号:14页码:2945-2948 |
| 关键词 | cycloaddition heterogeneous catalysis metal-organic frameworks nanoparticles tin sulfide |
| ISSN号 | 1867-3880 |
| DOI | 10.1002/cctc.201800411 |
| 文献子类 | Article |
| 英文摘要 | To overcome the limitations of metal-organic frameworks (MOFs) for catalysis (e.g., low catalytic activities resulting from blockage of the active metal centers by organic linkers) is of great importance. Herein, we demonstrate the formation of UiO-66 nanoparticles with ultrasmall size and linker defects with the aid of SnS2 nanosheets. The UiO-66 nanoparticles supported by SnS2 nanosheets were found to exhibit excellent catalytic activity for the cycloaddition reaction of CO2 with propylene oxide under solvent-free and co-catalyst-free conditions. Outstandingly, the catalytic activity was 11times higher than that of the pure UiO-66 catalyst under optimum conditions. We thus provide a promising route to modify MOF particles thus to promote their catalytic performance. |
| 电子版国际标准刊号 | 1867-3899 |
| WOS关键词 | METAL-ORGANIC FRAMEWORKS ; CYCLIC CARBONATES ; HETEROGENEOUS CATALYSTS ; CO2 ; EPOXIDES ; TRANSFORMATION ; NANOSHEETS ; DESIGN |
| WOS研究方向 | Chemistry |
| 语种 | 英语 |
| WOS记录号 | WOS:000439756600003 |
| 源URL | [http://ir.ihep.ac.cn/handle/311005/286256]  |
| 专题 | 高能物理研究所_多学科研究中心 高能物理研究所_实验物理中心 |
| 作者单位 | 中国科学院高能物理研究所 |
| 推荐引用方式 GB/T 7714 | Zhang, BX,Cheng, XY,Zheng LR,et al. Tin(IV) Sulfide Greatly Improves the Catalytic Performance of UiO-66 for Carbon Dioxide Cycloaddition[J]. CHEMCATCHEM,2018,10(14):2945-2948. |
| APA | Zhang, BX.,Cheng, XY.,郑黎荣.,张静.,Yang, GY.,...&Shi, JB.(2018).Tin(IV) Sulfide Greatly Improves the Catalytic Performance of UiO-66 for Carbon Dioxide Cycloaddition.CHEMCATCHEM,10(14),2945-2948. |
| MLA | Zhang, BX,et al."Tin(IV) Sulfide Greatly Improves the Catalytic Performance of UiO-66 for Carbon Dioxide Cycloaddition".CHEMCATCHEM 10.14(2018):2945-2948. |
入库方式： OAI收割
来源：高能物理研究所
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