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A Localized High-Concentration Electrolyte with Optimized Solvents and Lithium Difluoro(oxalate)borate Additive for Stable Lithium Metal Batteries

文献类型：期刊论文

作者Yu, Lu1; Chen, Shuru1; Lee, Hongkyung1; Zhang, Linchao1,2; Engelhard, Mark H.3; Li, Qiuyan1; Jiao, Shuhong1; Liu, Jun1; Xu, Wu1; Zhang, Ji-Guang1
刊名ACS ENERGY LETTERS
出版日期2018-09-01
卷号3期号:9页码:2059-2067
ISSN号2380-8195
DOI10.1021/acsenergylett.8b00935
通讯作者Xu, Wu(wu.xu@pnnl.gov) ; Zhang, Ji-Guang(jiguang.zhang@pnnl.gov)
英文摘要We report a carbonate-based localized high-concentration electrolyte (LHCE) with a fluorinated ether as a diluent for 4-V class lithium metal batteries (LMBs), which enables dendrite-free Li deposition with a high Li Coulombic efficiency (similar to 98.5%) and much better cycling stability for Li metal anodes than previously reported dimethyl carbonate-based LHCEs at lean electrolyte conditions. This electrolyte consists of 1.2 M lithium bis(fluorosulfonyl)imide (LiFSI) in a cosolvent mixture of ethylene carbonate (EC)/ethyl methyl carbonate (EMC) with bis(2,2,2-trifluoroethyl) ether (BTFE) as the diluent and 0.15 M lithium difluoro(oxalate)borate (LiDFOB) as an additive. A Li parallel to LiNi1/3Mn1/3 Co1/3O2 battery with a high areal loading of 3.8 mAh cm(-2) maintains 84% of its initial capacity after 100 cycles. The enhanced stability can be attributed to the robust solid-electrolyte interface (SEI) layer formed on the Li metal decomposition of LiDFOB salt and EC solvent molecules.
WOS关键词ION BATTERIES ; ANODE ; DIFLUORO(OXALATO)BORATE ; CAPACITY ; SALT
资助项目Assistant Secretary for Energy Efficiency and Renewable Energy, Office of Vehicle Technologies of the U.S. Department of Energy (DOE) through the Advanced Battery Materials Research (BMR) program (Battery500 Consortium)[DE-AC02-05CH11231] ; DOE's Office of Biological and Environmental Research ; DOE[DE-AC05-76RL01830] ; DOE Vehicle Technologies Program within Applied Battery Research (ABR) for Transportation Program
WOS研究方向Chemistry ; Electrochemistry ; Energy & Fuels ; Science & Technology - Other Topics ; Materials Science
语种英语
WOS记录号WOS:000445052900006
出版者AMER CHEMICAL SOC
资助机构Assistant Secretary for Energy Efficiency and Renewable Energy, Office of Vehicle Technologies of the U.S. Department of Energy (DOE) through the Advanced Battery Materials Research (BMR) program (Battery500 Consortium) ; Assistant Secretary for Energy Efficiency and Renewable Energy, Office of Vehicle Technologies of the U.S. Department of Energy (DOE) through the Advanced Battery Materials Research (BMR) program (Battery500 Consortium) ; Assistant Secretary for Energy Efficiency and Renewable Energy, Office of Vehicle Technologies of the U.S. Department of Energy (DOE) through the Advanced Battery Materials Research (BMR) program (Battery500 Consortium) ; Assistant Secretary for Energy Efficiency and Renewable Energy, Office of Vehicle Technologies of the U.S. Department of Energy (DOE) through the Advanced Battery Materials Research (BMR) program (Battery500 Consortium) ; Assistant Secretary for Energy Efficiency and Renewable Energy, Office of Vehicle Technologies of the U.S. Department of Energy (DOE) through the Advanced Battery Materials Research (BMR) program (Battery500 Consortium) ; Assistant Secretary for Energy Efficiency and Renewable Energy, Office of Vehicle Technologies of the U.S. Department of Energy (DOE) through the Advanced Battery Materials Research (BMR) program (Battery500 Consortium) ; Assistant Secretary for Energy Efficiency and Renewable Energy, Office of Vehicle Technologies of the U.S. Department of Energy (DOE) through the Advanced Battery Materials Research (BMR) program (Battery500 Consortium) ; Assistant Secretary for Energy Efficiency and Renewable Energy, Office of Vehicle Technologies of the U.S. Department of Energy (DOE) through the Advanced Battery Materials Research (BMR) program (Battery500 Consortium) ; Assistant Secretary for Energy Efficiency and Renewable Energy, Office of Vehicle Technologies of the U.S. Department of Energy (DOE) through the Advanced Battery Materials Research (BMR) program (Battery500 Consortium) ; Assistant Secretary for Energy Efficiency and Renewable Energy, Office of Vehicle Technologies of the U.S. Department of Energy (DOE) through the Advanced Battery Materials Research (BMR) program (Battery500 Consortium) ; 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源URL[http://ir.hfcas.ac.cn:8080/handle/334002/38852]  
专题合肥物质科学研究院_中科院固体物理研究所
通讯作者Xu, Wu; Zhang, Ji-Guang
作者单位1.Pacific Northwest Natl Lab, Energy & Environm Directorate, 902 Battelle Blvd, Richland, WA 99354 USA
2.Chinese Acad Sci, Inst Solid State Phys, Key Lab Mat Phys, Hefei 230026, Anhui, Peoples R China
3.Pacific Northwest Natl Lab, Environm Mol Sci Lab, 3335 Innovat Blvd, Richland, WA 99354 USA
推荐引用方式
GB/T 7714		 Yu, Lu,Chen, Shuru,Lee, Hongkyung,et al. A Localized High-Concentration Electrolyte with Optimized Solvents and Lithium Difluoro(oxalate)borate Additive for Stable Lithium Metal Batteries[J]. ACS ENERGY LETTERS,2018,3(9):2059-2067.
APA Yu, Lu.,Chen, Shuru.,Lee, Hongkyung.,Zhang, Linchao.,Engelhard, Mark H..,...&Zhang, Ji-Guang.(2018).A Localized High-Concentration Electrolyte with Optimized Solvents and Lithium Difluoro(oxalate)borate Additive for Stable Lithium Metal Batteries.ACS ENERGY LETTERS,3(9),2059-2067.
MLA Yu, Lu,et al."A Localized High-Concentration Electrolyte with Optimized Solvents and Lithium Difluoro(oxalate)borate Additive for Stable Lithium Metal Batteries".ACS ENERGY LETTERS 3.9(2018):2059-2067.

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来源：合肥物质科学研究院

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