中国科学院机构知识库网格
Chinese Academy of Sciences Institutional Repositories Grid
Low energy (e, 2e) study from the 1t(2) orbital of CH4

文献类型:期刊论文

作者Ullrich, J.1,6; Xu, S.1,2; Chaluvadi, Hari3; Ren, X.1; Pflueger, T.1; Senftleben, A.1; Ning, C. G.4,5; Yan, S.2; Zhang, P.2; Yang, J.2
刊名JOURNAL OF CHEMICAL PHYSICS
出版日期2012-07-14
卷号137
ISSN号0021-9606
DOI10.1063/1.4732539
文献子类Article
英文摘要Single ionization of the methane (CH4) 1t(2) orbital by 54 eV electron impact has been studied experimentally and theoretically. The measured triple differential cross sections cover nearly a 4 pi solid angle for the emission of low energy electrons and a range of projectile scattering angles. Experimental data are compared with theoretical calculations from the distorted wave Born approximation and the molecular three-body distorted wave models. It is found that theory can give a proper description of the main features of experimental cross section only at smaller scattering angles. For larger scattering angles, significant discrepancies between experiment and theory are observed. The importance of the strength of nuclear scattering from the H-nuclei was theoretically tested by reducing the distance between the carbon nuclei and the hydrogen nuclei and improved agreement with experiment was found for both the scattering plane and the perpendicular plane. (C) 2012 American Institute of Physics. [http://dx.doi.org/10.1063/1.4732539]
WOS关键词CROSS-SECTIONS ; MOLECULAR-ORBITALS ; ELECTRON-IMPACT ; IONIZATION ; DENSITY ; MODEL ; E,2E
资助项目National Natural Science Foundation of China (NNSFC)[10979007] ; National Natural Science Foundation of China (NNSFC)[10674140] ; National Natural Science Foundation of China (NNSFC)[10704046]
WOS研究方向Chemistry ; Physics
语种英语
WOS记录号WOS:000306361000011
出版者AMER INST PHYSICS
源URL[http://119.78.100.186/handle/113462/48747]  
专题近代物理研究所_实验物理中心
通讯作者Ma, X.
作者单位1.Max Planck Inst Kernphys, D-69117 Heidelberg, Germany
2.Chinese Acad Sci, Inst Modern Phys, Lanzhou 730000, Peoples R China
3.Missouri Univ Sci & Technol, Dept Phys, Rolla, MO 65409 USA
4.Tsinghua Univ, Dept Phys, Beijing 100084, Peoples R China
5.Tsinghua Univ, State Key Lab Low Dimens Quantum Phys, Beijing 100084, Peoples R China
6.Phys Tech Bundesanstalt, D-38116 Braunschweig, Germany
推荐引用方式
GB/T 7714
Ullrich, J.,Xu, S.,Chaluvadi, Hari,et al. Low energy (e, 2e) study from the 1t(2) orbital of CH4[J]. JOURNAL OF CHEMICAL PHYSICS,2012,137.
APA Ullrich, J..,Xu, S..,Chaluvadi, Hari.,Ren, X..,Pflueger, T..,...&Dorn, A..(2012).Low energy (e, 2e) study from the 1t(2) orbital of CH4.JOURNAL OF CHEMICAL PHYSICS,137.
MLA Ullrich, J.,et al."Low energy (e, 2e) study from the 1t(2) orbital of CH4".JOURNAL OF CHEMICAL PHYSICS 137(2012).

入库方式: OAI收割

来源:近代物理研究所

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