Highly stable graphene-oxide-based membranes with superior permeability
文献类型：期刊论文
| 作者 | Thebo, KH; Qian, XT; Zhang, Q; Chen, L; Cheng, HM; Ren, WC; Ren, WC (reprint author), Chinese Acad Sci, Inst Met Res, Shenyang Natl Lab Mat Sci, 72 Wenhua Rd, Shenyang 110016, Liaoning, Peoples R China. |
| 刊名 | NATURE COMMUNICATIONS
 |
| 出版日期 | 2018-04-16 |
| 卷号 | 9页码:- |
| 关键词 | Nanofiltration Membranes Water Reduction Separation Nanosheets Acids Ions |
| ISSN号 | 2041-1723 |
| 英文摘要 | Increasing fresh water demand for drinking and agriculture is one of the grand challenges of our age. Graphene oxide (GO) membranes have shown a great potential for desalination and water purification. However, it is challenging to further improve the water permeability without sacrificing the separation efficiency, and the GO membranes are easily delaminated in aqueous solutions within few hours. Here, we report a class of reduced GO membranes with enlarged interlayer distance fabricated by using theanine amino acid and tannic acid as reducing agent and cross-linker. Such membranes show water permeance over 10,000 Lm(-2) h(-1) bar(-1), which is 10-1000 times higher than those of previously reported GO-based membranes and commercial membranes, and good separation efficiency, e.g., rhodamine B and methylene blue rejection of similar to 100%. Moreover, they show no damage or delamination in water, acid, and basic solutions even after months.; Increasing fresh water demand for drinking and agriculture is one of the grand challenges of our age. Graphene oxide (GO) membranes have shown a great potential for desalination and water purification. However, it is challenging to further improve the water permeability without sacrificing the separation efficiency, and the GO membranes are easily delaminated in aqueous solutions within few hours. Here, we report a class of reduced GO membranes with enlarged interlayer distance fabricated by using theanine amino acid and tannic acid as reducing agent and cross-linker. Such membranes show water permeance over 10,000 Lm(-2) h(-1) bar(-1), which is 10-1000 times higher than those of previously reported GO-based membranes and commercial membranes, and good separation efficiency, e.g., rhodamine B and methylene blue rejection of similar to 100%. Moreover, they show no damage or delamination in water, acid, and basic solutions even after months. |
| 学科主题 | Multidisciplinary Sciences |
| 语种 | 英语 |
| 资助机构 | National Key R&D Program of China [2016YFA0200101]; National Natural Science Foundation of China [51325205, 51290273, 51521091]; Chinese Academy of Sciences [KGZD-EW-303-1, KGZD-EW-T06, 174321KYSB20160011, XDPB06]; CAS-TWAS President Fellowship |
| 公开日期 | 2018-06-05 |
| 源URL | [http://ir.imr.ac.cn/handle/321006/79359]  |
| 专题 | 金属研究所_中国科学院金属研究所 |
| 通讯作者 | Ren, WC (reprint author), Chinese Acad Sci, Inst Met Res, Shenyang Natl Lab Mat Sci, 72 Wenhua Rd, Shenyang 110016, Liaoning, Peoples R China. |
| 推荐引用方式 GB/T 7714 | Thebo, KH,Qian, XT,Zhang, Q,et al. Highly stable graphene-oxide-based membranes with superior permeability[J]. NATURE COMMUNICATIONS,2018,9:-. |
| APA | Thebo, KH.,Qian, XT.,Zhang, Q.,Chen, L.,Cheng, HM.,...&Ren, WC .(2018).Highly stable graphene-oxide-based membranes with superior permeability.NATURE COMMUNICATIONS,9,-. |
| MLA | Thebo, KH,et al."Highly stable graphene-oxide-based membranes with superior permeability".NATURE COMMUNICATIONS 9(2018):-. |
入库方式： OAI收割
来源：金属研究所
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