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Manganese(I)-Catalyzed Synthesis of Fused Eight- and Four-Membered Carbocycles via C-H Activation and Pericyclic Reactions

文献类型：期刊论文

作者Xu, Youwei1,3; Zheng, Guangfan2; Kong, Lingheng2; Li, Xingwei1,2
刊名ORGANIC LETTERS
出版日期2019-05-03
卷号21期号:9页码:3402-3406
ISSN号1523-7060
DOI10.1021/acs.orglett.9b01139
通讯作者Li, Xingwei(xwli@dicp.ac.cn)
英文摘要Pericyclic reactions have allowed facile construction of complex cycles. On the other hand, metal-catalyzed C-H activation has been established as an important strategy for rapid synthesis of complex structures. The two areas are integrated in Mn(I)-catalyzed redox-neutral coupling of 3-alkenyl- and 3-allylindoles with propargylic carbonates, which occurred via C-H allenylation with subsequent pericyclic reactions to afford fused eight- and four-membered carbocycles, respectively.
WOS关键词2+2 CYCLOADDITIONS ; DIRECTING GROUPS ; N BOND ; ALLENES ; FUNCTIONALIZATIONS ; ALLYLATION ; ALKYNES ; ARENES ; COMBINATION ; CYCLIZATION
资助项目Dalian Institute of Chemical Physics (Chinese Academy of Sciences) ; NSFC[21525208] ; NSFC[21472186]
WOS研究方向Chemistry
语种英语
WOS记录号WOS:000467320000090
出版者AMER CHEMICAL SOC
资助机构Dalian Institute of Chemical Physics (Chinese Academy of Sciences) ; Dalian Institute of Chemical Physics (Chinese Academy of Sciences) ; NSFC ; NSFC ; Dalian Institute of Chemical Physics (Chinese Academy of Sciences) ; Dalian Institute of Chemical Physics (Chinese Academy of Sciences) ; NSFC ; NSFC ; Dalian Institute of Chemical Physics (Chinese Academy of Sciences) ; Dalian Institute of Chemical Physics (Chinese Academy of Sciences) ; NSFC ; NSFC ; Dalian Institute of Chemical Physics (Chinese Academy of Sciences) ; Dalian Institute of Chemical Physics (Chinese Academy of Sciences) ; NSFC ; NSFC
源URL[http://cas-ir.dicp.ac.cn/handle/321008/172043]  
专题大连化学物理研究所_中国科学院大连化学物理研究所
通讯作者Li, Xingwei
作者单位1.Chinese Acad Sci, Dalian Inst Chem Phys, Dalian 116023, Peoples R China
2.Shaanxi Normal Univ SNNU, Sch Chem & Chem Engn, Xian 710062, Shaanxi, Peoples R China
3.Univ Chinese Acad Sci, Beijing 100049, Peoples R China
推荐引用方式
GB/T 7714		 Xu, Youwei,Zheng, Guangfan,Kong, Lingheng,et al. Manganese(I)-Catalyzed Synthesis of Fused Eight- and Four-Membered Carbocycles via C-H Activation and Pericyclic Reactions[J]. ORGANIC LETTERS,2019,21(9):3402-3406.
APA Xu, Youwei,Zheng, Guangfan,Kong, Lingheng,&Li, Xingwei.(2019).Manganese(I)-Catalyzed Synthesis of Fused Eight- and Four-Membered Carbocycles via C-H Activation and Pericyclic Reactions.ORGANIC LETTERS,21(9),3402-3406.
MLA Xu, Youwei,et al."Manganese(I)-Catalyzed Synthesis of Fused Eight- and Four-Membered Carbocycles via C-H Activation and Pericyclic Reactions".ORGANIC LETTERS 21.9(2019):3402-3406.

入库方式： OAI收割

来源：大连化学物理研究所

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