Recent Progress in Catalytic Oxidative Transformations of Alcohols by Supported Gold Nanoparticles
文献类型：期刊论文
| 作者 | Hui, Yonghai2; Zhang, Shiqi2; Wang, Wentao1 |
| 刊名 | ADVANCED SYNTHESIS & CATALYSIS
 |
| 出版日期 | 2019-05-14 |
| 卷号 | 361期号:10页码:2215-2235 |
| 关键词 | alcohols aldehydes gold nanoparticles heterogeneous catalysis ketones oxidation |
| ISSN号 | 1615-4150 |
| DOI | 10.1002/adsc.201801595 |
| 通讯作者 | Wang, Wentao(wentaowang@dicp.ac.cn) |
| 英文摘要 | Catalytic oxidative transformations of alcohols constitute one of the greatly important protocols for the synthesis of various aldehydes, ketones, acids, imines, amides, etc. that are required to make drug intermediates, food additives, plastics, detergents and cosmetics. The potential of gold nanoparticles (Au NPs) in catalytic oxidation reactions is generally competent owing to their tendency to activate oxygen. Supports play a conspicuous and increasingly important role not only in the preparation and stabilization of Au NPs, but also can address the issues of sustainability by facilitating separation and reusability of the catalyst. This review aims to systematically discuss the impressive developments in catalytic oxidative transformations of alcohols promoted by supported Au NPs in the last five years. These Au NPs exhibit unique electronic properties and crystal structures, which gives us an excellent opportunity to correlate atomic structure with intrinsic catalytic properties over Au NPs. The effect of a support on the significant properties of Au NPs in terms of catalytic activity, selectivity, recyclability, and stability is discussed at length. The tentative reaction mechanisms and the structure-performance relationships are also discussed at appropriate places, which will provide some clues for the design of efficient Au NPs-based catalysts. |
| WOS关键词 | SOLVENT-FREE OXIDATION ; SELECTIVE AEROBIC OXIDATION ; METAL-ORGANIC FRAMEWORKS ; HIGHLY EFFICIENT ; BENZYL ALCOHOL ; MOLECULAR-OXYGEN ; AU NANOPARTICLES ; STEP SYNTHESIS ; ETHANOL ; HYDROTALCITE |
| 资助项目 | National Natural Science Foundation of China[21672210] ; Doctoral Fund of Lingnan Normal University[ZL1817] |
| WOS研究方向 | Chemistry |
| 语种 | 英语 |
| WOS记录号 | WOS:000471326000002 |
| 出版者 | WILEY-V C H VERLAG GMBH |
| 资助机构 | National Natural Science Foundation of China ; National Natural Science Foundation of China ; Doctoral Fund of Lingnan Normal University ; Doctoral Fund of Lingnan Normal University ; National Natural Science Foundation of China ; National Natural Science Foundation of China ; Doctoral Fund of Lingnan Normal University ; Doctoral Fund of Lingnan Normal University ; National Natural Science Foundation of China ; National Natural Science Foundation of China ; Doctoral Fund of Lingnan Normal University ; Doctoral Fund of Lingnan Normal University ; National Natural Science Foundation of China ; National Natural Science Foundation of China ; Doctoral Fund of Lingnan Normal University ; Doctoral Fund of Lingnan Normal University |
| 源URL | [http://cas-ir.dicp.ac.cn/handle/321008/172067]  |
| 专题 | 大连化学物理研究所_中国科学院大连化学物理研究所 |
| 通讯作者 | Wang, Wentao |
| 作者单位 | 1.Chinese Acad Sci, Dalian Inst Chem Phys, Dalian 116023, Peoples R China 2.Lingnan Normal Univ, Coll Chem & Chem Engn, Zhanjiang 524048, Peoples R China |
| 推荐引用方式 GB/T 7714 | Hui, Yonghai,Zhang, Shiqi,Wang, Wentao. Recent Progress in Catalytic Oxidative Transformations of Alcohols by Supported Gold Nanoparticles[J]. ADVANCED SYNTHESIS & CATALYSIS,2019,361(10):2215-2235. |
| APA | Hui, Yonghai,Zhang, Shiqi,&Wang, Wentao.(2019).Recent Progress in Catalytic Oxidative Transformations of Alcohols by Supported Gold Nanoparticles.ADVANCED SYNTHESIS & CATALYSIS,361(10),2215-2235. |
| MLA | Hui, Yonghai,et al."Recent Progress in Catalytic Oxidative Transformations of Alcohols by Supported Gold Nanoparticles".ADVANCED SYNTHESIS & CATALYSIS 361.10(2019):2215-2235. |
入库方式： OAI收割
来源：大连化学物理研究所
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