A Microstructured Graphene/Poly(N-isopropylacrylamide) Membrane for Intelligent Solar Water Evaporation
文献类型:期刊论文
作者 | Zhang PP4,5; Liu F(刘峰)3![]() |
刊名 | ANGEWANDTE CHEMIE-INTERNATIONAL EDITION
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出版日期 | 2018-12-10 |
卷号 | 57期号:50页码:16343-16347 |
关键词 | irradiation membranes polymers self-adaptive materials water evaporation |
ISSN号 | 1433-7851 |
DOI | 10.1002/anie.201810345 |
通讯作者 | Qu, Liangti(lqu@mail.tsinghua.edu.cn) |
英文摘要 | Intelligent solar water evaporation (iSWE) was achieved with a thermally responsive and microstructured graphene/poly(N-isopropylacrylamide) (mG/PNIPAm) membrane. As the solar intensity varies, the water evaporation is tuned through reversible transformations of microstructures reminiscent of the stomatal opening and closing of leaves. Consequently, this mG/PNIPAm membrane displays a high water evaporation rate change (Delta WER) of 1.66 kg m(-2) h(-1) under weak sunlight (intensity < 1 sun) and a low WER of 0.24 kg m(-2) h(-1) under intense sunlight (1sun < intensity < 2 sun). Because of the double-layer structure with predictable shape and dynamics, the leaf-like membrane can further autonomously modulate the water evaporation by self-curling under intense solar irradiation in accordance with simulation results. This mG/PNIPAm membrane provides a smart material platform with self-adaptability in response to changing environments. |
分类号 | 一类 |
WOS关键词 | GRAPHENE OXIDE ; STEAM-GENERATION ; ONE SUN ; STOMATA ; HYDROGELS ; EFFICIENT ; PLANTS ; PNIPAM |
资助项目 | Ministry of Science and Technology of China[2017YFB1104300] ; Ministry of Science and Technology of China[2016YFA0200200] ; NSFC[51673026] ; NSFC[51433005] ; NSFC[21674056] ; Beijing Natural Science Foundation[2152028] ; Beijing Municipal Science and Technology Commission[Z161100002116022] ; Beijing Municipal Science and Technology Commission[Z161100002116029] ; National Natural Science Foundation of China[11602272] ; National Natural Science Foundation of China[11790292] ; Strategic Priority Research Program of the Chinese Academy of Sciences[XDB22040503] ; NSFCMAECI[51861135202] |
WOS研究方向 | Chemistry |
语种 | 英语 |
WOS记录号 | WOS:000453346300014 |
资助机构 | Ministry of Science and Technology of China ; NSFC ; Beijing Natural Science Foundation ; Beijing Municipal Science and Technology Commission ; National Natural Science Foundation of China ; Strategic Priority Research Program of the Chinese Academy of Sciences ; NSFCMAECI |
源URL | [http://dspace.imech.ac.cn/handle/311007/78964] ![]() |
专题 | 力学研究所_非线性力学国家重点实验室 |
作者单位 | 1.Beijing Inst Technol, Sch Chem & Chem Engn, Beijing 100081, Peoples R China 2.Tsinghua Univ, Dept Chem, Beijing 100084, Peoples R China; 3.Chinese Acad Sci, Inst Mech, State Key Lab Nonlinear Mech, Beijing 100190, Peoples R China; 4.Tsinghua Univ, Dept Mech Engn, State Key Lab Tribol, Beijing 100084, Peoples R China; 5.Minist Educ China, Key Lab Adv Mat Proc Technol, Beijing 100084, Peoples R China; |
推荐引用方式 GB/T 7714 | Zhang PP,Liu F,Liao QH,et al. A Microstructured Graphene/Poly(N-isopropylacrylamide) Membrane for Intelligent Solar Water Evaporation[J]. ANGEWANDTE CHEMIE-INTERNATIONAL EDITION,2018,57(50):16343-16347. |
APA | Zhang PP.,刘峰.,Liao QH.,Yao HZ.,Geng HY.,...&Qu LT.(2018).A Microstructured Graphene/Poly(N-isopropylacrylamide) Membrane for Intelligent Solar Water Evaporation.ANGEWANDTE CHEMIE-INTERNATIONAL EDITION,57(50),16343-16347. |
MLA | Zhang PP,et al."A Microstructured Graphene/Poly(N-isopropylacrylamide) Membrane for Intelligent Solar Water Evaporation".ANGEWANDTE CHEMIE-INTERNATIONAL EDITION 57.50(2018):16343-16347. |
入库方式: OAI收割
来源:力学研究所
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