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Molybdenum-Catalyzed Oxidative Cleavage of Raw Poplar Sawdust into Mono-Aromatics and Organic Acid Esters

文献类型：期刊论文

作者Ma, Yangyang1,2; Ma, Jiping1; Xia, Fei1; Lu, Fang1; Du, Zhongtian1; Xu, Jie1
刊名ASIAN JOURNAL OF ORGANIC CHEMISTRY
出版日期2019-07-10
页码7
关键词oxidation oxygen molybdenum mono-aromatics acid esters
ISSN号2193-5807
DOI10.1002/ajoc.201900310
通讯作者Ma, Jiping(majiping@dicp.ac.cn) ; Xu, Jie(xujie@dicp.ac.cn)
英文摘要Conversion of non-edible lignocellulosic biomass into value-added chemicals is of great significance and also particularly attractive. However, owing to the complexity and inertness, valorization of native lignocellulose remains to be quite challenging. Herein, catalytic oxidative cleavage of raw poplar sawdust was studied, mono-aromatics and organic acid esters with 34.8 wt% and 27.4 wt% yield respectively were achieved over MoO2(acac)(2) with molecular oxygen, which was suggested to be attributed to a prior cleavage of the carbohydrate fractions. This catalytic oxidation approach demonstrates the feasibility of transformation of raw woody biomass into valuable chemicals.
WOS关键词LIGNOCELLULOSIC BIOMASS ; WOODY BIOMASS ; FORMIC-ACID ; LIGNIN ; CONVERSION ; CHEMICALS ; DEPOLYMERIZATION ; CELLULOSE ; NICKEL ; HYDROGENOLYSIS
资助项目National Natural Science Foundation of China[21790331] ; National Natural Science Foundation of China[21473184] ; National Natural Science Foundation of China[30900326] ; Strategic Priority Research Program of Chinese Academy of Sciences[XDB17020300] ; Strategic Priority Research Program of Chinese Academy of Sciences[XDA21030400] ; Youth Innovation Promotion Association, CAS[2018219] ; DICP[ZZBS201811]
WOS研究方向Chemistry
语种英语
WOS记录号WOS:000477467000001
出版者WILEY-V C H VERLAG GMBH
资助机构National Natural Science Foundation of China ; National Natural Science Foundation of China ; Strategic Priority Research Program of Chinese Academy of Sciences ; Strategic Priority Research Program of Chinese Academy of Sciences ; Youth Innovation Promotion Association, CAS ; Youth Innovation Promotion Association, CAS ; DICP ; DICP ; National Natural Science Foundation of China ; National Natural Science Foundation of China ; Strategic Priority Research Program of Chinese Academy of Sciences ; Strategic Priority Research Program of Chinese Academy of Sciences ; Youth Innovation Promotion Association, CAS ; Youth Innovation Promotion Association, CAS ; DICP ; DICP ; National Natural Science Foundation of China ; National Natural Science Foundation of China ; Strategic Priority Research Program of Chinese Academy of Sciences ; Strategic Priority Research Program of Chinese Academy of Sciences ; Youth Innovation Promotion Association, CAS ; Youth Innovation Promotion Association, CAS ; DICP ; DICP ; National Natural Science Foundation of China ; National Natural Science Foundation of China ; Strategic Priority Research Program of Chinese Academy of Sciences ; Strategic Priority Research Program of Chinese Academy of Sciences ; Youth Innovation Promotion Association, CAS ; Youth Innovation Promotion Association, CAS ; DICP ; DICP
源URL[http://cas-ir.dicp.ac.cn/handle/321008/173878]  
专题大连化学物理研究所_中国科学院大连化学物理研究所
通讯作者Ma, Jiping; Xu, Jie
作者单位1.Chinese Acad Sci, Dalian Inst Chem Phys, Dalian Natl Lab Clean Energy, State Key Lab Catalysis, Dalian 116023, Peoples R China
2.Henan Agr Univ, Coll Food Sci & Technol, Zhengzhou 450002, Henan, Peoples R China
推荐引用方式
GB/T 7714		 Ma, Yangyang,Ma, Jiping,Xia, Fei,et al. Molybdenum-Catalyzed Oxidative Cleavage of Raw Poplar Sawdust into Mono-Aromatics and Organic Acid Esters[J]. ASIAN JOURNAL OF ORGANIC CHEMISTRY,2019:7.
APA Ma, Yangyang,Ma, Jiping,Xia, Fei,Lu, Fang,Du, Zhongtian,&Xu, Jie.(2019).Molybdenum-Catalyzed Oxidative Cleavage of Raw Poplar Sawdust into Mono-Aromatics and Organic Acid Esters.ASIAN JOURNAL OF ORGANIC CHEMISTRY,7.
MLA Ma, Yangyang,et al."Molybdenum-Catalyzed Oxidative Cleavage of Raw Poplar Sawdust into Mono-Aromatics and Organic Acid Esters".ASIAN JOURNAL OF ORGANIC CHEMISTRY (2019):7.

入库方式： OAI收割

来源：大连化学物理研究所

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