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Variations of Major Product Derived from Conversion of 5-Hydroxymethylfurfural over a Modified MOFs-Derived Carbon Material in Response to Reaction Conditions

文献类型：期刊论文

作者Wang, Zhenhua1,2; Chen, Qianwang3,4,5
刊名NANOMATERIALS
出版日期2018-07-01
卷号8期号:7页码:9
关键词biomass MOFs precursor 5-hydroxymethylfurfural catalysis carbon material
ISSN号2079-4991
DOI10.3390/nano8070492
通讯作者Wang, Zhenhua(zhenhuaw@mail.ustc.edu.cn)
英文摘要In recent years, the conversion of 5-hydroxymethylfurfural (HMF) into 5-ethoxymethylfurfural (EMF) and ethyl levulinate (EL) has become an attractive biomass transformation route due to their potential applications in the energy and chemical industries. In this study, we have developed an effective method to prepare a catalyst for this reaction. Sulfonic-acid-functionalized carbon nanomaterials (C-SO3H), prepared from the direct pyrolysis of Metal-Organic Frameworks (MOFs) precursor Cu-benzene-1,3,5-tricarboxylate (Cu-BTC) followed by acidification with sulfuric acid, show excellent catalytic activity with a total yield higher than 90%. It is interesting that, different from the previous catalysts, a different major product-EMF or EL-can be selectively obtained by controlling the reaction temperature and time.
WOS关键词SUPPORTED PHOSPHOTUNGSTIC ACID ; GAMMA-VALEROLACTONE ; ETHYL LEVULINATE ; LIGNOCELLULOSIC BIOMASS ; CATALYTIC CONVERSION ; IONIC LIQUIDS ; FRUCTOSE ; FUELS ; ETHERIFICATION ; CHEMICALS
资助项目National Natural Science Foundation (NSFC)[21271163] ; National Natural Science Foundation (NSFC)[U1232211] ; CAS/SAFEA international partnership program for creative research teams ; CAS Hefei Science Center[2016HSC-IU011]
WOS研究方向Science & Technology - Other Topics ; Materials Science
语种英语
WOS记录号WOS:000442523100043
出版者MDPI
资助机构National Natural Science Foundation (NSFC) ; National Natural Science Foundation (NSFC) ; National Natural Science Foundation (NSFC) ; National Natural Science Foundation (NSFC) ; National Natural Science Foundation (NSFC) ; National Natural Science Foundation (NSFC) ; National Natural Science Foundation (NSFC) ; National Natural Science Foundation (NSFC) ; National Natural Science Foundation (NSFC) ; National Natural Science Foundation (NSFC) ; National Natural Science Foundation (NSFC) ; National Natural Science Foundation (NSFC) ; National Natural Science Foundation (NSFC) ; National Natural Science Foundation (NSFC) ; National Natural Science Foundation (NSFC) ; National Natural Science Foundation (NSFC) ; National Natural Science Foundation (NSFC) ; National Natural Science Foundation (NSFC) ; National Natural Science Foundation (NSFC) ; National Natural Science Foundation (NSFC) ; National Natural Science Foundation (NSFC) ; National Natural Science Foundation (NSFC) ; National Natural Science Foundation (NSFC) ; 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源URL[http://ir.hfcas.ac.cn:8080/handle/334002/37945]  
专题中国科学院合肥物质科学研究院
通讯作者Wang, Zhenhua
作者单位1.Chongqing Univ Sci & Technol, Sch Met & Mat Engn, Chongqing 401331, Peoples R China
2.Chongqing Key Lab Nano Micro Composite Mat & Devi, Chongqing 401331, Peoples R China
3.Univ Sci & Technol China, Collaborat Innovat Ctr Suzhou Nano Sci & Technol, Hefei Natl Lab Phys Sci Microscale, Hefei 230026, Peoples R China
4.Univ Sci & Technol China, Collaborat Innovat Ctr Suzhou Nano Sci & Technol, Dept Mat Sci & Engn, Hefei 230026, Peoples R China
5.Chinese Acad Sci, High Field Magnet Lab, Hefei 230031, Peoples R China
推荐引用方式
GB/T 7714		 Wang, Zhenhua,Chen, Qianwang. Variations of Major Product Derived from Conversion of 5-Hydroxymethylfurfural over a Modified MOFs-Derived Carbon Material in Response to Reaction Conditions[J]. NANOMATERIALS,2018,8(7):9.
APA Wang, Zhenhua,&Chen, Qianwang.(2018).Variations of Major Product Derived from Conversion of 5-Hydroxymethylfurfural over a Modified MOFs-Derived Carbon Material in Response to Reaction Conditions.NANOMATERIALS,8(7),9.
MLA Wang, Zhenhua,et al."Variations of Major Product Derived from Conversion of 5-Hydroxymethylfurfural over a Modified MOFs-Derived Carbon Material in Response to Reaction Conditions".NANOMATERIALS 8.7(2018):9.

入库方式： OAI收割

来源：合肥物质科学研究院

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