Ultrasonic synthesis of nitrogen-doped carbon nanofibers as platinum catalyst support for oxygen reduction
文献类型：期刊论文
| 作者 | Jiang Y ; Zhang J ; Qin YH ; Niu DF ; Zhang XS ; Niu L ; Zhou XG ; Lu TH ; Yuan WK |
| 刊名 | journal of power sources
 |
| 出版日期 | 2011 |
| 卷号 | 196期号:22页码:9356-9360 |
| 关键词 | FUEL-CELLS HIGH-PERFORMANCE NANOTUBES ELECTRODES SURFACE PHTHALOCYANINE OXIDATION GRAPHITE FILM |
| ISSN号 | 0378-7753 |
| 通讯作者 | zhang xs |
| 中文摘要 | oxygen- and nitrogen-containing groups are successfully introduced onto the carbon nanofiber (cnf) surfaces by sonochemical treatment in mixed acids (concentrated sulfuric acid and nitric acid) and ammonia, respectively. pt electrocatalysts supported on the acid-treated cnf (cnf-o) and ammonia-treated cnf (cnf-on) are prepared and the effect of cnf surface functional groups on the electrocatalytic activities of supported catalysts for oxygen reduction reaction (orr) is investigated. high resolution transmission electron microscopy reveals that pt particles are uniformly dispersed on the two cnf supports and the cnf-on supported pt nanoparticles have a smaller average particle size and a more uniform particle size distribution. cyclic voltammetric analysis shows the pt/cnf-on has a larger electrochemically active surface area than pt/cnf-o. rotating disk electrode measurements show that the pt/cnf-on exhibits a considerably higher electrocatalytic activity toward orr as compared with pt/cnf-o. it is believed that the good electrocatalytic activity of pt/cnf-on can be attributed to the smaller pt particle size and more uniform particle size distribution, to the synergistic effect and the enhanced pt-cnf-on interaction, and to the unique structural and electronic properties of cnf-on. (c) 2011 elsevier b.v. all rights reserved. |
| 收录类别 | SCI收录期刊论文 |
| 语种 | 英语 |
| WOS记录号 | WOS:000295602400034 |
| 公开日期 | 2012-06-08 |
| 源URL | [http://ir.ciac.jl.cn/handle/322003/44223]  |
| 专题 | 长春应用化学研究所_长春应用化学研究所知识产出_期刊论文 |
| 推荐引用方式 GB/T 7714 | Jiang Y,Zhang J,Qin YH,et al. Ultrasonic synthesis of nitrogen-doped carbon nanofibers as platinum catalyst support for oxygen reduction[J]. journal of power sources,2011,196(22):9356-9360. |
| APA | Jiang Y.,Zhang J.,Qin YH.,Niu DF.,Zhang XS.,...&Yuan WK.(2011).Ultrasonic synthesis of nitrogen-doped carbon nanofibers as platinum catalyst support for oxygen reduction.journal of power sources,196(22),9356-9360. |
| MLA | Jiang Y,et al."Ultrasonic synthesis of nitrogen-doped carbon nanofibers as platinum catalyst support for oxygen reduction".journal of power sources 196.22(2011):9356-9360. |
入库方式： OAI收割
来源：长春应用化学研究所
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