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Simple Is Best: A p-Phenylene Bridging Methoxydiphenylamine-Substituted Carbazole Hole Transporter for High-Performance Perovskite Solar Cells

文献类型：期刊论文

作者Yu, Wei1,2; Yang, Qing1,3; Zhang, Jinhui1,4; Tu, Dandan1,3; Wang, Xuchao1; Liu, Xuan1,3; Li, Gang2; Guo, Xin1; Li, Can1
刊名ACS APPLIED MATERIALS & INTERFACES
出版日期2019-08-21
卷号11期号:33页码:30065-30071
ISSN号1944-8244
关键词perovskite solar cells hole-transporting materials power conversion efficiency carbazole pi-bridge
DOI10.1021/acsami.9b06933
通讯作者Guo, Xin(guoxin@dicp.ac.cn) ; Li, Can(canli@dicp.ac.cn)
英文摘要Methoxydiphenylamine-substituted carbazole (MODPACz) is widely used to construct hole-transporting materials (HTMs) for perovskite solar cells (PSCs), whose performances rely highly on the linking way of the MODPACz units and the simplicity of the pi-bridge. In this paper, we report a new HTM, pPh-2MODPACz, using one of the simplest pi-bridges p-phenylene to link the MODPACz units. The structural feature endows pPh-2MODPACz with high hole mobility and conductivity, efficient hole extraction ability, and good film-forming property. MAPbI(3)-based PSCs using doped and undoped pPh-2MODPACz as the HTM offer efficiencies of similar to 20% and 16.07%, respectively; both are better than those of the devices with spiro-OMeTAD as the HTM. The device stability of pPh-2MODPACz-based PSCs is also greatly enhanced. This work demonstrates that the simplest p-phenylene bridge for linking MODPACz can derive a promising HTM with a high device performance, providing a distinctive pathway to develop new HTMs.
WOS关键词LOW-COST ; EFFICIENT ; DOPANT ; DERIVATIVES
资助项目National Natural Science Foundation of China[61604152] ; National Natural Science Foundation of China[91733301] ; DICPQIBEBT[UN201705] ; DICP[ZZBS201813] ; Liaoning Revitalization Talents Program[XLYC1807231] ; Natural Science Foundation of Liaoning Province of China[20180540124] ; Hong Kong Scholars Program[XJ2017046]
WOS研究方向Science & Technology - Other Topics ; Materials Science
语种英语
出版者AMER CHEMICAL SOC
WOS记录号WOS:000482546000061
资助机构National Natural Science Foundation of China ; National Natural Science Foundation of China ; DICPQIBEBT ; DICPQIBEBT ; DICP ; DICP ; Liaoning Revitalization Talents Program ; Liaoning Revitalization Talents Program ; Natural Science Foundation of Liaoning Province of China ; Natural Science Foundation of Liaoning Province of China ; Hong Kong Scholars Program ; Hong Kong Scholars Program ; National Natural Science Foundation of China ; National Natural Science Foundation of China ; DICPQIBEBT ; DICPQIBEBT ; DICP ; DICP ; Liaoning Revitalization Talents Program ; Liaoning Revitalization Talents Program ; Natural Science Foundation of Liaoning Province of China ; Natural Science Foundation of Liaoning Province of China ; Hong Kong Scholars Program ; Hong Kong Scholars Program ; National Natural Science Foundation of China ; National Natural Science Foundation of China ; DICPQIBEBT ; DICPQIBEBT ; DICP ; DICP ; Liaoning Revitalization Talents Program ; Liaoning Revitalization Talents Program ; Natural Science Foundation of Liaoning Province of China ; Natural Science Foundation of Liaoning Province of China ; Hong Kong Scholars Program ; Hong Kong Scholars Program ; National Natural Science Foundation of China ; National Natural Science Foundation of China ; DICPQIBEBT ; DICPQIBEBT ; DICP ; DICP ; Liaoning Revitalization Talents Program ; Liaoning Revitalization Talents Program ; Natural Science Foundation of Liaoning Province of China ; Natural Science Foundation of Liaoning Province of China ; Hong Kong Scholars Program ; Hong Kong Scholars Program
源URL[http://cas-ir.dicp.ac.cn/handle/321008/173204]  
专题大连化学物理研究所_中国科学院大连化学物理研究所
通讯作者Guo, Xin; Li, Can
作者单位1.Chinese Acad Sci, Dalian Inst Chem Phys, State Key Lab Catalysis, Dalian Natl Lab Clean Energy, Dalian 116023, Peoples R China
2.Hong Kong Polytech Univ, Dept Elect & Informat Engn, Kowloon, Hung Hom, Hong Kong, Peoples R China
3.Univ Chinese Acad Sci, Beijing 100049, Peoples R China
4.Dalian Maritime Univ, Dept Mat Sci & Engn, Dalian 116023, Peoples R China
推荐引用方式
GB/T 7714		 Yu, Wei,Yang, Qing,Zhang, Jinhui,et al. Simple Is Best: A p-Phenylene Bridging Methoxydiphenylamine-Substituted Carbazole Hole Transporter for High-Performance Perovskite Solar Cells[J]. ACS APPLIED MATERIALS & INTERFACES,2019,11(33):30065-30071.
APA Yu, Wei.,Yang, Qing.,Zhang, Jinhui.,Tu, Dandan.,Wang, Xuchao.,...&Li, Can.(2019).Simple Is Best: A p-Phenylene Bridging Methoxydiphenylamine-Substituted Carbazole Hole Transporter for High-Performance Perovskite Solar Cells.ACS APPLIED MATERIALS & INTERFACES,11(33),30065-30071.
MLA Yu, Wei,et al."Simple Is Best: A p-Phenylene Bridging Methoxydiphenylamine-Substituted Carbazole Hole Transporter for High-Performance Perovskite Solar Cells".ACS APPLIED MATERIALS & INTERFACES 11.33(2019):30065-30071.

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来源：大连化学物理研究所

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