Surface Modulation of Hierarchical MoS2 Nanosheets by Ni Single Atoms for Enhanced Electrocatalytic Hydrogen Evolution
文献类型：期刊论文
| 作者 | Chen, Tao ; Lou, Xiong Wen (David); Chen T(陈涛); Yu, Le; Zhang, Huabin; Zhou, Wei
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| 刊名 | ADVANCED FUNCTIONAL MATERIALS
 |
| 出版日期 | 2018 |
| 卷号 | 28期号:51页码:1807086 |
| 关键词 | hydrogen evolution reaction MoS2 single atoms surface modulation |
| ISSN号 | 1616-301X |
| DOI | 10.1002/adfm.201807086 |
| 文献子类 | Article |
| 英文摘要 | Surface modulation at the atomic level is an important approach for tuning surface chemistry and boosting the catalytic performance. Here, a surface modulation strategy is demonstrated through the decoration of isolated Ni atoms onto the basal plane of hierarchical MoS2 nanosheets supported on multichannel carbon nanofibers for boosted hydrogen evolution activity. X-ray absorption fine structure investigation and density functional theory (DFT) calculation reveal that the MoS2 surface decorated with isolated Ni atoms displays highly strengthened H binding. Benefiting from the unique tubular structure and basal plane modulation, the newly developed MoS2 catalyst exhibits excellent hydrogen evolution activity and stability. This single-atom modification strategy opens up new avenues for tuning the intrinsic catalytic activity toward electrocatalytic water splitting and other energy-related processes. |
| 电子版国际标准刊号 | 1616-3028 |
| WOS关键词 | ACTIVE EDGE SITES ; CATALYTIC-ACTIVITY ; EFFICIENT ; CO ; GRAPHENE ; NANOWIRE ; ENERGY ; FILMS ; FE |
| WOS研究方向 | Chemistry ; Science & Technology - Other Topics ; Materials Science ; Physics |
| 语种 | 英语 |
| WOS记录号 | WOS:000453604700004 |
| 源URL | [http://ir.ihep.ac.cn/handle/311005/286853]  |
| 专题 | 高能物理研究所_多学科研究中心 高能物理研究所_核技术应用研究中心 |
| 作者单位 | 中国科学院高能物理研究所 |
| 推荐引用方式 GB/T 7714 | Chen, Tao,Lou, Xiong Wen ,Chen T,et al. Surface Modulation of Hierarchical MoS2 Nanosheets by Ni Single Atoms for Enhanced Electrocatalytic Hydrogen Evolution[J]. ADVANCED FUNCTIONAL MATERIALS,2018,28(51):1807086. |
| APA | Chen, Tao,Lou, Xiong Wen ,陈涛,Yu, Le,Zhang, Huabin,&Zhou, Wei.(2018).Surface Modulation of Hierarchical MoS2 Nanosheets by Ni Single Atoms for Enhanced Electrocatalytic Hydrogen Evolution.ADVANCED FUNCTIONAL MATERIALS,28(51),1807086. |
| MLA | Chen, Tao,et al."Surface Modulation of Hierarchical MoS2 Nanosheets by Ni Single Atoms for Enhanced Electrocatalytic Hydrogen Evolution".ADVANCED FUNCTIONAL MATERIALS 28.51(2018):1807086. |
入库方式： OAI收割
来源：高能物理研究所
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