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  4. 中科院等离子体物理研究所
Heavy-ion irradiation effects on U3O8 incorporated Gd2Zr2O7 waste forms

文献类型：期刊论文

作者Lu, Xirui1; Shu, Xiaoyan1; Chen, Shunzhang1; Zhang, Kuibao1; Chi, Fangtin1; Zhang, Haibin2; Shao, Dadong3; Mao, Xueli1
刊名JOURNAL OF HAZARDOUS MATERIALS
出版日期2018-09-05
卷号357页码:424-430
关键词Gd(2)Zr(2)O(7)pyrochlore U3O8 Heavy-ion irradiation Radiation tolerance Amorphization
ISSN号0304-3894
DOI10.1016/j.jhazmat.2018.06.026
通讯作者Lu, Xirui(luxiruimvp116@163.com) ; Zhang, Haibin(wsschbinzhang@163.com)
英文摘要In this research, the heavy-ion irradiation effects of U-bearing Gd2Zr2O7 ceramics were explored for nuclear waste immobilization. U3O8 was designed to be incorporated into Gd2Zr2O7 from two different routes in the form of (Gd1-4xU2x)(2)(Zr1-xUx)O-7 (x = 0.1, 0.14). The self-irradiation of actinide nuclides was simulated by Xe20+ heavy-ion radiation under different fluences. Grazing incidence X-ray diffraction (GIXRD) analysis reveals the relationship between radiation dose, damage and depth. The radiation tolerance is promoted with the increment of U3O8 content in the discussed range. Raman spectroscopy testifies the enhancement of radiation tolerance and microscopically existed phase evolution from the chemical bond vibrations. In addition, the microstructure and elemental distribution of the irradiated samples were analyzed as well. The amorphization degree of the sample surface declines as the U content was elevated from x = 0.1 to x = 0.14.
WOS关键词RAMAN-SPECTROSCOPY ; STRUCTURAL TRANSFORMATION ; PYROCHLORE STRUCTURE ; RESIDUAL-STRESS ; IMMOBILIZATION ; CERAMICS ; OXIDES ; URANIUM ; ACCUMULATION ; STABILITY
资助项目National Natural Science Foundation of China[21507105] ; National Natural Science Foundation of China[51672228] ; Key Project of Sichuan Education Department[15ZB0116] ; Foundation of Fundamental Science on Nuclear Wastes and Environmental Safety Laboratory, Southwest University of Science and Technology[15yyhk10]
WOS研究方向Engineering ; Environmental Sciences & Ecology
语种英语
WOS记录号WOS:000440958900046
出版者ELSEVIER SCIENCE BV
资助机构National Natural Science Foundation of China ; National Natural Science Foundation of China ; National Natural Science Foundation of China ; National Natural Science Foundation of China ; National Natural Science Foundation of China ; National Natural Science Foundation of China ; National Natural Science Foundation of China ; National Natural Science Foundation of China ; National Natural Science Foundation of China ; National Natural Science Foundation of China ; National Natural Science Foundation of China ; National Natural Science Foundation of China ; National Natural Science Foundation of China ; National Natural Science Foundation of China ; National Natural Science Foundation of China ; National Natural Science Foundation of China ; National Natural Science Foundation of China ; National Natural Science Foundation of China ; National Natural Science Foundation of China ; National Natural Science Foundation of China ; National Natural Science Foundation of China ; National Natural Science Foundation of China ; 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源URL[http://ir.hfcas.ac.cn:8080/handle/334002/37703]  
专题合肥物质科学研究院_中科院等离子体物理研究所
通讯作者Lu, Xirui; Zhang, Haibin
作者单位1.Southwest Univ Sci & Technol, Fundamental Sci Nucl Wastes & Environm Safety Lab, Mianyang 621010, Sichuan, Peoples R China
2.China Acad Engn Phys, Inst Nucl Phys & Chem, Mianyang 621010, Sichuan, Peoples R China
3.Chinese Acad Sci, Inst Plasma Phys, POB 1126, Hefei 230031, Peoples R China
推荐引用方式
GB/T 7714		 Lu, Xirui,Shu, Xiaoyan,Chen, Shunzhang,et al. Heavy-ion irradiation effects on U3O8 incorporated Gd2Zr2O7 waste forms[J]. JOURNAL OF HAZARDOUS MATERIALS,2018,357:424-430.
APA Lu, Xirui.,Shu, Xiaoyan.,Chen, Shunzhang.,Zhang, Kuibao.,Chi, Fangtin.,...&Mao, Xueli.(2018).Heavy-ion irradiation effects on U3O8 incorporated Gd2Zr2O7 waste forms.JOURNAL OF HAZARDOUS MATERIALS,357,424-430.
MLA Lu, Xirui,et al."Heavy-ion irradiation effects on U3O8 incorporated Gd2Zr2O7 waste forms".JOURNAL OF HAZARDOUS MATERIALS 357(2018):424-430.

入库方式： OAI收割

来源：合肥物质科学研究院

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