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  4. 中科院固体物理研究所
A Localized High-Concentration Electrolyte with Optimized Solvents and Lithium Difluoro(oxalate)borate Additive for Stable Lithium Metal Batteries

文献类型：期刊论文

作者Yu, Lu1; Chen, Shuru1; Lee, Hongkyung1; Zhang, Linchao1,2; Engelhard, Mark H.3; Li, Qiuyan1; Jiao, Shuhong1; Liu, Jun1; Xu, Wu1; Zhang, Ji-Guang1
刊名ACS ENERGY LETTERS
出版日期2018-09-01
卷号3期号:9页码:2059-2067
ISSN号2380-8195
DOI10.1021/acsenergylett.8b00935
通讯作者Xu, Wu(wu.xu@pnnl.gov) ; Zhang, Ji-Guang(jiguang.zhang@pnnl.gov)
英文摘要We report a carbonate-based localized high-concentration electrolyte (LHCE) with a fluorinated ether as a diluent for 4-V class lithium metal batteries (LMBs), which enables dendrite-free Li deposition with a high Li Coulombic efficiency (similar to 98.5%) and much better cycling stability for Li metal anodes than previously reported dimethyl carbonate-based LHCEs at lean electrolyte conditions. This electrolyte consists of 1.2 M lithium bis(fluorosulfonyl)imide (LiFSI) in a cosolvent mixture of ethylene carbonate (EC)/ethyl methyl carbonate (EMC) with bis(2,2,2-trifluoroethyl) ether (BTFE) as the diluent and 0.15 M lithium difluoro(oxalate)borate (LiDFOB) as an additive. A Li parallel to LiNi1/3Mn1/3 Co1/3O2 battery with a high areal loading of 3.8 mAh cm(-2) maintains 84% of its initial capacity after 100 cycles. The enhanced stability can be attributed to the robust solid-electrolyte interface (SEI) layer formed on the Li metal decomposition of LiDFOB salt and EC solvent molecules.
WOS关键词ION BATTERIES ; ANODE ; DIFLUORO(OXALATO)BORATE ; CAPACITY ; SALT
资助项目Assistant Secretary for Energy Efficiency and Renewable Energy, Office of Vehicle Technologies of the U.S. Department of Energy (DOE) through the Advanced Battery Materials Research (BMR) program (Battery500 Consortium)[DE-AC02-05CH11231] ; DOE's Office of Biological and Environmental Research ; DOE[DE-AC05-76RL01830] ; DOE Vehicle Technologies Program within Applied Battery Research (ABR) for Transportation Program
WOS研究方向Chemistry ; Electrochemistry ; Energy & Fuels ; Science & Technology - Other Topics ; Materials Science
语种英语
出版者AMER CHEMICAL SOC
WOS记录号WOS:000445052900006
资助机构Assistant Secretary for Energy Efficiency and Renewable Energy, Office of Vehicle Technologies of the U.S. Department of Energy (DOE) through the Advanced Battery Materials Research (BMR) program (Battery500 Consortium) ; Assistant Secretary for Energy Efficiency and Renewable Energy, Office of Vehicle Technologies of the U.S. Department of Energy (DOE) through the Advanced Battery Materials Research (BMR) program (Battery500 Consortium) ; Assistant Secretary for Energy Efficiency and Renewable Energy, Office of Vehicle Technologies of the U.S. Department of Energy (DOE) through the Advanced Battery Materials Research (BMR) program (Battery500 Consortium) ; Assistant Secretary for Energy Efficiency and Renewable Energy, Office of Vehicle Technologies of the U.S. Department of Energy (DOE) through the Advanced Battery Materials Research (BMR) program (Battery500 Consortium) ; Assistant Secretary for Energy Efficiency and Renewable Energy, Office of Vehicle Technologies of the U.S. Department of Energy (DOE) through the Advanced Battery Materials Research (BMR) program (Battery500 Consortium) ; Assistant Secretary for Energy Efficiency and Renewable Energy, Office of Vehicle Technologies of the U.S. Department of Energy (DOE) through the Advanced Battery Materials Research (BMR) program (Battery500 Consortium) ; Assistant Secretary for Energy Efficiency and Renewable Energy, Office of Vehicle Technologies of the U.S. Department of Energy (DOE) through the Advanced Battery Materials Research (BMR) program (Battery500 Consortium) ; Assistant Secretary for Energy Efficiency and Renewable Energy, Office of Vehicle Technologies of the U.S. Department of Energy (DOE) through the Advanced Battery Materials Research (BMR) program (Battery500 Consortium) ; Assistant Secretary for Energy Efficiency and Renewable Energy, Office of Vehicle Technologies of the U.S. Department of Energy (DOE) through the Advanced Battery Materials Research (BMR) program (Battery500 Consortium) ; Assistant Secretary for Energy Efficiency and Renewable Energy, Office of Vehicle Technologies of the U.S. Department of Energy (DOE) through the Advanced Battery Materials Research (BMR) program (Battery500 Consortium) ; 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源URL[http://ir.hfcas.ac.cn:8080/handle/334002/38852]  
专题合肥物质科学研究院_中科院固体物理研究所
通讯作者Xu, Wu; Zhang, Ji-Guang
作者单位1.Pacific Northwest Natl Lab, Energy & Environm Directorate, 902 Battelle Blvd, Richland, WA 99354 USA
2.Chinese Acad Sci, Inst Solid State Phys, Key Lab Mat Phys, Hefei 230026, Anhui, Peoples R China
3.Pacific Northwest Natl Lab, Environm Mol Sci Lab, 3335 Innovat Blvd, Richland, WA 99354 USA
推荐引用方式
GB/T 7714		 Yu, Lu,Chen, Shuru,Lee, Hongkyung,et al. A Localized High-Concentration Electrolyte with Optimized Solvents and Lithium Difluoro(oxalate)borate Additive for Stable Lithium Metal Batteries[J]. ACS ENERGY LETTERS,2018,3(9):2059-2067.
APA Yu, Lu.,Chen, Shuru.,Lee, Hongkyung.,Zhang, Linchao.,Engelhard, Mark H..,...&Zhang, Ji-Guang.(2018).A Localized High-Concentration Electrolyte with Optimized Solvents and Lithium Difluoro(oxalate)borate Additive for Stable Lithium Metal Batteries.ACS ENERGY LETTERS,3(9),2059-2067.
MLA Yu, Lu,et al."A Localized High-Concentration Electrolyte with Optimized Solvents and Lithium Difluoro(oxalate)borate Additive for Stable Lithium Metal Batteries".ACS ENERGY LETTERS 3.9(2018):2059-2067.

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来源：合肥物质科学研究院

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