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  4. 中科院固体物理研究所
Bifunctional Hybrid Ni/Ni2P Nanoparticles Encapsulated by Graphitic Carbon Supported with N, S Modified 3D Carbon Framework for Highly Efficient Overall Water Splitting

文献类型：期刊论文

作者Sun, Yiqiang1,2; Zhang, Tao1,2; Li, Xinyang1; Bai, Yu1; Lyu, Xianjun3; Liu, Guangqiang1; Cai, Weiping1; Li, Yue1
刊名ADVANCED MATERIALS INTERFACES
出版日期2018-08-09
卷号5期号:15页码:9
关键词bifunctional electrocatalyst hybrid structures hydrogen evolution water oxidation water splitting
ISSN号2196-7350
DOI10.1002/admi.201800473
通讯作者Li, Yue(yueli@issp.ac.cn)
英文摘要The novel hybrid Ni/Ni2P nanoparticles with graphitic carbon coating supported by 3D N, S dual modified binder-free macroporous carbon framework (Ni/Ni2P@3DNSC) are reported as an efficient bifunctional electrocatalysts for the production of hydrogen and oxygen. The obtained Ni/Ni2P@3DNSC electrode exhibits an excellent catalytic activity with a low overpotential of 231 mV for oxygen evolution reaction (OER) and 92 mV for hydrogen evolution reaction (HER) due to the strong coupled interface of Ni and Ni2P, synergistic effects between the hybrid Ni/Ni2P core and the graphitic carbon shell, the unique porous structure, and the heteroatoms doped effect. When both are used as cathode and anode, only a low cell voltage of 1.55 V is needed to achieve the current density of 10 mA cm(-2). This work demonstrates a new avenue for the development of bifunctional nonprecious electrocatalysts for the sustainable energy utilization.
WOS关键词HYDROGEN EVOLUTION REACTION ; NANOSTRUCTURED NICKEL PHOSPHIDE ; OXYGEN EVOLUTION ; ACTIVE ELECTROCATALYST ; MELAMINE FOAM ; DOPED CARBON ; OXIDATION ; SULFIDE ; ARRAYS ; NANOCRYSTALS
资助项目National Key Research and Development Program of China[2017YFA0207101] ; Natural Science Foundation of China[51771188] ; Natural Science Foundation of China[51571189] ; Anhui Provincial Natural Science Foundation[1508085JGD07] ; Cross-disciplinary Collaborative Teams Program in CAS ; CAS/SAFEA International Partnership Program for Creative Research Teams
WOS研究方向Chemistry ; Materials Science
语种英语
WOS记录号WOS:000441125500023
出版者WILEY
资助机构National Key Research and Development Program of China ; National Key Research and Development Program of China ; National Key Research and Development Program of China ; National Key Research and Development Program of China ; National Key Research and Development Program of China ; National Key Research and Development Program of China ; National Key Research and Development Program of China ; National Key Research and Development Program of China ; National Key Research and Development Program of China ; National Key Research and Development Program of China ; National Key Research and Development Program of China ; National Key Research and Development Program of China ; National Key Research and Development Program of China ; National Key Research and Development Program of China ; National Key Research and Development Program of China ; National Key Research and Development Program of China ; Natural Science Foundation of China ; Natural Science Foundation of China ; Natural Science Foundation of China ; 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源URL[http://ir.hfcas.ac.cn:8080/handle/334002/37661]  
专题合肥物质科学研究院_中科院固体物理研究所
通讯作者Li, Yue
作者单位1.Chinese Acad Sci, Inst Solid State Phys, Anhui Key Lab Nanomat & Nanotechnol, Key Lab Mat Phys, Hefei 230031, Peoples R China
2.Univ Sci & Technol China, Sci Isl Branch, Hefei 230026, Peoples R China
3.Shandong Univ Sci & Technol, Coll Chem & Environm Engn, Qingdao 266590, Shandong, Peoples R China
推荐引用方式
GB/T 7714		 Sun, Yiqiang,Zhang, Tao,Li, Xinyang,et al. Bifunctional Hybrid Ni/Ni2P Nanoparticles Encapsulated by Graphitic Carbon Supported with N, S Modified 3D Carbon Framework for Highly Efficient Overall Water Splitting[J]. ADVANCED MATERIALS INTERFACES,2018,5(15):9.
APA Sun, Yiqiang.,Zhang, Tao.,Li, Xinyang.,Bai, Yu.,Lyu, Xianjun.,...&Li, Yue.(2018).Bifunctional Hybrid Ni/Ni2P Nanoparticles Encapsulated by Graphitic Carbon Supported with N, S Modified 3D Carbon Framework for Highly Efficient Overall Water Splitting.ADVANCED MATERIALS INTERFACES,5(15),9.
MLA Sun, Yiqiang,et al."Bifunctional Hybrid Ni/Ni2P Nanoparticles Encapsulated by Graphitic Carbon Supported with N, S Modified 3D Carbon Framework for Highly Efficient Overall Water Splitting".ADVANCED MATERIALS INTERFACES 5.15(2018):9.

入库方式： OAI收割

来源：合肥物质科学研究院

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