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A broadband sum-frequency generation vibrational spectrometer to probe adsorbed molecules on nanoparticles

文献类型：期刊论文

作者Luo, Ting2,6; Zhang, Ruidan2,3,4; Peng, Xingxing2,3,4; Liu, Xinting2,5; Zhou, Chuanyao2; Yang, Xueming1,2; Ren, Zefeng2
刊名SURFACE SCIENCE
出版日期2019-11-01
卷号689页码:7
关键词Sum frequency generation Vibrational spectroscopy Nanoparticle Heterogeneous catalysis High pressure High temperature
ISSN号0039-6028
DOI10.1016/j.susc.2019.121459
通讯作者Ren, Zefeng(zfren@dicp.ac.cn)
英文摘要Characterizing high-surface-area powders under near-ambient and high-pressure environments has obtained more and more attraction in the field of heterogeneous catalysis in the last decades. Here, we present an easyoperated internal heterodyne phase-resolved sum-frequency generation vibrational spectroscopy (SFG-VS) setup with the z-cut alpha-quartz as the internal phase reference. It is equipped with CO2 laser to heat the substrate of alpha-quartz in a non-contacted way, which enables us to realize high sensitive SFG vibrational spectral measurements under high pressure and high temperature conditions. It has been demonstrated with CO adsorbed on platinum nanoparticles under the high CO pressure and the high temperature environment and sodium dodecyl sulfate film on alpha-quartz.
WOS关键词REFLECTION-ABSORPTION SPECTROSCOPY ; IN-SITU ; CARBON-MONOXIDE ; HIGH-PRESSURES ; ETHYLENE HYDROGENATION ; CO ADSORPTION ; SURFACE ; PT(111) ; INTERFACES ; PROTEINS
资助项目Ministry of Science and Technology[2018YFA0208700] ; Ministry of Science and Technology[2016YFA0200602] ; Chinese Academy of Sciences[XDB17000000] ; Chinese Academy of Sciences[ZDKYYQ20170003] ; National Natural Science Foundation of China[91645125] ; National Natural Science Foundation of China[21688102] ; Youth Innovation Promotion Association of CAS[2017224]
WOS研究方向Chemistry ; Physics
语种英语
WOS记录号WOS:000490046500008
出版者ELSEVIER
资助机构Ministry of Science and Technology ; Ministry of Science and Technology ; Chinese Academy of Sciences ; Chinese Academy of Sciences ; National Natural Science Foundation of China ; National Natural Science Foundation of China ; Youth Innovation Promotion Association of CAS ; Youth Innovation Promotion Association of CAS ; Ministry of Science and Technology ; Ministry of Science and Technology ; Chinese Academy of Sciences ; Chinese Academy of Sciences ; National Natural Science Foundation of China ; National Natural Science Foundation of China ; Youth Innovation Promotion Association of CAS ; Youth Innovation Promotion Association of CAS ; Ministry of Science and Technology ; Ministry of Science and Technology ; Chinese Academy of Sciences ; Chinese Academy of Sciences ; National Natural Science Foundation of China ; National Natural Science Foundation of China ; Youth Innovation Promotion Association of CAS ; Youth Innovation Promotion Association of CAS ; Ministry of Science and Technology ; Ministry of Science and Technology ; Chinese Academy of Sciences ; Chinese Academy of Sciences ; National Natural Science Foundation of China ; National Natural Science Foundation of China ; Youth Innovation Promotion Association of CAS ; Youth Innovation Promotion Association of CAS
源URL[http://cas-ir.dicp.ac.cn/handle/321008/172328]  
专题大连化学物理研究所_中国科学院大连化学物理研究所
通讯作者Ren, Zefeng
作者单位1.Southern Univ Sci & Technol, Dept Chem, 1088 Xueyuan Rd, Shenzhen 518055, Guangdong, Peoples R China
2.Chinese Acad Sci, Dalian Inst Chem Phys, Res Ctr Energy & Environm Mat, State Key Lab Mol React Dynam & Dynam, 457 Zhongshan Rd, Dalian 116023, Peoples R China
3.Peking Univ, ICQM, 5 Yiheyuan Rd, Beijing 100871, Peoples R China
4.Peking Univ, Sch Phys, 5 Yiheyuan Rd, Beijing 100871, Peoples R China
5.Dalian Univ Technol, 2 Linggong Rd, Dalian 116024, Peoples R China
6.Univ Chinese Acad Sci, 19A Yuquan Rd, Beijing 100049, Peoples R China
推荐引用方式
GB/T 7714		 Luo, Ting,Zhang, Ruidan,Peng, Xingxing,et al. A broadband sum-frequency generation vibrational spectrometer to probe adsorbed molecules on nanoparticles[J]. SURFACE SCIENCE,2019,689:7.
APA Luo, Ting.,Zhang, Ruidan.,Peng, Xingxing.,Liu, Xinting.,Zhou, Chuanyao.,...&Ren, Zefeng.(2019).A broadband sum-frequency generation vibrational spectrometer to probe adsorbed molecules on nanoparticles.SURFACE SCIENCE,689,7.
MLA Luo, Ting,et al."A broadband sum-frequency generation vibrational spectrometer to probe adsorbed molecules on nanoparticles".SURFACE SCIENCE 689(2019):7.

入库方式： OAI收割

来源：大连化学物理研究所

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