Ordered Zinc Antimonate Nanoisland Attachment and Morphology Control of ZnO Nanobelts by Sb Doping
文献类型:期刊论文
作者 | Cheng BC ; Tian BX ; Sun W ; Xiao YH ; Lei SJ ; Wang ZG |
刊名 | journal of physical chemistry c
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出版日期 | 2009 |
卷号 | 113期号:22页码:9638-9643 |
关键词 | DOPED ZNO QUANTUM DOTS PHOTOLUMINESCENCE GROWTH OXIDES NANOSTRUCTURES SEMICONDUCTORS RECOMBINATION NANOPARTICLES NANOCRYSTALS |
ISSN号 | 1932-7447 |
通讯作者 | cheng bc nanchang univ inst adv studying nanchang 330031 peoples r china. e-mail address: bcheng@vip.sina.com |
中文摘要 | hierarchical heterostructures of zinc antimonate nanoislands on zno nanobelts were prepared by simple annealing of the polymeric precursor. sb can promote the growth of zno nanobelts along the [552] direction because of the segregation of sb dopants on the +(001) and (110) surfaces of zno nanobelts. furthermore, the ordered nanoislands of toothlike znsb2o6 along the [001](zno) direction and rodlike zn7sb2o12 along the [110](zno) direction can be formed because of the match relation of the lattice and polar charges between zno and zinc antimonate. the incorporation of sb in a zno lattice induces composition fluctuation, and the growth of zinc antimonate nanoislands on nanobelt sides induces interface fluctuation, resulting in dominance of the bound exciton transition in the room temperature near-band-edge (nbe) emission at relatively low excitation intensity. at high excitation intensity, however, auger recombination makes photogenerated electrons release phonon and relax from the conduction band to the trap states, causing the nbe emission to gradually saturate and redshift with increasing excitation intensity. the green emission more reasonably originates from the recombination of electrons in shallow traps with doubly charged v-o** oxygen vacancies. because a v-o** center can trap a photoactivated electron and change to a singly charged oxygen vacancy v-o* state, its emission intensity exhibits a maximum with increasing excitation intensity. |
学科主题 | 半导体化学 |
收录类别 | SCI |
资助信息 | foundation of jiangxi educational committee gjj09024 natural science foundation of jiangxi province 2007gqc1720 program for innovative research team of nanchang university this work was supported by the foundation of jiangxi educational committee (gjj09024), the natural science foundation of jiangxi province (2007gqc1720), and funds from the program for innovative research team of nanchang university. |
语种 | 英语 |
公开日期 | 2010-03-08 |
源URL | [http://ir.semi.ac.cn/handle/172111/7161] ![]() |
专题 | 半导体研究所_中国科学院半导体研究所(2009年前) |
推荐引用方式 GB/T 7714 | Cheng BC,Tian BX,Sun W,et al. Ordered Zinc Antimonate Nanoisland Attachment and Morphology Control of ZnO Nanobelts by Sb Doping[J]. journal of physical chemistry c,2009,113(22):9638-9643. |
APA | Cheng BC,Tian BX,Sun W,Xiao YH,Lei SJ,&Wang ZG.(2009).Ordered Zinc Antimonate Nanoisland Attachment and Morphology Control of ZnO Nanobelts by Sb Doping.journal of physical chemistry c,113(22),9638-9643. |
MLA | Cheng BC,et al."Ordered Zinc Antimonate Nanoisland Attachment and Morphology Control of ZnO Nanobelts by Sb Doping".journal of physical chemistry c 113.22(2009):9638-9643. |
入库方式: OAI收割
来源:半导体研究所
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