Fundamentals of TiO2 Photocatalysis: Concepts, Mechanisms, and Challenges
文献类型：期刊论文
| 作者 | Guo, Qing1,2; Zhou, Chuanyao1; Ma, Zhibo1; Yang, Xueming1,2 |
| 刊名 | ADVANCED MATERIALS
 |
| 出版日期 | 2019-08-18 |
| 页码 | 26 |
| 关键词 | charge carriers nonadiabatic processes reaction mechanisms TiO2 photocatalysis |
| ISSN号 | 0935-9648 |
| DOI | 10.1002/adma.201901997 |
| 通讯作者 | Yang, Xueming(xmyang@dicp.ac.cn) |
| 英文摘要 | Photocatalysis has been widely applied in various areas, such as solar cells, water splitting, and pollutant degradation. Therefore, the photochemical mechanisms and basic principles of photocatalysis, especially TiO2 photocatalysis, have been extensively investigated by various surface science methods in the last decade, aiming to provide important information for TiO2 photocatalysis under real environmental conditions. Recent progress that provides fundamental insights into TiO2 photocatalysis at a molecular level is highlighted. Insights into the structures of TiO2 and the basic principles of TiO2 photocatalysis are discussed first, which provides the basic concepts of TiO2 photocatalysis. Following this, details of the photochemistry of three important molecules (oxygen, water, methanol) on the model TiO2 surfaces are presented, in an attempt to unravel the relationship between charge/energy transfer and bond breaking/forming in TiO2 photocatalysis. Lastly, challenges and opportunities of the mechanistic studies of TiO2 photocatalysis at the molecular level are discussed briefly, as well as possible photocatalysis models. |
| WOS关键词 | PHOTOINDUCED ELECTRON-TRANSFER ; INTERFACIAL HOLE TRANSFER ; REAL-TIME OBSERVATION ; UV-INDUCED DESORPTION ; TITANIUM-DIOXIDE ; RUTILE TIO2(110) ; MOLECULAR-OXYGEN ; CHARGE-TRANSFER ; ANATASE TIO2 ; REDUCED RUTILE |
| 资助项目 | National Natural Science Foundation of China[21673235] ; Strategic Priority Research Program of Chinese Academy of Sciences[XDB17000000] ; Youth Innovation Promotion Association CAS |
| WOS研究方向 | Chemistry ; Science & Technology - Other Topics ; Materials Science ; Physics |
| 语种 | 英语 |
| WOS记录号 | WOS:000481820900001 |
| 出版者 | WILEY-V C H VERLAG GMBH |
| 资助机构 | National Natural Science Foundation of China ; National Natural Science Foundation of China ; Strategic Priority Research Program of Chinese Academy of Sciences ; Strategic Priority Research Program of Chinese Academy of Sciences ; Youth Innovation Promotion Association CAS ; Youth Innovation Promotion Association CAS ; National Natural Science Foundation of China ; National Natural Science Foundation of China ; Strategic Priority Research Program of Chinese Academy of Sciences ; Strategic Priority Research Program of Chinese Academy of Sciences ; Youth Innovation Promotion Association CAS ; Youth Innovation Promotion Association CAS ; National Natural Science Foundation of China ; National Natural Science Foundation of China ; Strategic Priority Research Program of Chinese Academy of Sciences ; Strategic Priority Research Program of Chinese Academy of Sciences ; Youth Innovation Promotion Association CAS ; Youth Innovation Promotion Association CAS ; National Natural Science Foundation of China ; National Natural Science Foundation of China ; Strategic Priority Research Program of Chinese Academy of Sciences ; Strategic Priority Research Program of Chinese Academy of Sciences ; Youth Innovation Promotion Association CAS ; Youth Innovation Promotion Association CAS |
| 源URL | [http://cas-ir.dicp.ac.cn/handle/321008/173462]  |
| 专题 | 大连化学物理研究所_中国科学院大连化学物理研究所 |
| 通讯作者 | Yang, Xueming |
| 作者单位 | 1.Chinese Acad Sci, Dalian Inst Chem Phys, State Key Lab Mol React Dynam, 457 Zhongshan Rd, Dalian 116023, Liaoning, Peoples R China 2.Southern Univ Sci & Technol, Dept Chem, 1088 Xueyuan Ave, Shenzhen 518055, Peoples R China |
| 推荐引用方式 GB/T 7714 | Guo, Qing,Zhou, Chuanyao,Ma, Zhibo,et al. Fundamentals of TiO2 Photocatalysis: Concepts, Mechanisms, and Challenges[J]. ADVANCED MATERIALS,2019:26. |
| APA | Guo, Qing,Zhou, Chuanyao,Ma, Zhibo,&Yang, Xueming.(2019).Fundamentals of TiO2 Photocatalysis: Concepts, Mechanisms, and Challenges.ADVANCED MATERIALS,26. |
| MLA | Guo, Qing,et al."Fundamentals of TiO2 Photocatalysis: Concepts, Mechanisms, and Challenges".ADVANCED MATERIALS (2019):26. |
入库方式： OAI收割
来源：大连化学物理研究所
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