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Decorated Traditional Zeolites with Subunits of Metal-Organic Frameworks for CH4/N-2 Separation

文献类型：期刊论文

作者Wu, Yaqi1,2; Yuan, Danhua2; He, Dawei1,2; Xing, Jiacheng1,2; Zeng, Shu1,2; Xu, Shutao2; Xu, Yunpeng2; Liu, Zhongmin2
刊名ANGEWANDTE CHEMIE-INTERNATIONAL EDITION
出版日期2019-07-22
卷号58期号:30页码:10241-10244
关键词gas adsorption metal-organic frameworks surface decoration zeolites
ISSN号1433-7851
DOI10.1002/anie.201905014
通讯作者Xu, Yunpeng(xuyp@dicp.ac.cn) ; Liu, Zhongmin(liuzm@dicp.ac.cn)
英文摘要Metal-organic frameworks (MOF) materials are promising materials for gas separation, but their application still faces various challenges. A strategy is now reported for introducing subunits of MOFs into traditional zeolite frameworks to obtain applicable adsorbents with advantages of both zeolites and MOFs. The subunits of ZIFs were introduced into zeolite Y and zeolite ZSM-5 for CH4/N-2 separation. Both the molecular simulation and experimental results validated that the IAST CH4/N-2 selectivity of the resulting samples greatly improved (above 8, at 100 kPa and 25 degrees C) with the incorporation of ZIF subunits into zeolites structure, and the selectivities were obviously higher than that of zeolites and even better than that of ZIFs. This strategy not only gave rise to an efficient adsorbent for CH4/N-2 separation but also provided ideas for design of other adsorption and separation materials.
WOS关键词IMIDAZOLATE FRAMEWORKS ; NMR ; ADSORPTION ; ZIF-8 ; CO2 ; TEMPERATURE ; MEMBRANES ; MOBILITY ; DESIGN ; XENON
资助项目National Key Research and Development Program of China[2016YFB0301603]
WOS研究方向Chemistry
语种英语
WOS记录号WOS:000476452700032
出版者WILEY-V C H VERLAG GMBH
资助机构National Key Research and Development Program of China ; National Key Research and Development Program of China ; National Key Research and Development Program of China ; National Key Research and Development Program of China ; National Key Research and Development Program of China ; National Key Research and Development Program of China ; National Key Research and Development Program of China ; National Key Research and Development Program of China
源URL[http://cas-ir.dicp.ac.cn/handle/321008/173968]  
专题大连化学物理研究所_中国科学院大连化学物理研究所
通讯作者Xu, Yunpeng; Liu, Zhongmin
作者单位1.Univ Chinese Acad Sci, Beijing 100049, Peoples R China
2.Chinese Acad Sci, Dalian Inst Chem Phys, Natl Engn Lab Methanol Olefins, Dalian Natl Lab Clean Energy, Dalian 116023, Peoples R China
推荐引用方式
GB/T 7714		 Wu, Yaqi,Yuan, Danhua,He, Dawei,et al. Decorated Traditional Zeolites with Subunits of Metal-Organic Frameworks for CH4/N-2 Separation[J]. ANGEWANDTE CHEMIE-INTERNATIONAL EDITION,2019,58(30):10241-10244.
APA Wu, Yaqi.,Yuan, Danhua.,He, Dawei.,Xing, Jiacheng.,Zeng, Shu.,...&Liu, Zhongmin.(2019).Decorated Traditional Zeolites with Subunits of Metal-Organic Frameworks for CH4/N-2 Separation.ANGEWANDTE CHEMIE-INTERNATIONAL EDITION,58(30),10241-10244.
MLA Wu, Yaqi,et al."Decorated Traditional Zeolites with Subunits of Metal-Organic Frameworks for CH4/N-2 Separation".ANGEWANDTE CHEMIE-INTERNATIONAL EDITION 58.30(2019):10241-10244.

入库方式： OAI收割

来源：大连化学物理研究所

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