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Strong Electronic Interaction in Dual-Cation-Incorporated NiSe2 Nanosheets with Lattice Distortion for Highly Efficient Overall Water Splitting

文献类型：期刊论文

作者Sun, Yiqiang1,2; Xu, Kun3; Wei, Zengxi4; Li, Huilin1,2; Zhang, Tao1,2; Li, Xinyang1; Cai, Weiping1; Ma, Jianmin4; Fan, Hong Jin3; Li, Yue1
刊名ADVANCED MATERIALS
出版日期2018-08-29
卷号30期号:35页码:7
关键词bifunctional electrocatalyst dual-cation metal doping electronic interaction lattice distortion water splitting
ISSN号0935-9648
DOI10.1002/adma.201802121
通讯作者Fan, Hong Jin(fanhj@ntu.edu.sg) ; Li, Yue(yueli@issp.ac.cn)
英文摘要Exploring highly efficient and low-cost electrocatalysts for electrochemical water splitting is of importance for the conversion of intermediate energy. Herein, the synthesis of dual-cation (Fe, Co)-incorporated NiSe2 nanosheets (Fe, Co-NiSe2) and systematical investigation of their electrocatalytic performance for water splitting as a function of the composition are reported. The dual-cation incorporation can distort the lattice and induce stronger electronic interaction, leading to increased active site exposure and optimized adsorption energy of reaction intermediates compared to single-cation-doped or pure NiSe2. As a result, the obtained Fe0.09Co0.13-NiSe2 porous nanosheet electrode shows an optimized catalytic activity with a low overpotential of 251 mV for oxygen evolution reaction and 92 mV for hydrogen evolution reaction (both at 10 mA cm(-2) in 1 m KOH). When used as bifunctional electrodes for overall water splitting, the current density of 10 mA cm(-2) is achieved at a low cell voltage of 1.52 V. This work highlights the importance of dual-cation doping in enhancing the electrocatalyst performance of transition metal dichalcogenides.
WOS关键词OXYGEN EVOLUTION REACTION ; HYDROGEN EVOLUTION ; BIFUNCTIONAL ELECTROCATALYST ; OXIDATION ; CATALYSTS ; GENERATION ; NANOWIRES ; FILM ; NANOPARTICLES ; SCAFFOLDS
资助项目National Key Research and Development Program of China[2017YFA0207101] ; Natural Science Foundation of China[51771188] ; Natural Science Foundation of China[51371165] ; Natural Science Foundation of China[51571189] ; Cross-disciplinary Collaborative Teams Program in CAS ; CAS/SAFEA International Partnership Program for Creative Research Teams ; Major Program of Development Foundation of Hefei Center for Physical Science and Technology[2017FXZY002] ; Singapore Ministry of Education Tier 1 grant[RG117/16]
WOS研究方向Chemistry ; Science & Technology - Other Topics ; Materials Science ; Physics
语种英语
WOS记录号WOS:000442732400016
出版者WILEY-V C H VERLAG GMBH
资助机构National Key Research and Development Program of China ; National Key Research and Development Program of China ; National Key Research and Development Program of China ; National Key Research and Development Program of China ; National Key Research and Development Program of China ; National Key Research and Development Program of China ; National Key Research and Development Program of China ; National Key Research and Development Program of China ; National Key Research and Development Program of China ; National Key Research and Development Program of China ; National Key Research and Development Program of China ; National Key Research and Development Program of China ; National Key Research and Development Program of China ; National Key Research and Development Program of China ; National Key Research and Development Program of China ; National Key Research and Development Program of China ; Natural Science Foundation of China ; Natural Science Foundation of China ; Natural Science Foundation of China ; 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Singapore Ministry of Education Tier 1 grant ; Singapore Ministry of Education Tier 1 grant ; Singapore Ministry of Education Tier 1 grant ; Singapore Ministry of Education Tier 1 grant ; Singapore Ministry of Education Tier 1 grant ; Singapore Ministry of Education Tier 1 grant ; Singapore Ministry of Education Tier 1 grant ; Singapore Ministry of Education Tier 1 grant ; Singapore Ministry of Education Tier 1 grant ; Singapore Ministry of Education Tier 1 grant ; Singapore Ministry of Education Tier 1 grant ; Singapore Ministry of Education Tier 1 grant ; Singapore Ministry of Education Tier 1 grant ; Singapore Ministry of Education Tier 1 grant
源URL[http://ir.hfcas.ac.cn:8080/handle/334002/38049]  
专题合肥物质科学研究院_中科院固体物理研究所
通讯作者Fan, Hong Jin; Li, Yue
作者单位1.Chinese Acad Sci, Inst Solid State Phys, Anhui Key Lab Nanomat & Nanotechnol, Key Lab Mat Phys, Hefei 230031, Anhui, Peoples R China
2.Univ Sci & Technol China, Sci Isl Branch, Hefei 230026, Anhui, Peoples R China
3.Nanyang Technol Univ, Sch Phys & Math Sci, 21 Nanyang Link, Singapore 637371, Singapore
4.Hunan Univ, Sch Phys & Elect, Changsha 410082, Hunan, Peoples R China
推荐引用方式
GB/T 7714		 Sun, Yiqiang,Xu, Kun,Wei, Zengxi,et al. Strong Electronic Interaction in Dual-Cation-Incorporated NiSe2 Nanosheets with Lattice Distortion for Highly Efficient Overall Water Splitting[J]. ADVANCED MATERIALS,2018,30(35):7.
APA Sun, Yiqiang.,Xu, Kun.,Wei, Zengxi.,Li, Huilin.,Zhang, Tao.,...&Li, Yue.(2018).Strong Electronic Interaction in Dual-Cation-Incorporated NiSe2 Nanosheets with Lattice Distortion for Highly Efficient Overall Water Splitting.ADVANCED MATERIALS,30(35),7.
MLA Sun, Yiqiang,et al."Strong Electronic Interaction in Dual-Cation-Incorporated NiSe2 Nanosheets with Lattice Distortion for Highly Efficient Overall Water Splitting".ADVANCED MATERIALS 30.35(2018):7.

入库方式： OAI收割

来源：合肥物质科学研究院

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