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Soybean milk derived carbon intercalated with reduced graphene oxide as high efficient electrocatalysts for oxygen reduction reaction

文献类型：期刊论文

作者Sun, Yue1,2; Zhong, Ruyi2; Zhang, Haizhou3; Huang, Taizhong1; Yu, Jiemei1; Fang, Hengyi1; Liang, Dong1; Guo, Zhongqin1
刊名INTERNATIONAL JOURNAL OF HYDROGEN ENERGY
出版日期2019-08-13
卷号44期号:39页码:21790-21802
ISSN号0360-3199
关键词Soybean milk derived carbon Electrocatalysts Oxygen reduction reaction Nitridation Reduced graphene oxide Nitrogen-doped carbons
DOI10.1016/j.ijhydene.2019.06.174
通讯作者Zhang, Haizhou(zhz_doctor@163.com) ; Huang, Taizhong(chm_huangtz@ujn.edu.cn)
英文摘要Exploring high-performance and low-cost metal-free oxygen reduction reaction (ORR) catalysts from biomass-derived materials is vital to the development of novel energy conversion devices such as fuel cells, etc. Herein, nitrogen-enriched soybean milk derived carbon (BDC/rGO-HT-NH3) intercalated with reduced graphene oxide (rGO) electrocatalyst is prepared via one-pot hydrothermal synthesis method followed with nitridation by NH3. The resultant catalyst with high surface area, good conductivity and high content of N (9.4 at.%) shows high electrocatalytic activity towards ORR in alkaline medium, which mainly happens through the direct 4-electron pathway. The onset potential of BDC/rGO-HT-NH3 catalyzed ORR is 0.96 V vs RHE, which is only 0.11 V lower than that of the commercial Pt/C (20 wt%) catalyst. In addition, the BDC/rGO-HT-NH3 catalyst shows superior long-term running durability. The desirable catalytic performances enable the facile synthesis approach of BDC/rGO-HT-NH3 to be a promising methodology for transforming other biomass materials to N-enriched carbon based materials as low-cost and environmental friendly catalysts for ORR. (C)2019 Hydrogen Energy Publications LLC. Published by Elsevier Ltd. All rights reserved.
WOS关键词METAL-FREE ELECTROCATALYST ; DOPED POROUS CARBON ; MESOPOROUS CARBON ; TEMPLATE-FREE ; NITROGEN ; CATALYST ; BIOMASS ; ENERGY ; NANOSHEETS ; ELECTRODE
资助项目Shandong Natural Science Foundation[ZR2018MB036] ; Shandong Natural Science Foundation[ZR2017QB009] ; Science Development Project of Shandong Province[2017GGX40115] ; Science Development Project of Shandong Province[2016GGX102038] ; Project of Shandong Province Higher Educational Science and Technology Program[J13LD08] ; Project of Shandong Province Higher Educational Science and Technology Program[J17KA094] ; Scientific Research Fund of University of Jinan[XBS1644] ; National Key R&D Program of China[2017YFC1308000]
WOS研究方向Chemistry ; Electrochemistry ; Energy & Fuels
语种英语
出版者PERGAMON-ELSEVIER SCIENCE LTD
WOS记录号WOS:000483634100051
资助机构Shandong Natural Science Foundation ; Shandong Natural Science Foundation ; Science Development Project of Shandong Province ; Science Development Project of Shandong Province ; Project of Shandong Province Higher Educational Science and Technology Program ; Project of Shandong Province Higher Educational Science and Technology Program ; Scientific Research Fund of University of Jinan ; Scientific Research Fund of University of Jinan ; National Key R&D Program of China ; National Key R&D Program of China ; Shandong Natural Science Foundation ; Shandong Natural Science Foundation ; Science Development Project of Shandong Province ; Science Development Project of Shandong Province ; Project of Shandong Province Higher Educational Science and Technology Program ; Project of Shandong Province Higher Educational Science and Technology Program ; Scientific Research Fund of University of Jinan ; Scientific Research Fund of University of Jinan ; National Key R&D Program of China ; National Key R&D Program of China ; Shandong Natural Science Foundation ; Shandong Natural Science Foundation ; Science Development Project of Shandong Province ; Science Development Project of Shandong Province ; Project of Shandong Province Higher Educational Science and Technology Program ; Project of Shandong Province Higher Educational Science and Technology Program ; Scientific Research Fund of University of Jinan ; Scientific Research Fund of University of Jinan ; National Key R&D Program of China ; National Key R&D Program of China ; Shandong Natural Science Foundation ; Shandong Natural Science Foundation ; Science Development Project of Shandong Province ; Science Development Project of Shandong Province ; Project of Shandong Province Higher Educational Science and Technology Program ; Project of Shandong Province Higher Educational Science and Technology Program ; Scientific Research Fund of University of Jinan ; Scientific Research Fund of University of Jinan ; National Key R&D Program of China ; National Key R&D Program of China
源URL[http://cas-ir.dicp.ac.cn/handle/321008/173368]  
专题大连化学物理研究所_中国科学院大连化学物理研究所
通讯作者Zhang, Haizhou; Huang, Taizhong
作者单位1.Univ Jinan, Sch Chem & Chem Engn, Jinan 250022, Shandong, Peoples R China
2.Chinese Acad Sci, Dalian Inst Chem Phys, 457 Zhongshan Rd, Dalian 116023, Peoples R China
3.Shandong Univ, Dept Cardiac Surg, Shandong Prov Hosp, 324 Jingwu Rd, Jinan 250021, Shandong, Peoples R China
推荐引用方式
GB/T 7714		 Sun, Yue,Zhong, Ruyi,Zhang, Haizhou,et al. Soybean milk derived carbon intercalated with reduced graphene oxide as high efficient electrocatalysts for oxygen reduction reaction[J]. INTERNATIONAL JOURNAL OF HYDROGEN ENERGY,2019,44(39):21790-21802.
APA Sun, Yue.,Zhong, Ruyi.,Zhang, Haizhou.,Huang, Taizhong.,Yu, Jiemei.,...&Guo, Zhongqin.(2019).Soybean milk derived carbon intercalated with reduced graphene oxide as high efficient electrocatalysts for oxygen reduction reaction.INTERNATIONAL JOURNAL OF HYDROGEN ENERGY,44(39),21790-21802.
MLA Sun, Yue,et al."Soybean milk derived carbon intercalated with reduced graphene oxide as high efficient electrocatalysts for oxygen reduction reaction".INTERNATIONAL JOURNAL OF HYDROGEN ENERGY 44.39(2019):21790-21802.

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来源：大连化学物理研究所

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